Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00292J, Paper

Jinkai Hu, Chenglei Yang, Xiaotao Qin, Hui Liu, Tongtong Ma, Ao-tong Shi, Qing-Long Lv, Xingman Liu, Jinhui Yang, Dianjun Li
A visible light-enabled photocatalyst-free radical trihalomethylation/cyano (or benzo[d]thiazol-2-yl) 1,4-migration/carbonylation reaction of 2-hydroxy-2-hex-5-enenitrile (or (benzo[d]thiazol-2-yl)-pent-4-enol) with CX₃SO₂Cl (X = F, Cl) is reported.
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Org. Biomol. Chem., 2024, 22,2992-3000
DOI: 10.1039/D4OB00234B, Paper

Kimberly S. Taylor, Madison M. McMonagle, Schaelee C. Guy, Ariana M. Human-McKinnon, Shumpei Asamizu, Heidi J. Fletcher, Bradley W. Davis, Takashi L. Suyama
An organo–ruthenium catalyst conjugated to albumin efficiently unmasks an alloc group under physiologically relevant conditions.
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Org. Biomol. Chem., 2024, Accepted Manuscript
DOI: 10.1039/D4OB00160E, Paper

João Pedro Albuquerque Souza, Amanda Krauskopf Jacobs, Leandro Piovan, Renan Borsoi Campos
The energetic viability of several mechanistic variations of the reductive amination of acetophenones via the Borch approach was reexamined through density functional theory calculations. The crucial involvement of the acid...
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Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00171K, Review Article

Bor-Cherng Hong, Ranadheer Reddy Indurmuddam
This review summarizes recent developments in visible-light or near-visible-light photocatalysis reactions enabled by the TBADT catalyst.
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Mater. Chem. Front., 2024, 8,3634-3642
DOI: 10.1039/D4QM00366G, Research Article

Junjie Wang, Bo Wang, Xinmeng He, Jun Lv, Zhiyong Bao, Jiewu Cui, Guangqing Xu, Wangqiang Shen
NiS_x nanoparticles enhance Si substrate's hydrogen evolution to 189.15 μmol h⁻¹ cm⁻², outperforming Ni/SiNWs by 3.04 times and pristine SiNWs by 30.86 times.
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Mater. Chem. Front., 2024, 8,3558-3568
DOI: 10.1039/D4QM00800F, Research Article

Open Access

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Elisabetta Grazia Tomarchio, Chiara Zagni, Vincenzo Paratore, Guglielmo Guido Condorelli, Sabrina Carola Carroccio, Antonio Rescifina
A phenylalanine-based palladium catalyst was developed for the Suzuki–Miyaura reaction, preventing palladium leaching. It demonstrated high yield (up to 99%) in aqueous media and can be reused up to seven times, making it scalable for industrial use.
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Mater. Chem. Front., 2024, 8,3741-3746
DOI: 10.1039/D4QM00555D, Research Article

Jiejie Ping, Mei Wu, Manyu Liu, Yan Jiang, Wenhui Shang, Menggai Jiao, Jiahao Ruan, Nan Wang, Zhiyu Jia
Porphyrin-linked graphdiyne anchored with transition metals exhibits outstanding electrochemical performance, attributed to the modifications in the coordination environment.
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Mater. Chem. Front., 2024, Accepted Manuscript
DOI: 10.1039/D4QM00798K, Research Article

Jin Li, Wei Zhang, Xiujing Xing, Yaokang Lv, Renliang Lyu, Wei Xiong, Hao Li
Gold nanoparticles are extensively employed in the field of electrocatalytic nitrite reduction for ammonia synthesis, due to their exceptional conductivity and remarkable stability. However, the properties of a single metal...
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Nanoscale Horiz., 2024, Accepted Manuscript
DOI: 10.1039/D4NH00424H, Communication

Liang Xie, Wei Zhou, Zhibin Qu, Yuming Huang, Longhao Li, Chaowei Yang, Junfeng Li, Xiaoxiao Meng, Fei Sun, Jihui Gao, Guangbo Zhao
M-N₄-C single-atom catalysts (MN₄) have gained attention for their efficient use at the atomic level and adjustable properties in electrocatalytic reactions like ORR, OER, and HER. Yet, understanding MN₄'s activity...
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J. Mater. Chem. A, 2024, 12,30279-30288
DOI: 10.1039/D4TA04014G, Paper

Kotaro Ishihara, Akinobu Nakada, Hajime Suzuki, Osamu Tomita, Shunsuke Nozawa, Akinori Saeki, Ryu Abe
Function-/site-selective hybridisation of two specific Ru(II) complex catalysts on donor–acceptor conjugated polymers enables bifunctional visible-light water oxidation and CO₂ reduction.
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J. Mater. Chem. A, 2024, 12,30676-30684
DOI: 10.1039/D4TA05099A, Paper

Yangfan Liu, Yejun Li, Xinghan Liu, Jinming Li, Gufei Zhang, Jun Gong, Yanbin Jiang, Zhou Li
A synergistic adsorption mechanism of the oxygen evolution reaction for the dual atom catalysts (DACs) was proposed, which dominates the adsorption strength of intermediate species, potential determining step, and catalytic activity of DACs.
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J. Mater. Chem. A, 2024, 12,30498-30507
DOI: 10.1039/D4TA05741D, Paper

Yandi Zhu, Weihu Li, Xiaoyan Ren, Lili Zhang, Xingju Zhao, Shunfang Li
Transition metal single-atom catalysts (TM = Mn, Zr, Nb, Mo, Hf, Ta, and W) promote growth of a h-BN-G heterostructure on C-dimer-unpreferred Rh(111).
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J. Mater. Chem. A, 2024, 12,30522-30533
DOI: 10.1039/D4TA05436A, Paper

Open Access

  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.

Basundhara Dasgupta, Suptish Ghosh, Carsten Walter, Markus S. Budde, Georg J. Marquardt, Han-Hsu Chen, Markus G. M. Breithaupt, Tolga Yilmaz, Christoph Garmatter, Tamanna Ahamad, Ingo Zebger, Matthias Driess, Prashanth W. Menezes
A nanocrystalline Co₉S₈ (pre)catalyst derived from a novel {Co^IIS₄} complex is reported for the oxygen evolution reaction (OER) and selective biomass valorization. During OER, Co₉S₈ reconstructs completely into a CoOOH active phase via S-leaching.
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J. Mater. Chem. A, 2024, 12,30722-30728
DOI: 10.1039/D4TA05018E, Paper

Jun Zhu, Mengdan Song, Qiling Qian, Yang Yue, Guangren Qian, Jia Zhang
Machine learning deconstructed the atomic contribution of a perovskite to catalytic toluene decomposition and found that wider hybridization resulted in smaller impedance, faster electron transfer speed, and enhanced catalytic activity.
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J. Mater. Chem. A, 2024, 12,30798-30809
DOI: 10.1039/D4TA04194A, Paper

Manigandan Ramadoss, Hesheng Yu, Anand Rajkamal, Gun Jin Yun, Ziheng Zhang, Chengtao Yang, Fei Ma, Yu Wu, Chen Daiqian, Yuanfu Chen
Fe-single-atom-coupled Fe₃C multifunctional catalysts on P-, F-, N-doped CNT deliver comparable OER behavior to RuO₂, better ORR performance than Pt/C, and better ZAB performance than Pt/C–RuO₂, due to the nanoarchitecture and abundant active sites.
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J. Mater. Chem. A, 2024, 12,30692-30706
DOI: 10.1039/D4TA05801A, Paper

Yunshuo Wu, Haiqiang Wang, Zhongbiao Wu
The development of catalysts with high-density interfacial sites is crucial for enhancing catalytic performance.
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J. Mater. Chem. A, 2024, 12,30810-30820
DOI: 10.1039/D4TA05985A, Paper

Anubha Rajput, Ankita Kumari, Hirak Kumar Basak, Dibyajyoti Ghosh, Biswarup Chakraborty
MnMoO₄ is a barely explored material for the electrocatalytic oxygen evolution reaction (OER) and in situ tracking of the reactive intermediates and final active species during the OER in an alkaline pH lacks a sequential study.
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J. Mater. Chem. A, 2024, 12,30885-30891
DOI: 10.1039/D4TA03559C, Paper

Vasilis Nikolaou, Deborah Romito, Clément Maheu, Jonathan Hamon, Eric Gautron, Florian Massuyeau, Pierre-Emmanuel Petit, Stéphane Jobic, Fabrice Odobel
The first use of the successive ionic layer adsorption and reaction (SILAR) method to grow CdS quantum dots on TiO₂ nanoparticles, achieving efficient photocatalytic alcohol oxidation and H₂ evolution without catalysts or sacrificial donors.
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J. Mater. Chem. A, 2024, 12,30269-30278
DOI: 10.1039/D4TA06794K, Paper

Dong Hyeon Lee, Rahul Kerkar, Deepak Arumugam, Jayaraman Theerthagiri, Shankar Ramasamy, Soorathep Kheawhom, Myong Yong Choi
This study introduces a NiFe LDH-based catalyst via pulsed laser irradiation in liquids and microwave methods, achieving superior oxygen evolution performance. In situ electrode casting optimizes the catalyst for water-splitting applications.
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J. Mater. Chem. A, 2024, 12,30409-30419
DOI: 10.1039/D4TA05443A, Paper

Yue Cao, Shengbo Yuan, Wenbo Zhou, Yan Hai, Xiaoman Li, Min Luo
NO₃⁻ and H₂O molecules adsorbed on the surface of Co–N–C-500 are activated and dissociated. The generated active hydrogen species (*H) can promote the hydrogenation of the intermediates and thus increase the NH₃ yield.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06650B, Paper

Shiyao Li, Honghao Chen, Yue Qiu, Chengxing Cui, Wenhui Zhong, Jun Jiang
As the first attempt to reveal the intrinsic relationship between electron spins and catalytic selectivity, this work offers new insights into the rational design of efficient transition metal atom-dispersed catalysts through spin regulation.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06515H, Communication

Hefeng Wang, Zixiao Li, Zhengwei Cai, Chaoxin Yang, Shengjun Sun, Xiaoyan Wang, Min Zhang, Meng Yue, Dongdong Zheng, Asmaa Farouk, Mohamed S. Hamdy, Xuping Sun, Bo Tang
Ir nanoparticle decorated NiFe metal–organic framework on Ni foam (Ir@NiFe-MOF/NF) acts as a bifunctional catalyst for the oxygen evolution reaction and the hydrogen evolution reaction in alkaline seawater with excellent performance and stability.
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06592A, Paper

Jingwei Wang, Lejuan Cai, Zhipeng Yu, Hao Tan, Xinyi Xiang, Kaiyang Xu, Yang Chao, Sitaramanjaneya Mouli Thalluri, Fei Lin, Haoliang Huang, Chenyue Zhang, Yang Zhao, Wenlong Wang, Lifeng Liu
Proton exchange membrane water electrolysis (PEMWE) is considered a promising technology for green hydrogen production in combination with renewable energy. However, the high cost and particularly the scarcity of iridium...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06468B, Review Article

Hansai Wu, junming Zhang, Zicong Wang, Xianglong Kong, Gaofu Li, Ying Zhao, Piaoping Yang, Zhiliang Liu
N-ethylcarbazole (NEC) hydrogen storage has garnered significant attention owing to its large-scale safe storage of hydrogen superiority. However, the sluggish hydrogenation kinetics in NEC are extremely dependent on catalysts with...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06455K, Paper

Irlan Santos Lima, Josué M. Gonçalves, Lúcio Angnes
Catalysts capable of overcoming the bottleneck of water splitting, known as the oxygen evolution reaction (OER), are indispensable to the expansion of renewable energy systems. Thus, we report the synthesis...
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Chem. Soc. Rev., 2024, Advance Article
DOI: 10.1039/D3CS00967J, Review Article

Yuhang Liu, Xiaozhi Su, Jie Ding, Jing Zhou, Zhen Liu, Xiangjun Wei, Hong Bin Yang, Bin Liu
Single-atom catalysts (SACs) represent the ultimate size limit of nanoscale catalysts, combining the advantages of homogeneous and heterogeneous catalysts.
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Chem. Soc. Rev., 2024, 53,10620-10659
DOI: 10.1039/D4CS00217B, Review Article

Yiqiong Zhang, Jingjing Liu, Yangfan Xu, Chao Xie, Shuangyin Wang, Xiangdong Yao
This review focuses on the synthesis and characterization of defective electrocatalysts, the internal correlation between defects and catalytic activity, and the development and application of defective electrocatalysts in various catalytic fields.
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Mater. Horiz., 2024, 11,1719-1731
DOI: 10.1039/D3MH02115G, Communication

Liang Xie, Wei Zhou, Yuming Huang, Zhibin Qu, Longhao Li, Chaowei Yang, Yani Ding, Junfeng Li, Xiaoxiao Meng, Fei Sun, Jihui Gao, Guangbo Zhao, Yukun Qin
While current experimental and computational studies often concentrate on introducing external structures or idealized MN₄ models, we emphasize the often-overlooked impact of inherent OGs within the carbon structure of MN₄ materials, presenting a new perspective on their catalytic activity origin.
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Mater. Horiz., 2024, 11,1769-1778
DOI: 10.1039/D3MH01945D, Communication

Neng Li, Zhongyong Zhang, Zheng Wang, Bin Liu, Deyong Zhou, Xing Zhou, Peng Zhang, Xiujian Zhao
Gibbs free energy for electrocatalytic nitrogen reduction on Cr₂CO₂ with four magnetic states: NM, FM, Inter-AFM, and In-AFM.
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Mater. Horiz., 2024, 11,2032-2040
DOI: 10.1039/D3MH01909H, Communication

Jialei Yang, Zhenyu Yang, Jiafu Li, Hao Gang, Donghai Mei, Dongming Yin, Ruiping Deng, Yifeng Zhu, Xingyun Li, Ning Wang, Sameh M. Osman, Yusuke Yamauchi
A sub-nano interfacial catalytic structure is orchestrated by tailor-designing a hollow bowl-like porous carbon-confined Ru–MgO hetero-structured nanopair as a high-performance catalyst for ammonia borane hydrolysis.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D3MH01951A, Communication

Qingxin Han, Qiangqiang Lu, Xuechuan Wang, Chao Wei, Xiaoyu Guan, Luming Chen, Xiao Wang, Ji Li
Chrome shavings produce electrocatalysts with atomically dispersed Ru sites. The CN/Cr₂O₃/Ru-1 catalyst has excellent HER catalytic performance under the synergistic effect of RuN₄ and Cr₂O₃.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D4MH00285G, Communication

Mengting Liu, Wanyu Zhang, Ruiting Ni, Zhenxiao Wang, Hongyao Zhao, Xiu Zhong, Yanyun Wang, Danhong Shang, Zengjing Guo, Edison Huixiang Ang, Fu Yang
Novel metallic Co integration onto MnO nanorods enhances catalyst efficiency for wastewater treatment.
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Inorg. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QI00255E, Review Article

Xunhuai Huang, Junpeng Song, Guanyu Wu, Zhihuan Miao, Yanhua Song, Zhao Mo
Modification strategy and synthesis method of a metal sulfide-mediated carbon nitride photocatalytic H₂ production system.
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Inorg. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QI00458B, Research Article

Liangjun Chen, Zhuowen Huangfu, Xuelin Yang, Hang Lei, Zilong Wang, Wenjie Mai
This study presents a methodology that enables the development of efficient and scalable ZIF-derived electrocatalysts for industrial water electrolysis, resulting in significant time and energy savings.
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Inorg. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QI00262H, Research Article

Xinyi Wang, Jing Jin, Zeyuan Gao, Li Hou, Xiwen Tao, Jing Wang, Yueqi Zhao, Faming Gao
Two-dimensional (2D) molybdenum disulfide (MoS₂) with a large surface area and unique electronic properties has emerged as a promising noble metal-free catalyst for electrochemical energy storage/conversion applications.
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Inorg. Chem. Front., 2024, 11,2319-2338
DOI: 10.1039/D3QI02499G, Research Article

Open Access

  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.

Marco Pietro Mezzapesa, Fabio Salomone, Hilmar Guzmán, Federica Zammillo, Roberto Millini, Letizia Bua, Gianluigi Marra, Alessandra Tacca, Rosamaria Marrazzo, Nunzio Russo, Raffaele Pirone, Simelys Hernández, Samir Bensaid
Carbon dioxide (CO₂) hydrogenation to obtain valuable chemicals and fuels via thermocatalysis or electrocatalysis is a promising and sustainable method for CO₂ utilization.
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Inorg. Chem. Front., 2024, 11,2489-2497
DOI: 10.1039/D4QI00090K, Research Article

Haoran Yin, Shibiao Su, Di Yao, Lixia Wang, Xinqiang Liu, Tayirjan Taylor Isimjan, Xiulin Yang, Dandan Cai
An ultrathin NiFe LDH/MOF catalyst is grown on carbon paper by an in situ self-dissociation–assembly strategy. Studies reveal that the strong electronic interaction between Fe and Ni species with rich active sites results in good OER and OWS performance.
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Inorg. Chem. Front., 2024, 11,2479-2488
DOI: 10.1039/D4QI00145A, Research Article

Yiwei Zhao, Chao Zhang, Shuangxi Xing, Zuhang Jin, Tingting Xiao
ECO of HMF to FDCA and ECR to BHMF with high yield have been studied on CuNi-based bimetallic catalysts. The presence of the Cu–O–Ni interfacial area was beneficial for promoting the catalytic performance in ECO.
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Inorg. Chem. Front., 2024, Accepted Manuscript
DOI: 10.1039/D4QI00101J, Research Article

Qian Sun, Xiaoyu Hao, Tianyi Zhang, Zelin Ma, Kui Hu, Ming Yang, Xiaolei Huang, Xuqing Liu
Electrocatalytic water splitting stands at the forefront of advancing renewable energy technologies. A critical challenge in this realm is the detrimental effect of gas bubble adhesion on electrode surfaces, which...
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Chem. Sci., 2024, 15,18146-18160
DOI: 10.1039/D4SC05289G, Edge Article

Open Access

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Ewan McQueen, Noritaka Sakakibara, Kei Kamogawa, Martijn A. Zwijnenburg, Yusuke Tamaki, Osamu Ishitani, Reiner Sebastian Sprick
This highly efficient hybrid photocatalytic system can quantitatively convert CO₂ to formate and produce 0.4 M of formate solution without additional concentration enrichment.
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Chem. Sci., 2024, 15,18085-18092
DOI: 10.1039/D4SC03763D, Edge Article

Open Access

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Ruyu Xie, Kaitao Li, Rui Tian, Chao Lu
We have proposed an oxygen intermediate-boosted electrochemiluminescence probe for rapid spotting of the d-band centers of single-atom catalysts: the d-band centers closer to the Fermi level contributed to higher luminol ECL intensities.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC90219J, Correction

Open Access

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Tayyaba Najam, Syed Shoaib Ahmad Shah, Hanqing Yin, Xin Xiao, Shamraiz Talib, Qianqian Ji, Yonggui Deng, Muhammad Sufyan Javed, Jie Hu, Ruo Zhao, Aijun Du, Xingke Cai, Qiang Xu
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC03942D, Edge Article

Open Access

  This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence.

Darren Dolan, Rebekah Brucato, Christopher William Reid, Adam F. Lee, Karen Wilson, Adelina M Voutchkova-Kostal
Cleavage of lignin ether bonds via transfer hydrogenolysis is a promising route to valorize lignin, but processes that use mild reaction conditions and exploit renewable hydrogen donor solvents (rather than...
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RSC Med. Chem., 2024, 15,3444-3459
DOI: 10.1039/D4MD00318G, Research Article

Anuja Gracy Joseph, Mohanan Biji, Vishnu Priya Murali, Daisy R. Sherin, Alisha Valsan, Vimalkumar P. Sukumaran, Kokkuvayil Vasu Radhakrishnan, Kaustabh Kumar Maiti
Niloticin, a triterpenoid from Aphanamixis polystachya, induces apoptosis in HeLa cells which is primarily validated through in silico analysis and subsequently in vitro apoptotic evaluation by modulating the apoptotic proteins.
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