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Development of an engineered thermostable amine dehydrogenase for the synthesis of structurally diverse chiral amines

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Catal. Sci. Technol., 2020, 10,2353-2358
DOI: 10.1039/D0CY00071J, Paper
Lei Liu, Dong-Hao Wang, Fei-Fei Chen, Zhi-Jun Zhang, Qi Chen, Jian-He Xu, Zhi-Long Wang, Gao-Wei Zheng
Structurally diverse chiral amines and amino alcohols were synthesized using an engineered thermostable amine dehydrogenase, demonstrating its extensive synthesis potential.
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Pd–Au bimetallic catalysts supported on ZnO for selective 1,3-butadiene hydrogenation

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Catal. Sci. Technol., 2020, 10,2503-2512
DOI: 10.1039/C9CY02395J, Paper
Open Access
Belén Bachiller-Baeza, Ana Iglesias-Juez, Giovanni Agostini, Eva Castillejos-López
The effect of the ZnO morphology on the properties of Pd–Au bimetallic catalysts has been discussed.
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Hourglass-type polyoxometalate-based crystalline materials as efficient cooperating photocatalysts for the reduction of Cr(VI) and oxidation of dyes

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Catal. Sci. Technol., 2020, 10,2593-2601
DOI: 10.1039/D0CY00208A, Paper
Xuerui Tian, Yaqi Zhang, Yuanyuan Ma, Qing Zhao, Zhangang Han
Hourglass-type polyoxometalate-based crystalline materials exhibit efficient photocatalytic activities towards simultaneous photocatalytic Cr(VI) reduction and organic MB oxidation.
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980 nm NIR light driven overall water splitting over a combined CdS–RGO–NaYF4–Yb3+/Er3+ photocatalyst

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Catal. Sci. Technol., 2020, 10,2389-2397
DOI: 10.1039/D0CY00256A, Paper
Wei Gao, Yuqi Wu, Gongxuan Lu
Infrared light (NIR) accounts for more than 50% of the energy donated by the Sun to the Earth, but most of this type of energy is not utilized in photocatalytic reactions.
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Enhanced and selective photocatalytic reduction of CO2 by H2O over strategically doped Fe and Cr into porous boron carbon nitride

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Catal. Sci. Technol., 2020, 10,2663-2680
DOI: 10.1039/D0CY00343C, Paper
Niwesh Ojha, Abhinav Bajpai, Sushant Kumar
Strategic doping of metals and non-metals into a photocatalyst can help in tuning the band gap and alignment of band structure.
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Adjustable anchoring of Ni/Co cations by oxygen-containing functional groups on functionalized graphite paper and accelerated mass/electron transfer for overall water splitting

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Catal. Sci. Technol., 2020, 10,2627-2643
DOI: 10.1039/D0CY00181C, Paper
Yiyi Huang, Lei Sun, Zebin Yu, Ronghua Jiang, Jun Huang, Yanping Hou, Fei Yang, Boge Zhang, Runzhi Zhang, Yalan Zhang
NCS–NCO/FGP0.44 with a cellular network of porous nanosheets and close-contact heterointerface reveals accelerated interfacial mass/electron transportation for overall water splitting.
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Bimetallic scorpionate-based helical organoaluminum complexes for efficient carbon dioxide fixation into a variety of cyclic carbonates

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Catal. Sci. Technol., 2020, Advance Article
DOI: 10.1039/D0CY00593B, Paper
Marta Navarro, Luis F. Sánchez-Barba, Andrés Garcés, Juan Fernández-Baeza, Israel Fernández, Agustín Lara-Sánchez, Ana M. Rodríguez
The binuclear aluminum complexes [AlR2(κ2-NN';κ2-NN')AlR2] with TBAB/PPNCl behave as excellent systems for cyclic carbonate formation from CO2 with challenging epoxides.
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Photocatalytic hydrogen evolution over nickel cobalt bimetallic phosphate anchored graphitic carbon nitrides by regulation of d-band electronic structure

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Catal. Sci. Technol., 2020, Accepted Manuscript
DOI: 10.1039/D0CY00556H, Paper
Yuanzheng Zhang, Yunrong Dai, Lifeng Yin, Huihui Li, Xiang Chen, Bin Chen
Non-precious metal co-catalysts with high activity and stability are extremely desirable for economically viable photocatalytic molecular hydrogen (H2) evolution. Herein, nickel cobalt phosphate (NiCo-Pi) was introduced into graphitic carbon nitride...
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Phosphine-catalyzed [3 + 2] annulation of 2-aminoacrylates with allenoates and mechanistic studies

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Catal. Sci. Technol., 2020, Accepted Manuscript
DOI: 10.1039/D0CY00092B, Paper
Xiao-Yun Wu, Hou-Ze Gui, Harish Jangra, Yin Wei, Min Shi, Hendrik Zipse
A convenient and efficient strategy for the synthesis of 3-pyrrolines containing an amino quaternary stereogenic center via phosphine-catalyzed formal [3 + 2] annulation of allenoates with 2-aminoacrylates is disclosed. A...
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Photocatalytic degradation of tetracycline hydrochloride over rugby-like β-Ga2O3 with a 3D hierarchically assembled porous structure for environmental remediation

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Catal. Sci. Technol., 2020, Advance Article
DOI: 10.1039/D0CY00562B, Paper
Lingxing Zeng, Jiaqi Wang, Qingrong Qian, Qinghua Chen, Xin-Ping Liu, Yongjin Luo, Hun Xue, Zhaohui Li
A novel rugby ball-like β-Ga2O3 photocatalyst with a 3D hierarchically assembled porous structure was constructed via a facile precipitation–calcination method. The as-synthesized Ga2O3 exhibits a high photocatalytic efficiency compared to commercial Ga2O3 and Degussa P25.
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Photoswitchable catalysis using organometallic complexes

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Catal. Sci. Technol., 2020, Advance Article
DOI: 10.1039/D0CY00431F, Minireview
Zoraida Freixa
Photoswitchable catalysis using organometallic complexes: a ligand design perspective.
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Shapoorji Pallonji group subsidiary announces plan to list Eureka Forbes

By www.business-standard.com
Published On :: Tue, 19 Nov 2019 15:50:00 +0530

Forbes & Company, a Shapoorji Pallonji group firm on Tuesday announced plans to list its subsidiary Eureka Forbes to unlock value for shareholders. The company's board has authorised the management to evaluate any such scheme in this regard, Forbes & Company said in a regulatory filing. "The Board of Directors of the company has authorised the management...to evaluate a scheme of arrangement and/or other appropriate mechanisms to enable an eventual listing of Eureka Forbes with an intention to unlock value in the hands of all the shareholders of the company," it said. These may also include listing, dilution/sale or combination thereof of Eureka Forbes, it added. Eureka Forbes is a wholly-owned subsidiary of Forbes & Company. "The Board will consider the above (schemes) when the relevant proposals are placed before it in the near future, but in principle has approved supporting the endeavours of the management in this regard," it said. It operates in water purifier, air ...


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Ujjivan Small Finance Bank eyes Rs 750 cr via IPO; issue to open on Dec 2

By www.business-standard.com
Published On :: Wed, 27 Nov 2019 19:07:00 +0530

The lender commenced operations in February 2017 and the bank will also have to bring the promoters' holding to 40 percent by 2022


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Equitas Small Finance Bank files draft papers for IPO, to raise Rs 550 cr

By www.business-standard.com
Published On :: Mon, 16 Dec 2019 20:10:00 +0530

The equity shares of the company will be listed on the BSE and the NSE.


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SBI Cards IPO opens March 2: All you need to know about the $1.4 bn offer

By www.business-standard.com
Published On :: Wed, 26 Feb 2020 20:14:00 +0530

No multi-bagger like IRCTC, but can deliver 50% listing gains, says Ambareesh Baliga, an independent market expert


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SBI Cards allots shares worth nearly Rs 2,800 crore to anchor investors

By www.business-standard.com
Published On :: Sat, 29 Feb 2020 09:54:00 +0530

The SBI Cards IPO will be a test for investor appetite, which has been battered by the coronavirus outbreak.


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Equitas Small Finance Bank gets Sebi nod for IPO worth Rs 550 crore

By www.business-standard.com
Published On :: Tue, 03 Mar 2020 13:36:00 +0530

JM Financial, Edelweiss Financial Services and IIFL Securities are managing the offer


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SBI Cards IPO: Allotment of shares finalised, steps to check status

By www.business-standard.com
Published On :: Thu, 12 Mar 2020 14:34:00 +0530

The SBI Cards IPO is one of the largest share sale in recent times, both in terms of size and oversubscription


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ESAF Small Finance Bank gets Sebi approval to float Rs 976 crore IPO

By www.business-standard.com
Published On :: Thu, 26 Mar 2020 23:55:00 +0530

SEBI issued the final observations to the lenders proposal on March 20, 2020.


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Black Panther. writer[s], Nnedi Okorafor, Aaron Covington ; artists, André Lima Araújo, Mario del Pennino ; color artist[s], Chris O'Halloran, Ian Herring, Irma Knivila ; penciler, Tana Ford ; inkers, Tana Ford, Terry Pallot, Scott Hanna ;

By library.mit.edu
Published On :: Sun, 23 Feb 2020 07:00:06 EST

Barker Library - PN6728.B53 L66 2018


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Frankenstein: Junji Ito story collection / story & art by Junji Ito ; translation, Jocelyn Allen ; English adaptation, Nick Mamatas ; other stories translation & adaptation, Jocelyn Allen ; touch-up art & lettering, James Dashiell ; cover &

By library.mit.edu
Published On :: Sun, 23 Feb 2020 07:00:06 EST

Barker Library - PN6790.J33 I73413 2018


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My solo exchange diary / (true) story & art, Nagata Kabi ; translation, Jocelyne Allen ; adaptation, Lianne Sentar

By library.mit.edu
Published On :: Sun, 23 Feb 2020 07:00:06 EST

Barker Library - PN6790.J33 N243413 2017


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Influence of the mechanical properties of biomaterials on degradability, cell behaviors and signaling pathways: current progress and challenges

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00269K, Review Article
Lu Wang, Cunyang Wang, Shuai Wu, Yubo Fan, Xiaoming Li
We have clarified the influence of the mechanical properties of biomaterials on degradability and cell response, and also mechanical design targets and approaches.
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High antimicrobial photodynamic activity of photosensitizer encapsulated dual-functional metallocatanionic vesicles against drug-resistant bacteria S. aureus

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00323A, Paper
Bunty Sharma, Gurpreet Kaur, Ganga Ram Chaudhary, Santosh L. Gawali, P. A. Hassan
Developments in the field of photodynamic therapy (PDT) are being made by investigating appropriate photosensitizers (PSs) and enhancing the penetration effect of light by developing new metallocatanionic vesicles.
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Arbitrarily-shaped microgels composed of chemically unmodified biopolymers

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/C9BM02056J, Paper
Yadu N. Vakkipurath Kodakkadan, Kristyna Idzakovicova, Josef Sepitka, Daniël ten Napel, Eric Safai, Petr Cigler, Frantisek Štěpánek, Ivan Rehor
We introduce a method for photolithographic synthesis of arbitrarily shaped microgels composed purely of a biopolymer of choice.
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A photothermal-hypoxia sequentially activatable phase-change nanoagent for mitochondria-targeting tumor synergistic therapy

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Published On ::

Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00003E, Paper
Jia Qu, Dengke Teng, Guoqing Sui, Shihui Guan, Yang Wang, Qimeihui Wang, Yuanqiang Lin, Haitao Ran, Zhigang Wang, Hui Wang
The advantages of PCM@Lip/IT NPs include mitochondrial-targeting, on-demand drug release, and prodrug activation by hypoxia with guidance/monitoring by PA and FL imaging.
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A Fe3+-crosslinked pyrogallol-tethered gelatin adhesive hydrogel with antibacterial activity for wound healing

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00188K, Paper
Ning Han, Ziyang Xu, Chunyan Cui, Yuan Li, Dongfei Zhang, Meng Xiao, Chuanchuan Fan, Tengling Wu, Jianhai Yang, Wenguang Liu
A tunicate-inspired gelatin-based hydrogel prepared by a simple mixing method, exhibits strong adhesion and antibacterial capacity, and facilitates wound healing.
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Additively manufactured functionally graded biodegradable porous zinc

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Biomater. Sci., 2020, 8,2404-2419
DOI: 10.1039/C9BM01904A, Paper
Open Access
Y. Li, P. Pavanram, J. Zhou, K. Lietaert, F. S. L. Bobbert, Yusuke Kubo, M. A. Leeflang, H. Jahr, A. A. Zadpoor
First report on the effect of topology design on the biodegradation, mechanical properties, and cell responses of additively manufactured Zn.
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Naturally available hypericin undergoes electron transfer for type I photodynamic and photothermal synergistic therapy

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Biomater. Sci., 2020, 8,2481-2487
DOI: 10.1039/D0BM00021C, Paper
Zhen Ke, Aize Xie, Jianjiao Chen, Zhenyuan Zou, Lei Shen, Yansong Dai, Dengfeng Zou
Hypericin undergoing electron transfer can be used for type I PDT and PTT.
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Enhanced selectivity, cellular uptake, and in vitro activity of an intrinsically fluorescent copper–tirapazamine nanocomplex for hypoxia targeted therapy in prostate cancer

By pubs.rsc.org
Published On ::

Biomater. Sci., 2020, 8,2420-2433
DOI: 10.1039/C9BM01905G, Paper
Vera L. Silva, Abdessamad Kaassis, Ashkan Dehsorkhi, Cédrik-Roland Koffi, Maja Severic, Moustafa Abdelhamid, Duuamene Nyimanu, Christopher J. Morris, Wafa’ T. Al-Jamal
Cu(TPZ)2 complex as a promising hypoxia selective cytotoxin in prostate cancer.
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The electrospinning of a thermo-responsive polymer with peptide conjugates for phenotype support and extracellular matrix production of therapeutically relevant mammalian cells

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Biomater. Sci., 2020, 8,2611-2626
DOI: 10.1039/C9BM01965K, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
F. A. A. Ruiter, L. E. Sidney, K. L. Kiick, J. I. Segal, C. Alexander, F. R. A. J. Rose
The fabrication and application of a biocompatible peptide conjugated thermo-responsive fibrous scaffolds for cellular phenotype support and enzymatic-free passaging of mammalian cells.
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Optically controlled hybrid metamaterial of plasmonic spiky gold inbuilt graphene sheets for bimodal imaging guided multimodal therapy

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00312C, Paper
Kunnumpurathu Jibin, Jayaram S. Prasad, Giridharan Saranya, Sachin J. Shenoy, Kaustabh K. Maiti, Ramapurath S. Jayasree
Gold–graphene nanohybrid for simultaneous dual-imaging guided triple therapy as a new paradigm in light-triggered cancer theranostics. The material demonstrates excellent therapeutic efficacy and treatment monitoring features.
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A transport system based on a quantum dot-modified nanotracer is genetically and developmentally stable in pregnant mice

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00311E, Paper
Open Access
Hye Jin Kim, Ji Sun Park, Se Won Yi, Minyeon Go, Hye-Ryun Kim, Su Jin Lee, Jong Min Park, Dong Hyun Cha, Sung Han Shim, Keun-Hong Park
The use of nanoscale materials (NMs) could cause problems such as cytotoxicity, genomic aberration, but the impacts of NM exposure during pregnancy remain uncharacterized in the context of clinical applications.
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Surface engineering of titanium alloy using metal-polyphenol network coating with magnesium ions for improved osseointegration

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Biomater. Sci., 2020, Advance Article
DOI: 10.1039/D0BM00566E, Paper
Sangmin Lee, Yun-Young Chang, Jinkyu Lee, Sajeesh Kumar Madhurakkat Perikamana, Eun Mi Kim, Yang-Hun Jung, Jeong-Ho Yun, Heungsoo Shin
Although titanium-based implants are widely used in orthopedic and dental clinics, improved osseointegration at the bone–implant interface is still required.
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A biomimetic orally targeted delivery of Bindarit for immunotherapy of atherosclerosis

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Biomater. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0BM00418A, Paper
Luqi Yin, Cuiping Peng, Yue Tang, Yuchuan Yuan, Jiaxing Liu, Tingting Xiang, Feila Liu, Zhou Xing, Xiaohui Li
Monocyte chemoattractant protein-1 (MCP-1) plays an important role in the development of atherosclerosis. However, the application of bindarit (a specific synthetic inhibitor of MCP-1) in atherosclerosis has not been confirmed...
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Serum miRNAs are differentially altered by ethanol and caffeine consumption in rats

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Toxicol. Res., 2019, 8,842-849
DOI: 10.1039/C9TX00069K, Paper
M. Martinez, I. M. U. Rossetto, R. M. S. Arantes, F. S. N. Lizarte, L. F. Tirapelli, D. P. C. Tirapelli, L. G. A. Chuffa, F. E. Martinez
Alcoholism is a multifactorial disease with high risk for dependence determined by genetic background, environmental factors and neuroadaptations.
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Gynura divaricata ameliorates hepatic insulin resistance by modulating insulin signalling, maintaining glycolipid homeostasis and reducing inflammation in type 2 diabetic mice

By pubs.rsc.org
Published On ::

Toxicol. Res., 2019, 8,928-938
DOI: 10.1039/C9TX00191C, Paper
Xuan Dong, Shu-Xiang Zhao, Bing-Qing Xu, Yu-Qing Zhang
Oral lyophilized powder of Gynura divaricata, an edible medicinal plant, can alleviate both hyperglycaemia and hepatic insulin resistance in type 2 diabetic mice.
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Thyroid endocrine status and biochemical stress responses in adult male Wistar rats chronically exposed to pristine polystyrene nanoplastics

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Published On ::

Toxicol. Res., 2019, 8,953-963
DOI: 10.1039/C9TX00147F, Paper
Fatemeh Amereh, Akbar Eslami, Simin Fazelipour, Mohammad Rafiee, Mohammad Ismail Zibaii, Mohammad Babaei
At this time, little is known about the long-term effects of micro(nano)plastics on public health. In the present study, early warning signs of thyroid endocrine disruption were noticed in adult Wistar rats from the ingestion of virgin polystyrene nanoparticles.
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Biogenic Aspergillus tubingensis silver nanoparticles’ in vitro effects on human umbilical vein endothelial cells, normal human fibroblasts, HEPG2, and Galleria mellonella

By pubs.rsc.org
Published On ::

Toxicol. Res., 2019, 8,789-801
DOI: 10.1039/C9TX00091G, Paper
Cristiane Angélica Ottoni, Durvanei Augusto Maria, Priscila Jane Romano de Oliveira Gonçalves, Welington Luiz de Araújo, Ana Olívia de Souza
Biogenic silver nanoparticles are ecofriendly and offers valuable possibilities of applications in several industrial areas.
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HC orders closure of Liquor shops in Tamil Nadu, allows online sales

By www.business-standard.com
Published On :: Fri, 08 May 2020 22:48:00 +0530

The opening of shops in districts, except Chennai on May 7, has resulted in people thronging the outlets without maintaining social distancing norms


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Dy2@C79N: A New Member of Dimetalloazafullerenes with Strong Single Molecular Magnetism

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Published On ::

Nanoscale, 2020, Accepted Manuscript
DOI: 10.1039/D0NR02519D, Paper
Yuanyuan Wang, Jin Xiong, Jie Su, Zi-Qi Hu, Fang Ma, Rong Sun, Xue-You Tan, Hao-Ling Sun, Bingwu Wang, Zujin Shi, Song Gao
Enhancing the exchange interaction between magnetic ions is a long-term target in molecular magnetism. Endohedral metallofullerenes (EMFs) provide a possibility for achieving such a goal by imprisoning multiple magnetic centers...
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Correction: Anomalous polarization dependence of Raman scattering and crystallographic orientation of black phosphorus

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Nanoscale, 2020, Advance Article
DOI: 10.1039/D0NR90098B, Correction
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Jungcheol Kim, Jae-Ung Lee, Jinhwan Lee, Hyo Ju Park, Zonghoon Lee, Changgu Lee, Hyeonsik Cheong
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Strong plasmon–exciton coupling between lithographically defined single metal nanoparticles and monolayer WSe2

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Nanoscale, 2020, 12,9708-9716
DOI: 10.1039/D0NR01056A, Paper
Xiaohong Yan, Hong Wei
Strong coupling between monolayer WSe2 and lithographically defined single gold nanobowties is realized for the first time, and smaller nanobowties lead to larger coupling strength.
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Interfacial synergy between dispersed Ru sub-nanoclusters and porous NiFe layered double hydroxide on accelerated overall water splitting by intermediate modulation

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Nanoscale, 2020, 12,9669-9679
DOI: 10.1039/D0NR01491E, Paper
Yao Wang, Peng Zheng, Mingxuan Li, Yunrui Li, Xin Zhang, Juan Chen, Xu Fang, Yujie Liu, Xiaolin Yuan, Xiaoping Dai, Hai Wang
Benefitting from the desired potential-induced interfacial synergy, the Ru–NiFe LDH interfaces will convert to RuO2–NiFe(OOH)x interfaces to meet the requirements of an anode and cathode reaction, respectively.
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Facile synthesis of core–shell structured Si@graphene balls as a high-performance anode for lithium-ion batteries

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Nanoscale, 2020, 12,9616-9627
DOI: 10.1039/D0NR01346C, Paper
Anif Jamaluddin, Bharath Umesh, Fuming Chen, Jeng-Kuei Chang, Ching-Yuan Su
Encapsulating silicon (Si) nanoparticles with graphene nanosheets in a microspherical structure is proposed to increase electrical conductivity and solve stability issues when using Si as an anode material in lithium-ion batteries (LIBs).
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A solution-processed zero-dimensional all-inorganic perovskite scintillator for high resolution gamma-ray spectroscopy detection

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Published On ::

Nanoscale, 2020, 12,9727-9732
DOI: 10.1039/D0NR00772B, Paper
Qiang Xu, Juan Wang, Wenyi Shao, Xiao Ouyang, Xiang Wang, Xinlei Zhang, Yong Guo, Xiaoping Ouyang
A zero-dimensional all-inorganic CsPbBr3 nanocrystal embedded Cs4PbBr6 scintillator has been achieved. Owing to the low dimensional quantum effect, this all-inorganic scintillator exhibits desirable scintillation performance.
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N- & S-co-doped carbon nanofiber network embedded with ultrafine NiCo nanoalloy for efficient oxygen electrocatalysis and Zn–air batteries

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Nanoscale, 2020, 12,9581-9589
DOI: 10.1039/D0NR01516D, Paper
Chaojun Liu, Zhuang Wang, Xin Zong, Yingmin Jin, Dong Li, Yueping Xiong, Gang Wu
A 3D carbon nanofiber network embedded with ultrafine nanoparticles is prepared by electrospinning. Thioacetamide is used to prevent the aggregation of active sites.
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Reply to the ‘Comment on “Hierarchically porous, ultra-strong reduced graphene oxide–cellulose nanocrystal sponges for exceptional adsorption of water contaminants”’ by J. Ma, Y. Xiong and F. Yu, Nanoscale, 2019, 11, DOI: 10.1039/C8NR08780F

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Nanoscale, 2020, 12,9899-9901
DOI: 10.1039/D0NR01846E, Comment
Nariman Yousefi, Nathalie Tufenkji
We respond to the comments of Ma et al. and clarify the rationale behind our methodology and why it is suitable for our work.
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Ternary PtFeCo alloys on graphene with high electrocatalytic activities for methanol oxidation

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Nanoscale, 2020, 12,9824-9832
DOI: 10.1039/D0NR00757A, Paper
Hongfei Wang, Kefu Zhang, Jun Qiu, Juan Wu, Jingwen Shao, Huijuan Wang, Yujuan Zhang, Jie Han, Yong Zhang, Lifeng Yan
Ternary PtFeCo alloys as alternatives to conventional Pt electrocatalysts are highly important in the field of the methanol oxidation reaction.
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Characteristics of crystalline sputtered LaFeO3 thin films as photoelectrochemical water splitting photocathodes

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Nanoscale, 2020, 12,9653-9660
DOI: 10.1039/D0NR01762K, Paper
Min-Kyu Son, Hyunwoong Seo, Motonori Watanabe, Masaharu Shiratani, Tatsumi Ishihara
A transparent crystalline sputtered LaFeO3 photocathode with an early onset potential for stable photoelectrochemical water splitting.
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