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Modulating the Thermomechanical Properties and Self-Healing Efficiency of Siloxane-Based Soft Polymers Through Metal-Ligand Coordination

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01119C, Paper
Julia Pignanelli, Zhiyuan Qian, Xiaodan Gu, Mohammed Jalal Ahamed, Simon Rondeau-Gagné
Short oligomeric species end-capped with imine-based ligands can generate intrinsic autonomous self-healable soft polymer upon metal coordination, allowing for the preparation of materials that can be easily fine-tuned in terms...
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A first-principles study of the substitutional doping of MgCl2 monolayer for spintronics applications

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01264E, Paper
Igo Torres Lima, Railson Vasconcelos, Ricardo Gargano, Edson Nunes Costa Paura
Based on first-principles calculations, we studied the functionalization of MgCl2 monolayer with nonmetal (NM) and transition-metal (TM) atoms. Our results indicate that energetically it is more favorable to create a...
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Synergic effect of pore size engineering and an applied electric field on the controlled permeation of alkali metal atoms and ions across pristine and defect-containing h-BN sheets

New J. Chem., 2020, Advance Article
DOI: 10.1039/C9NJ03962G, Paper
Sajida Munsif, Naveen Kosar, Muhammad Ali Hashmi, Tariq Mahmood, Mazhar Amjad Gilani, Khurshid Ayub
Electric field facilitates the diffusion of Na and Li+.
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Ultrasonic Promoted Synthesis of Ag Nanoparticles Decorated Thiourea–Functionalized Magnetic Hydroxyapatite: A Robust Inorganic–Organic Hybrid Nanocatalyst for Oxidation and Reduction Reactions

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00829J, Paper
Saeed Bahadorikhalili, Hosein Arshadi, Zahra Afrouzandeh, Leila Ma'mani
In this research, ultrasonic synthesis is applied for the fabrication of a novel catalyst, based on immobilization of silver nanoparticles (AgNPs) on thiourea functionalized magnetic hydroxyapatite. Recoverable Ag nano–catalyst is...
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Multifunctional polymers with interpenetrating structures: luminescent sensing, ECL behaviors, selective detection of Fe3+ ion and rapid removal of anionic dyes

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01066A, Paper
Lingshu Meng, Lun Zhao, Guanlin Guo, Xin Liu
Three novel 3D coordination polymers (CPs), {[Cd(L)(bimb)](H2O)4}n (1), {[Zn(L)(bibp)](H2O)(DMF)}n (2) and {[Zn(L)(bif)](H2O)4}n (3) (bimb= 1,4-bis(imidazoly-1-yl)benzene, bibp= 4,4'-bis(imidazol-1-yl)biphenyl, bif= 2,7-bis(1-imidazoly)fluorene, H2L=1-(4-carbxoylphenyl)piperidine-4-caboylic acid) have been synthesized under solvothermal conditions. Compound 1 featured...
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Photoelectrocatalytic properties and mechanism of rhodamine B degradation using a graphene oxide/Ag3PO4/Ni film electrode

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00864H, Paper
Di Zhao, Fu-Cai Dai, Ai-Chang Li, Yu Chen, Gui-Hua Li, Qian Wang, Wen-Shuo Hou, Hong-Zhi Zhou
Graphene oxide (GO)/Ag3PO4/Ni composite film electrodes were prepared by composite electrodeposition using a mixture of ammonium phosphate and GO aqueous suspension as the electrolyte. The morphology, crystallinity, and optical characteristics...
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Nitrogen doped graphitic porous carbon from Almond Shell as an efficient persulfate activator for organic compounds degradation

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01148G, Paper
Zakaria Anfar, Abdellah Ait El Fakir, Hassan Ait Ahsaine, Mohamed Zbair, Salaheddine Farsad, Fabrice Morlet-Savary, Amane Jada, Noureddine El Alem
Here, we have developed a simple and efficient low-temperature process for doping N into graphitic porous carbon to prepare a catalyst: N-GPC. Almond Shell (AS) as Bio-sourced material was used...
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Catalytic oxidation mechanisms of carbon monoxide over single and double vacancy Mn-embedded graphene

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01500H, Paper
Mingming Luo, Zhao Liang, Mingwei Chen, Shaik Gouse Peera, Chao Liu, Hui Yang, Xiaopeng Qi, Juan Liu, Tongxiang Liang
Single-atom catalysts (SACs) have been extensively investigated in recent times due to their highly dispersed atomic levels and the improved distribution of their metallic active sites, maximizing the specific activity...
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Fabrication of a 3D self-supporting Ni–P/Ni2P/CC composite and its robust hydrogen evolution reaction properties in alkaline solution

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00727G, Paper
Fan Yang, Shuqin Yang, Qianqian Niu, Siyue Huo, Zimo Song, Laizhou Song
The Ni–P/Ni2P/CC composite exhibits excellent alkaline HER properties derived from Ni–P filling the sites on the CC not occupied by Ni2P nanosheets.
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A nickel molybdenum oxide nanoarray as an efficient and stable electrocatalyst for overall water splitting

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01232G, Paper
Xiaoshuang Zhang, Hui Su, Xiaoqiang Du
Experimental and DFT calculation results show that the presence of oxygen vacancies can decrease the adsorption energy of intermediates at active sites and facilitate their adsorption, thus improving the catalytic properties.
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Catalytic transfer hydrogenation of biomass-derived levulinic acid to γ-valerolactone over Sn/Al-SBA-15 catalysts

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01288B, Paper
Sakthivel Kumaravel, Sivakumar Thiripuranthagan, Mani Durai, Elangovan Erusappan, Thanigaivel Vembuli
The synthesized inexpensive catalysts show high catalytic transfer hydrogenation activity at ambient N2 pressure under non-corrosive conditions. The Sn/Al-SBA-15 (25) catalyst exhibited the highest catalytic activity with 99% conversion of levulinic acid and 100% selectivity towards GVL.
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Narrow bandgap difluorobenzochalcogenadiazole-based polymers for high-performance organic thin-film transistors and polymer solar cells

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01006E, Paper
Shengbin Shi, Qiaogan Liao, Hang Wang, Guomin Xiao
A series of difluorobenzochalcogenadiazole-bithiophene copolymers are developed for high-performance organic semiconductors.
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Unraveling the helianane family: a complementary quantum mechanical study

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01396J, Paper
Lucas H. Martorano, Alessandra L. Valverde, Carlos Magno R. Ribeiro, Ana Carolina F. de Albuquerque, José Walkimar de M. Carneiro, Rodolfo G. Fiorot, Fernando M. dos Santos Junior
Comprehensive work suggesting the amendment of helianane to the open ring curcudiol by means of computational spectroscopy and thermodynamic reasons.
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Water-soluble poly(N-isopropylacrylamide) nanoparticles grafted to trivalent lanthanide complexes as highly sensitive ratiometric nanothermometers

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01263G, Paper
Josiane Aparecida Sobrinho, Gilmar Araújo Brito Júnior, Italo Odone Mazali, Fernando Aparecido Sigoli
A new water-soluble, luminescent ratiometric nanothermometer with a tunable temperature-responsive range, high thermal sensitivity and good repeatability was designed and synthesized by grafting lanthanide complexes to pNIPAM polymeric nanoparticles.
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Oligoaniline-functionalized polysiloxane/Prussian blue composite towards bifunctional electrochromic supercapacitors

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00736F, Paper
Yanyan Wang, Xiaoteng Jia, Meihua Zhu, Xincai Liu, Danming Chao
We report the preparation of a novel oligoaniline-functionalized polysiloxane/Prussian blue composite, which exhibits improved electrochromic properties and approving supercapacitor performance featuring charge storage indicating functionalization.
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Hydroamination of isocyanates and isothiocyanates by alkaline earth metal initiators supported by bulky iminopyrrolyl ligand

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01509A, Paper
Tarun Kanti Panda, Kulsum Bano, Srinivas Anga, Archana Jain, Hari Pada Nayek
A series of new heteroleptic alkaline earth (Ae) metal complexes of general formula [{(Ph2CHN=CH)2C4H2N}AeI(THF)3] {Ae = Ca (2), Sr (3), and Ba (4)} were synthesized via salt metathesis by reacting...
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Application of Modifier-free Gold Nanoparticle Colorimetric Sensing for Rapid Screening and Detecting Vitamin B1

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01401J, Paper
Paweenar Duenchay, Kantima Kaewjua, Orawon Chailapakul, Weena Siangproh
In this report, we present a transparency sheet-based colorimetric sensor as an alternative platform for the simple, sensitive and selective determination of vitamin B1 in urine samples by using unmodified...
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Facile functionalization of boron nitride (BN) for the development of high-performance asymmetric supercapacitors

New J. Chem., 2020, Advance Article
DOI: 10.1039/C9NJ06284J, Paper
Chandan Kumar Maity, Sumanta Sahoo, Kartikey Verma, Ajaya Kumar Behera, Ganesh Chandra Nayak
Ternary composites based on functionalized BN, a carbonaceous material, and PANI are developed for real-time asymmetric supercapacitor application.
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Synthesis of eight isostructural 2D lanthanide coordination polymers assembled by rigid furan-2,5-dicarboxylic acid and flexible adipic acid as linkers and exploration of luminescent Eu/Tb polymers as efficient and sensitive sensors for nitroaromatic comp

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ01018A, Paper
Zaib ul Nisa, Lobzang Tashi, Charanjeet Sen, Nargis Akhter Ashashi, Subash Chandra Sahoo, Haq Nawaz Sheikh
Eight isostructural coordination polymers were synthesized by a solvothermal method. The luminescent Eu/Tb polymers function as efficient sensors for nitroaromatics via turn-off mode.
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Novel nitro substituted formazan derivatives: Selective ratiometric and colorimetric chemosensors for fluoride anion sensing detectable by the naked eye

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01860K, Paper
Gulsen Turkoglu
Novel two formazan derivatives FNB and FDNB were synthesized from their corresponding phenylhydrazone and characterized by various spectroscopic methods. The sensing ability of these formazan sensors towards different anions was...
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Synthesis of a new Ni complex supported on CoFe2O4 and its application as an efficient and green catalyst for the synthesis of bis(pyrazolyl)methane and polyhydroquinoline derivatives

New J. Chem., 2020, Advance Article
DOI: 10.1039/D0NJ00223B, Paper
Taiebeh Tamoradi, Seyedeh Masoumeh Mousavi, Masoud Mohammadi
A novel and magnetic nanocatalyst was synthesized for the synthesis of multicomponent compounds.
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Fast and easy conversion of ortho amidoaryldiselenides into the corresponding Ebselen-like derivatives driven by theoretical investigations.

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01605E, Paper
Vanessa Nascimento, Pâmella da Silva Cordeiro, Massimiliano Arca, Francesca Marini, Luca Sancineto, Antonio Luiz Braga, Vito Lippolis, Michio Iwaoka, Claudio Santi
DFT calculations performed on amidoaryldiselenides as electrophilic derivatives evidenced the presence of a prevalent Se···O weak interaction when selenium is bonded to a Se atom (diselenides), a Br atom (selenenyl...
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Linear dicarboxylate based pyridyl appended cobalt(II) coordination polymers in search of opto-electronic properties

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00567C, Paper
Faruk Ahmed, Joydeep Datta, Samim Khan, Basudeb Dutta, Sakhiul Islam, Sanobar Naaz, Partha Pratim Ray, Mohammad Hedayetullah Mir
Two new coordination polymers (CPs) [Co(adc)(4-ppy)(H2O)2]n, (1) and [Co(adc)(4-bppy)(H2O)2]n, (2) (H2adc = acetylenedicarboxylic acid, 4-ppy = 4-phenylpyridine and 4-bppy = 4-(4-bromophenyl)pyridine) have been synthesized and characterized by various techniques including...
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Conjugated Small Organic Molecules: Synthesis and Characterization of 4- Arylpyrazole-decorated Dibenzothiophenes

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01887B, Paper
M. Bhanuchandra, Satyajit Panda, Ram Singh Jat, Amir Fayaz, Jony Saha, Ramalingam Thirumoorthi , Tapta Kanchan Roy
4-Arylpyrazole-decorated dibenzothiophenes have been synthesized. The synthesis involves the treatment of 2,8-dibromodibenzothiophene with pyrazole under Ullmann-type amination conditions for the dual C-N bond formation. The selective bromination of the resulting...
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Novel phthalocyanine-based micelles/PNIPAM composite hydrogels: spatial/temporal-controlled drug release triggered by NIR laser irradiation

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01882A, Letter
Tao Jia, Lu Li, Enna Ha, Zheng Qu, Lei Shi, Tiedong Sun, Shengnan Tan, Wancheng Zhao
Near-infrared (NIR) light-responsive hydrogels hold significant potential for biomedical application, especially in remote-controlled release of anticancer drugs. Herein we report a novel NIR light responsive composite hydrogel system that undergoes...
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Construction and application of nonenzymatic ascorbic acid sensor based on NiO1.0/polyaniline3.0 hybrid

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ00696C, Paper
shichao Zhu, Aijuan Xie, Bingyan Wei, Xiang Tao, Jianghui Zhang, Wenhao Peng, Chenyang Liu, Linyang Gu, Chenfei Xu, Shiping Luo
NiO1.0/PANI3.0 was prepared by in-situ polymerization method in one-pot and applied in detection of ascorbic acid (AA). Cyclic voltammetry (CV) and Differential pulse voltammetry (DPV) were used to optimize the...
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Facile assemble of 2D α-zirconium phosphate supported silver nanoparticles: superior and recyclable catalysis

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01378A, Paper
Yonghang Xu, Fangya Zhou, Min Chen, Huawen Hu, Limiao Lin, Jingshu Wu, Min Zhang
A novel, efficient and durable ZrP@PDA/Ag nanocatalyst was prepared via facile reduction and deposition of silver nanoparticles (AgNPs) on two dimensional (2D) α-zirconium phosphate (ZrP) nanosheets using bio-inspired dopamine chemistry....
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Cu(II)Cl2 Containing Bispyridine-based Porous Organic Polymer Support Prepared via Alkyne-Azide Cycloaddition as a Heterogeneous Catalyst for Oxidation of Various Olefins

New J. Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0NJ01174F, Letter
Jong Ho Yoon, Hye Min Choi, Suk Joong Lee
New class of porous organic polymer (POP) based heterogeneous catalyst Cu-POP was prepared from immobilizing Cu(II)Cl2 into bpy containing POP prepared via alkyne-azide cycloaddition. This new catalyst showed efficient catalytic...
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The Burning Room

Harry Bosch has a new partner.




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[ASAP] Potentiation of Antibiotics against Gram-Negative Bacteria by Polymyxin B Analogue SPR741 from Unique Perturbation of the Outer Membrane

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.9b00159




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[ASAP] Broadening Activity of Polymyxin by Quaternary Ammonium Grafting

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.0c00037




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[ASAP] A Chemically Stable Fluorescent Mimic of Dihydroartemisinin, Artemether, and Arteether with Conserved Bioactivity and Specificity Shows High Pharmacological Relevance to the Antimalarial Drugs

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.9b00430




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[ASAP] Discovery of Cephalosporin-3'-Diazeniumdiolates That Show Dual Antibacterial and Antibiofilm Effects against <italic toggle="yes">Pseudomonas aeruginosa</italic> Clinical Cystic Fibrosis Isolates and Efficacy in a Murine R

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.0c00070




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[ASAP] <italic toggle="yes">Plasmodium falciparum</italic> Artemisinin Resistance: The Effect of Heme, Protein Damage, and Parasite Cell Stress Response

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.9b00527




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[ASAP] Intracellular Metal Speciation in <italic toggle="yes">Streptococcus sanguinis</italic> Establishes SsaACB as Critical for Redox Maintenance

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.0c00132




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[ASAP] <italic toggle="yes">Leishmania infantum</italic> Enhances Migration of Macrophages via a Phosphoinositide 3-Kinase ?-Dependent Pathway

ACS Infectious Diseases
DOI: 10.1021/acsinfecdis.0c00080




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Snips and snails and puppy-dogs’ tails

It’s that time of year again. March 23rd marks National Puppy Day! Founded in 2006 by Colleen Paige, National Puppy Day educates the public about the atrocities of puppy mills, and helps save orphaned puppies around the world. Although some of these four-legged poseurs below are well past puppyhood, we couldn’t wait until National Dog Day...

The post Snips and snails and puppy-dogs’ tails appeared first on New-York Historical Society.




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Wiring Manhattan: Sterling Communications and Cable Television in New York City

Between 1945 and 1960 the number of television sets in use in the United States rose from a few thousand to approximately 60 million. Although many of the programs shown originated in New York City, many of Gotham’s denizens had to endure a steadily degrading signal reception. The cause: new buildings in the vertically growing...

The post Wiring Manhattan: Sterling Communications and Cable Television in New York City appeared first on New-York Historical Society.




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Highway to Hell: Tensions in the La Guardia Administration

Despite the effects of the Great Depression, the City Planning Commission under Mayor Fiorello La Guardia reported for the period 1920–1939 a staggering increase in New York City motor vehicle registrations from 225,000 to nearly one million. As a result of the evolving needs of constituents, and with a glimmering post-war economic boom on the horizon,...

The post Highway to Hell: Tensions in the La Guardia Administration appeared first on New-York Historical Society.




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A Cabinet Staff of Cutthroats, Picaroons, and Nincumpoops

We are upon a new year and a new political season, as recently-elected governors and legislators take their oaths and move into their offices. Hiring staff is always the first task at hand.  Does one “clean house” of the holdovers or retain them? This question may have had its most relevance in the early American...

The post A Cabinet Staff of Cutthroats, Picaroons, and Nincumpoops appeared first on New-York Historical Society.




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Mercury, Sulphur and Vitriol: A Colonial Physician’s Accounts

Harry Potter may have come and gone here at the New-York Historical Society but it turns out that the interplay of magic and science that enlivens the Potter series can still be found in the Historical Society’s collections. On this occasion, it emerges from an unidentified colonial physician’s account book. Although it’s generally written in legible scripts, the...

The post Mercury, Sulphur and Vitriol: A Colonial Physician’s Accounts appeared first on New-York Historical Society.




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A Centennial Salute to the Daily News

People like to say that the daily newspaper is dying, but, as you pass a newsstand and glance at a headline, do not take those tabloids for granted. We pause here to wish the New York Daily News a happy birthday on its centennial. The Illustrated Daily News first appeared on the morning of June...

The post A Centennial Salute to the Daily News appeared first on New-York Historical Society.




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Highlights from the Bill Cunningham “Facades” Photograph Collection

September in New York City marks the beginning of the fall season, but the fashion industry is already looking ahead towards spring with the showcasing of Spring/Summer 2020 collections at New York Fashion Week (NYFW). To celebrate the start of a new fashion season, we’re highlighting the work of world famous fashion photographer, Bill Cunningham...

The post Highlights from the Bill Cunningham “Facades” Photograph Collection appeared first on New-York Historical Society.




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The Battle of Golden Hill: New York’s Opening Act of Revolutionary Bloodshed

New Yorkers and Bostonians have a number of things to dispute—Yankees versus Red Sox, Manhattan versus New England clam chowder, good or bad memories of the Super Bowl in 2008 and 2012. We will avoid adding, “Where was the first blood of the American Revolution shed?” as another. Yes, we concede the Boston Massacre of...

The post The Battle of Golden Hill: New York’s Opening Act of Revolutionary Bloodshed appeared first on New-York Historical Society.




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Benjamin Franklin’s Plan for Unification

Twenty years before the United States declared its independence from Great Britain, a group of colonial representatives from nine colonies met in Albany, New York during the onset of the French and Indian War. The Albany Congress of 1754 brought together colonial and Indigenous leaders in an attempt to strengthen relations while defending the northern...

The post Benjamin Franklin’s Plan for Unification appeared first on New-York Historical Society.




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Changes in Trends in Thyroid Cancer Incidence in the United States, 1992 to 2016

This study uses Surveillance, Epidemiology, and End Results (SEER) registry data to describe trends in thyroid cancer incidence overall and by tumor size in the United States from 1992 to 2016.




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Help Send Mathematica Staff and Our Community Partners to SXSW EDU

Mathematica staff and their local community partners are vying for an opportunity to share insights from cutting-edge projects related to equity, early learning, the science of learning, and K–12 education.




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Mathematica Marks National Rural Health Day: Pennsylvania Rural Health Model Drives Payment Innovation

The National Organization of State Offices of Rural Health sets aside the third Thursday of every November—this year, it’s November 21—to celebrate National Rural Health Day.




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New Toolkit Highlights How Medicare Accountable Care Organizations Engage Beneficiaries

Under a contract with the Centers for Medicare & Medicaid Services (CMS), Mathematica’s health experts worked with 24 Medicare Accountable Care Organizations (ACOs) and End-Stage Renal Disease (ESRD) Seamless Care Organizations participating in the Shared Savings Program, Next Generation ACO Model, and the Comprehensive ESRD Care Model to identify the strategies that ACOs use to engage beneficiaries in their care.




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Howard University and Mathematica to Host Computational Social Science Summer Institute

Mathematica and Howard University have partnered to host the Summer Institute in Computational Social Science (SICSS), which will give social and data scientists opportunities to explore how they can use real-world data to address ethics and equity in artificial intelligence.