J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA07077A, Paper

Weisheng Zhang, Chen-Xing Zhang, Xianhe Chen, H.J. Yin, Wenli Hu, Shilin Mei, Chang-Jiang Yao
Sodium dual ion batteries (SDIBs) have received considerable attention recently for large-scale energy storage systems due to their low cost and inherent safety. Nevertheless, SDIBs remain a subject of investigation,...
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J. Mater. Chem. A, 2024, 12,30279-30288
DOI: 10.1039/D4TA04014G, Paper

Kotaro Ishihara, Akinobu Nakada, Hajime Suzuki, Osamu Tomita, Shunsuke Nozawa, Akinori Saeki, Ryu Abe
Function-/site-selective hybridisation of two specific Ru(II) complex catalysts on donor–acceptor conjugated polymers enables bifunctional visible-light water oxidation and CO₂ reduction.
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J. Mater. Chem. A, 2024, 12,30442-30453
DOI: 10.1039/D4TA03701D, Paper

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Samuel Emilsson, Göran Lindbergh, Mats Johansson
In an effort to increase the thermomechanical stability of lithium-ion battery separators, thermoset membranes (TMs) are a viable alternative to commercial polyolefin separators.
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J. Mater. Chem. A, 2024, 12,30508-30521
DOI: 10.1039/D4TA05908E, Paper

Abdul Basit, Yang-Chin Kao, Yasser A. El-Ossaily, Shiao-Wei Kuo, Mohamed Gamal Mohamed
The Py-Th-TzTz CMP was synthesized through a Schiff base reaction and exhibited a decomposition temperature (T_d10) of 352 °C. In a three-electrode system, it demonstrated a specific capacitance of 652 F g⁻¹.
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06028H, Review Article

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Febri Baskoro, Santosh U. Sharma, Andre Lammiduk Lubis, Hung-Ju Yen
Lithium-ion batteries stand at the forefront of energy storage technologies, facilitating the transition towards sustainable and electrified systems. To meet the increasing demands for energy density, safety, and longevity, the...
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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06242F, Paper

Tong Guan, Quan-Ao He, Shuang Chen
Poly(vinylidene fluoride-trifluoroethylene) [P(VDF-TrFE)] relaxor ferroelectrics have drawn a lot of attention nowadays due to their excellent multifunctionality and extensive applications. However, the microstructures behind their relaxor behaviors have not been...
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J. Mater. Chem. C, 2024, 12,17469-17474
DOI: 10.1039/D4TC03038A, Paper

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Suraya Kazi, Pravallika Bandaru, Haoran Tang, Yulong Duan, Shangzhi Chen, Fei Huang, Magnus P. Jonsson
We show that the n-type conducting polymer PBFDO can be optically metallic for wavelengths above around 695 nm after post-treatment, and that nanostructures of the material can act as optical nanoantennas that are dynamically switchable.
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J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC03668A, Paper

Shuyun Zhuo, Jie Jiang, Yaru Ma, Yiming Chen, Yue Zhao
Stimuli-triggered actuation and capability of sensing are two important prerequisites for self-sensing soft robots. Currently, liquid crystal polymer (LCP) based soft robots face difficulties in balancing the actuation and sensing...
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J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC04226C, Paper

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Nina Tverdokhleb, Biagio Audia, Pasquale Pagliusi, Marina Saphiannikova
This study aims to test and validate the modern orientation approach of Saphiannikova & co. within the context of viscoplastic photoalignment (VPA) modeling. We focus on the formation of topographical...
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J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC03666B, Perspective

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Megan M. Westwood, Bob C. Schroeder
The functionalisation of conjugated polymers with hydrogen bonding motifs, to impart self-healing or stretchability for wearable electronic applications. Through refinement of characterization techniques in recent years, the effect of these...
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D3MH02034G, Communication

Wei Ren, Haoning Li, Xiao Huang, Xiujing Xing, Guangming Yan, Jie Yang, Gang Zhang
We propose an innovative strategy that utilizes the space charge distribution characteristics of the co-monomer to solve the trade-off between optimizing the dielectric performance of polymers and maintaining the other comprehensive properties.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D3MH01641B, Review Article

Xuebing Li, Luohuizi Li, Dehui Wang, Jun Zhang, Kangfeng Yi, Yucai Su, Jing Luo, Xu Deng, Fei Deng
A systematic summary of fabrication technologies, a variety of structures and biomedical applications of polymeric microspheres.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D4MH00267A, Communication

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Latifah Almulla, Victor Druet, Christopher E. Petoukhoff, Wentao Shan, Nisreen Alshehri, Sophie Griggs, Yazhou Wang, Maryam Alsufyani, Wan Yue, Iain McCulloch, Frédéric Laquai, Sahika Inal
An n-type organic photoelectrochemical transistor produces large and reversible current changes in response to light-intensity variations in aqueous electrolytes. A long exciton lifetime of the n-type gate ensures a high photovoltage response.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D4MH00106K, Communication

Joshua O. Holloway, Laura Delafresnaye, Emily M. Cameron, Jochen A. Kammerer, Christopher Barner-Kowollik
Polymeric nanospheres can be synthesised within minutes using photo-flow chemistry, without the need for initiators, additives, or surfactants. The particles can be selectively degraded on demand, emitting light in the process.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D4MH00002A, Communication

Jianfeng Cheng, Xianhua Yao, Zhipeng Zhang, Yizhong Tan, Nan Hu, Chunfeng Ma, Guangzhao Zhang
Utilizing the modular construction strategy, intelligent anti-impact elastomers with varying topology network structures have been prepared by tailoring the stereoscopic and linear building blocks as independent modules.
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Mater. Horiz., 2024, 11,1843-1866
DOI: 10.1039/D3MH01585H, Review Article

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Soon Mo Park, Dong Ki Yoon
This review encapsulates recent progress in evaporation-induced self-assembly of liquid crystal biopolymers. It introduces various anisotropic structures of biopolymers in thin film and try to figure out the formation mechanism of the structures.
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Inorg. Chem. Front., 2024, 11,2471-2478
DOI: 10.1039/D4QI00233D, Research Article

Bingfeng Shi, Wanchao Hu, Shiyi Li, Zhinan Xia, Changli Lü
An efficient strategy is proposed to construct PQD/polymer organic–inorganic nanohybrids by PET-RAFT polymerization-mediated PISA and the nanohybrid assemblies can maintain excellent luminescence originating from PQDs with enhanced stability.
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Inorg. Chem. Front., 2024, 11,2300-2311
DOI: 10.1039/D4QI00391H, Research Article

Qiujun Wang, Xin He, Di Zhang, Zhaojin Li, Huilan Sun, Qujiang Sun, Bo Wang, Li-Zhen Fan
The introduction of Al₂O₃ regulates the solvation structure of Na⁺, which is conducive to the formation of inorganic-rich SEI. Na|THFA-5|Na cell maintains low polarization voltage, indicating that uniform Na depositions was successfully achieved.
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Inorg. Chem. Front., 2024, Accepted Manuscript
DOI: 10.1039/D4QI00200H, Research Article

Yong-Sheng Shi, Tong Xiao, Dong-Dong Yang, Xiangjun Zheng
A viologen derivative- and a carboxylic acid -based one-dimensional (1D) cocrystal Zn(Ⅱ) coordination polymer, {[Zn(bcbpy)2][Zn(sip)Cl]·4H2O}n (1, bcbpy = 1,1'-bis (3-carboxybenzyl)-4,4'-bipyridinium, sip = 5-Sulfoisophthalate) has been produced solvothermally and structurally characterized....
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC03942D, Edge Article

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Darren Dolan, Rebekah Brucato, Christopher William Reid, Adam F. Lee, Karen Wilson, Adelina M Voutchkova-Kostal
Cleavage of lignin ether bonds via transfer hydrogenolysis is a promising route to valorize lignin, but processes that use mild reaction conditions and exploit renewable hydrogen donor solvents (rather than...
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC05935B, Edge Article

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Yanbin Xu, Huangsheng Yang, Anlian Huang, Linjing Tong, Wei Huang, Guosheng Chen, Wei Yi, Siming Huang, Gangfeng Ouyang
A biocompatible polymer deposition-mediated surface-charge reformation strategy is reported that enables the in-place MOF biomineralization onto different enzyme templates.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC06012A, Edge Article

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Menglu Chen, Shuai You, Tingting Guo, Haohao Ren, Longzu Zhu, Peize Wang, Wenbo Sheng, Chenliang Gong, Wei Li
CuBr-mediated surface-initiated controlled radical polymerization for polymer brushes with patterned and block architectures over large areas in air is reported.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC06403H, Edge Article

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Dan-Dan Zhou, Chun-Li Hu, Xin-Wei Zhang, Jiang-Gao Mao, Fang Kong
Successful synthesis of centrosymmetric Ga(Te₃O₇)Br and non-centrosymmetric M₂(OH)(TeO₃)(Te₂O₅)X (M = Al, Ga; X = Br, Cl) using a depolymerization strategy.
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Chem. Sci., 2024, Advance Article
DOI: 10.1039/D4SC06083K, Edge Article

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Minhye Kim, Heekyoung Choi, Minjoo Kim, Seonghan Kim, Seohyeon Yun, Eunji Lee, Jaeheung Cho, Sung Ho Jung, Jong Hwa Jung
The modification of metalloligands based on bis-type amideterpyridine platinum(II) complexes not only induces the formation of helical supramolecular polymers but also introduces a kinetic trapping strategy in competitive conditions.
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC06902A, Edge Article

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August J. Rothenberger, Harrison M. Bergman, He Li, Miao Qi, Yunfei Wang, Yi Liu, T. Don Tilley
Conjugated ladder polymers (CLPs) are difficult yet captivating synthetic targets due to their fully unsaturated fused backbones. Inherent challenges associated with their synthesis often lead to low yields, structural defects,...
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC06466F, Edge Article

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Jiahui Lin, Zhiyuan Ma, Weiwei Zuo, Meifang Zhu
Porphyrin derivatives serve as photocatalysts in reversible-deactivation radical polymerization and as photosensitizers in photodynamic therapy (PDT). Herein, a triple function porphyrin, ZnTPPC6Br, was synthesized as photocatalyst and initiator for photoATRP....
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Chem. Sci., 2024, Accepted Manuscript
DOI: 10.1039/D4SC05891G, Edge Article

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Sophie Ellis, Antoine Buchard, Tanja Junkers
Poly(L-lactic acid) (PLLA) is commercially successful bio-based plastic, where end-of-life materials can undergo industrial composting. To create a circular economy, a desirable alternative to composting is chemical recycling to monomer...
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Lab Chip, 2024, 24,4962-4973
DOI: 10.1039/D4LC00485J, Paper

Sanjay S. Timilsina, XiuJun Li
A reusable and cost-effective paper-in-polymer-pond (PiPP) hybrid microfluidic microplate with unique features for ultrasensitive and high-throughput multiplexed detection of disease biomarkers within an hour without using specialized instruments.
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Anal. Methods, 2024, Advance Article
DOI: 10.1039/D4AY00146J, Paper

Dumei Ma, Yiting Luo, Xiaoya Zhang, Zehu Xie, Yinghua Yan, Chuan-Fan Ding
A fluorescence method based on Cu-triggered click reaction of azide modified CD63 aptamer and alkyne capped Pdots was developed for breast cancer derived exosome detection.
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Anal. Methods, 2024, Accepted Manuscript
DOI: 10.1039/D4AY00263F, Paper

Xinyao Wang, Guohua Cui, Rongning Liang, Wei Qin
Currently, Nernstian-response-based polymeric membrane potentiometric sensors using the molecularly imprinted polymers (MIPs) as the receptors have been successfully developed for determination of organic ionic species. However, the preparation of these...
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Anal. Methods, 2024, Accepted Manuscript
DOI: 10.1039/D4AY00251B, Paper

Ahmad Aqel, Ayman Ghafr, A. Yacine Badjah-Hadj-Ahmed, Zeid Abdullah ALOthman
Polymer monolithic stationary phases were prepared based on a cyclic anhydride as a reactive and tunable platform via ring-opening post-polymerization using primary amines; octadecylamine and benzylamine. The characterization techniques indicated...
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RSC Med. Chem., 2024, Advance Article
DOI: 10.1039/D4MD00541D, Research Article

Mikhail N. Anisimov, Maksim A. Boichenko, Vitaly V. Shorokhov, Julia N. Borzunova, Marina Janibekova, Vadim V. Mustyatsa, Ilya A. Lifshits, Andrey Yu. Plodukhin, Ivan A. Andreev, Nina K. Ratmanova, Sergey S. Zhokhov, Elena A. Tarasenko, Daria A. Ipatova, Alexander R. Pisarev, Ivan A. Vorobjev, Igor V. Trushkov, Olga A. Ivanova, Nikita B. Gudimchuk
New 1,5-disubstituted pyrrolidin-2-ones 1, 2 and 5-aryl-3,3a,4,5-tetrahydropyrrolo[1,2-a]quinoline-1(2H)-ones 3 were explored as inhibitors of tubulin polymerization.
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Soft Matter, 2024, 20,8291-8302
DOI: 10.1039/D4SM00830H, Paper

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Eman Alasadi, Carlos R. Baiz
Compared to bulk water, ions in confined environments or heterogeneous solutions can significantly disrupt hydrogen bond networks.
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Soft Matter, 2024, 20,8312-8325
DOI: 10.1039/D4SM00935E, Paper

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Brian K. Wilson, Robert K. Prud’homme
Composite nanoparticles co-encapsulate organic materials with inorganic primary colloids. Producing “stoichiometric NPs”, where all NPs contain organic and inorganic species at similar ratios, requires matched diffusion-aggregation time scale.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01040J, Paper

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Lorenzo Miele, Antonio Abate, Kentaro Taki, Ernesto Di Maio
The inverse pressure quenching treatment is proposed to decouple bubble nucleation from growth, advancing our understanding of the physics governing bubble growth and evolution in polymer foaming.
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Soft Matter, 2024, 20,8505-8514
DOI: 10.1039/D4SM00994K, Paper

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Conner H. Chee, Rotem Benharush, Lexi R. Knight, Jennifer E. Laaser
Complexes of strong polyelectrolytes prepared well above the binodal are shown to undergo hydrophobicity-driven segregative phase separation.
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Soft Matter, 2024, 20,8385-8394
DOI: 10.1039/D4SM00616J, Paper

D. A. Mitkovskiy, A. A. Lazutin, A. L. Talis, V. V. Vasilevskaya
Amphiphilic macromolecules grafted onto spherical nanoparticles can self-assemble into morphological structures corresponding to the family of complete embedded minimal surfaces. They arise situationally, can coexist and transform into each other.
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Soft Matter, 2024, 20,8493-8504
DOI: 10.1039/D4SM00721B, Paper

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Stephen Kronenberger, Nitant Gupta, Benjamin Gould, Colin Peterson, Arthi Jayaraman
We present a computational method to analyze 2D small-angle scattering data from three-phase soft materials systems with structural anisotropy and output representative real-space structures of the three phases.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00761A, Paper

Setarehalsadat Changizrezaei, Mikko Karttunen, Colin Denniston
A polymer confined in a nanochannel undergoes a crossover to a jammed state when pushed by a large spherical colloid. We examine the system using simulations that incorporate the full hydrodynamic driving and fluctuating forces.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00987H, Paper

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Sunilkumar Khandavalli, Jae Hyung Park, Robin Rice, Diana Y. Zhang, Sarah A. Berlinger, Guido Bender, Deborah J. Myers, Michael Ulsh, Scott A. Mauger
Steady-shear rheology showing evolution of the microstructure of iridium oxide catalyst inks of PEM water electrolyzers with aging time.
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Soft Matter, 2024, 20,8663-8674
DOI: 10.1039/D4SM00578C, Paper

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L. V. Tiihonen, M. P. Weir, A. J. Parnell, S. C. Boothroyd, D. W. Johnson, R. M. Dalgliesh, M. Bleuel, C. P. Duif, W. G. Bouwman, R. L. Thompson, K. S. Coleman, N. Clarke, W. A. Hamilton, A. L. Washington, S. R. Parnell
Spin-echo small-angle neutron scattering (SESANS) revealed structure in polymer–carbon nanocomposites over multiple length scales with unprecedented range (10 nm–16 μm). Data from two SESANS instruments and other methods were analysed with SasView.
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Soft Matter, 2024, 20,8589-8600
DOI: 10.1039/D4SM00084F, Paper

Akihiro Ohara, Ko Okumura
We constructed a theory and method for measuring the compressive modulus by combining tensile and bending tests. Elastic asymmetry was confirmed in an industrial PET film.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00837E, Paper

Temitope Orimolade, Ngoc-Tram Le, Lyle Trimble, Bandaru Ramarao, Sitaraman Krishnan
Algal flocculation using alum shows dynamic fractal restructuring over time, while Moringa oleifera protein induces faster densification, enhancing floc strength.
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Soft Matter, 2024, 20,8549-8560
DOI: 10.1039/D4SM01053A, Review Article

Ruslan Kashapov, Yuliya Razuvayeva, Elena Fedorova, Lucia Zakharova
Supramolecular self-assembly of polymers with macrocycles has attracted the attention because it enables the spontaneous creation of nanostructures with unique properties.
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM01098A, Communication

Léo Hervéou, Gauthier Legrand, Thibaut Divoux, Guilhem Pablo Baeza
The present work emphasizes the relevance of low-field NMR relaxometry to investigate colloid-polymer hydrogels by probing water dynamics across a wide range of formulations between 10°C and 80°C. By examining...
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00968A, Paper

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Zahra Valei, Karolina Wamsler, Alex J Parker, Therese A Obara, Alex Klotz, Tyler Nathan Shendruk
Polymers are a primary building block in many biomaterials, often interacting with anisotropic backgrounds. While previous studies have considered polymer dynamics within nematic solvents, rarely are the the effects of...
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00977K, Paper

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Shin-nosuke Nishimura, Naoya Kurahashi, Shohei Shiomoto, Yoshihisa Harada, Masaru Tanaka
Given that the hydration water of polymer matrices may differ from that of outermost polymer surfaces, processes at biomaterial–biofluid interfaces and role of hydration water therein cannot be adequately examined...
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Org. Chem. Front., 2024, Advance Article
DOI: 10.1039/D4QO01382D, Research Article

Ajay Kumar Sahoo, Parag Tamuly, Jarugu Narasimha Moorthy
An IPOP, constructed constructed from cyanuric chloride and the readily accessible 2,5-di(pyridin-4-yl)thiazolo[5,4-d]thiazole (BpyTzTz), is shown to exhibit excellent visible light absorption and serve as a metal-free heterogeneous photocatalyst.
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Org. Chem. Front., 2024, Accepted Manuscript
DOI: 10.1039/D4QO01848F, Research Article

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Tobias B. Tischer, Zulema Fernandez, Lorenz Borsdorf, Constantin Daniliuc, Shigehiro Yamaguchi, Soichiro Ogi, Gustavo Fernandez
Supramolecular polymers are often investigated for highly symmetric and planar molecules, such as typically explored BF2-substituted BODIPY dyes . However, it is surprising that the possibility of desymmetrizing the sp3...
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