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Modulating the band gap of a pyrazinoquinoxaline-based metal–organic framework through orbital hybridization for enhanced visible light-driven CN bond construction

J. Mater. Chem. A, 2024, 12,30582-30590
DOI: 10.1039/D4TA06282E, Paper
Zitong Chen, Linghui Cao, Aogang Liu, Pengda Liu, Yuan Chen, Juntao Yan, Bao Li
An indium-based metal–organic framework bearing a pyrazinoquinoxaline derivative is synthesized to facilitate two methods for the construction of CN bonds, and their mechanisms are investigated through detailed theoretical calculations.
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Unsaturated coordination modulation and enlarged pore size in nanoflower-like metal organic frameworks for enhanced lithium–oxygen battery performance

J. Mater. Chem. A, 2024, 12,30591-30600
DOI: 10.1039/D4TA06346E, Paper
Lingwen Zhao, Juanjuan Feng, Adeel Abbas, Hao Sun, Chunlei Wang, Hongchao Wang
Unsaturated coordination modulation alters the discharge path and increased pore size accelerates ion exchange and oxygen transport, synergistically improving the electrochemical performance of LOBs.
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Multifunctional characteristics of a one-dimensional bimetallic oxyhydroxide nanorod-coupled polyaniline interface for accelerated water and urea electrolysis

J. Mater. Chem. A, 2024, 12,30743-30756
DOI: 10.1039/D4TA05082G, Paper
Niranjanmurthi Lingappan, Sandhiya Lakshmanan, Wonoh Lee
Designing an efficient and durable electrocatalyst is central to hydrogen production technologies such as hydrogen evolution reaction, oxygen evolution reaction, and urea oxidation reaction.
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Synthesis of a Cu@ZnO1−x/Al2O3 catalyst with high-density ZnO1−x–Cu interfacial sites for enhanced CO2 hydrogenation to methanol

J. Mater. Chem. A, 2024, 12,30692-30706
DOI: 10.1039/D4TA05801A, Paper
Yunshuo Wu, Haiqiang Wang, Zhongbiao Wu
The development of catalysts with high-density interfacial sites is crucial for enhancing catalytic performance.
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A review on instability factors of mono- and divalent metal ion batteries: from fundamentals to approaches

J. Mater. Chem. A, 2024, 12,30190-30248
DOI: 10.1039/D4TA05386A, Review Article
Elmira Kohan, Roushan Khoshnavazi, Mir Ghasem Hosseini, Abdollah Salimi, Mehdi Salami-Kalajahi
Degradation phenomena in different components (cathode, anode, current collectors (CCs)) of mono- and divalent metal-based batteries affect their performance.
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Electrochemical synthesis of wormcast-like Pd-based polycrystalline high entropy aggregates for methanol water co-electrocatalysis

J. Mater. Chem. A, 2024, 12,30757-30767
DOI: 10.1039/D4TA06304J, Paper
Yaxing Liu, Wenhao Ding, Jiaxin Liu, Guizhe Zhao, Weiyin Li, Yaqing Liu
A wormcast-like nanostructure of PdFeCoNiCu-pHENs with enriched grain boundary defects was synthesized via electrodeposition. This work opens new possibilities for designing advanced nanomaterials aimed at efficient electrochemical energy conversion.
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One-pot spatial engineering of multi-enzymes in metal–organic frameworks for enhanced cascade activity

J. Mater. Chem. A, 2024, 12,30318-30328
DOI: 10.1039/D4TA06211F, Paper
Wenqing Fan, Kang Liang, Jieying Liang
A one-pot strategy was developed for the first time to achieve the precise spatial arrangement of multiple enzymes in MOFs, improving multi-enzyme cascade efficiency.
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Dual solar-driven hydrogen evolution and alcohol oxidation with CdS quantum dot-sensitized photocatalysts prepared by the SILAR methodology

J. Mater. Chem. A, 2024, 12,30885-30891
DOI: 10.1039/D4TA03559C, Paper
Vasilis Nikolaou, Deborah Romito, Clément Maheu, Jonathan Hamon, Eric Gautron, Florian Massuyeau, Pierre-Emmanuel Petit, Stéphane Jobic, Fabrice Odobel
The first use of the successive ionic layer adsorption and reaction (SILAR) method to grow CdS quantum dots on TiO2 nanoparticles, achieving efficient photocatalytic alcohol oxidation and H2 evolution without catalysts or sacrificial donors.
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Design and construction of porphyrin box-based metal–organic frameworks with hierarchical superstructures for efficient energy transfer and photooxidation

J. Mater. Chem. A, 2024, 12,30685-30691
DOI: 10.1039/D4TA05576D, Paper
Qian Xu, Peng Zhang, Yuanyuan Sun, Jishi Chen, Chuantao Hou, Zonghua Wang
A porphyrin box-based MOF with hierarchical superstructures was synthesized, exhibiting enhanced performance in singlet oxygen-mediated photooxidation.
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A sustainable redox-mediated pathway for improved transition metal organic framework activation and CO2 uptake performance

J. Mater. Chem. A, 2024, 12,30454-30464
DOI: 10.1039/D4TA02526A, Paper
Taylor Jade Self, Jiabin Niu, Wen Liu, Chaobin He, Mei Chee Tan
Sustainable substitutions in MOF fabrication and processing can confidently be made by employing redox engineering for synergistic valency and defect constitution, based on application, without sacrificing active site functionality.
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Metal–organic framework derived low-crystallinity cobalt–nitrogen–carbon electrocatalysts for nitrate reduction to ammonia

J. Mater. Chem. A, 2024, 12,30409-30419
DOI: 10.1039/D4TA05443A, Paper
Yue Cao, Shengbo Yuan, Wenbo Zhou, Yan Hai, Xiaoman Li, Min Luo
NO3 and H2O molecules adsorbed on the surface of Co–N–C-500 are activated and dissociated. The generated active hydrogen species (*H) can promote the hydrogenation of the intermediates and thus increase the NH3 yield.
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Smart fabrics with liquid metal reinforced PU/CNT/MXene multilayer structures for constructing multifunctional sensors and wearable electronics

J. Mater. Chem. A, 2024, 12,30872-30884
DOI: 10.1039/D4TA05266H, Paper
Haijiao Lin, Hui Wang, Yongguang Yang, Yuxuan Zhang, Ling Li, Youwei Zhao, Wenming Zhang
Smart fabrics with liquid metal reinforced PU/CNT/MXene multilayer structures for constructing multifunctional sensors and wearable electronics.
The content of this RSS Feed (c) The Royal Society of Chemistry




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Development and application of Few-shot learning methods in materials science under data scarcity

J. Mater. Chem. A, 2024, 12,30249-30268
DOI: 10.1039/D4TA06452F, Review Article
Yongxing Chen, Peng Long, Bin Liu, Yi Wang, Junlong Wang, Tian Ma, Huilin Wei, Yue Kang, Haining Ji
Machine learning, as a significant branch of artificial intelligence, shortens the cycle of material discovery and synthesis by exploring the characteristics of data.
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Ir nanoparticles decorated NiFe metal–organic framework as a highly efficient and stable heterostructure electrocatalyst for overall seawater splitting

J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06515H, Communication
Hefeng Wang, Zixiao Li, Zhengwei Cai, Chaoxin Yang, Shengjun Sun, Xiaoyan Wang, Min Zhang, Meng Yue, Dongdong Zheng, Asmaa Farouk, Mohamed S. Hamdy, Xuping Sun, Bo Tang
Ir nanoparticle decorated NiFe metal–organic framework on Ni foam (Ir@NiFe-MOF/NF) acts as a bifunctional catalyst for the oxygen evolution reaction and the hydrogen evolution reaction in alkaline seawater with excellent performance and stability.
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A doubly interpenetrated perylene diimide-based zirconium metal–organic framework for selective oxidation of sulfides powered by blue light

J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06294A, Paper
Chao Wei, Ming Lu, Jing-Jing Li, Ze-Jiu Diao, Guoliang Liu, Xiao-Qin Liu, Lin-Bing Sun
A doubly interpenetrated perylene diimide-based zirconium metal–organic framework is developed as a heterogeneous photocatalyst for selective photocatalytic oxidation of organic sulfides powered by blue light.
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Recent Advances on Non-noble Metal Catalysts toward N-ethylcarbazole Hydrogen Storage

J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06468B, Review Article
Hansai Wu, junming Zhang, Zicong Wang, Xianglong Kong, Gaofu Li, Ying Zhao, Piaoping Yang, Zhiliang Liu
N-ethylcarbazole (NEC) hydrogen storage has garnered significant attention owing to its large-scale safe storage of hydrogen superiority. However, the sluggish hydrogenation kinetics in NEC are extremely dependent on catalysts with...
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A π–d conjugated metal–organic framework decorated on a MXene-carbon nanofiber as a self-standing electrode for flexible supercapacitors

J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06232A, Paper
Zahir Abbas, Shaikh M. Mobin
A c-MOF is grown on MX-CNF, which was prepared via electrospining method. Furthermore, it utilized for flexible supercapcitors with different flexibility angles.
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High-throughput Screening of Mechanically Interlocked Catenane Metal Complexes for Enhanced Electrocatalytic Activity

J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06497F, Paper
Mohsen Tamtaji, William A. Goddard III, Guanhua Chen
Metal complexes have been thoroughly investigated for a wide range of electrochemical reactions. However, mechanically interlocked molecular machines (MIM) have not been investigated for electrochemistry through a systematic high throughput...
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Methods to Create Amazing Interracial Marriages

A marriage between a couple of different backrounds can be a beautiful and rewarding encounter, however it is not really without its obstacles. It is important just for couples to keep yourself informed of these possible risks and take the necessary precautions in order to avoid them. A new study from University of Washington found […]




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Using the Engineering Method to Teach Important Thinking and Problem-Solving Skills to Vibrant Minds

The technological innovation process is acknowledged as a sequence of procedures that engineers follow to find the best solution to a problem. That allows designers to use math concepts, applied research and technological innovation sciences to obtain a high level of optimization that meets the requirements of an goal. The steps incorporate defining the situation, […]




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Methods to Manage an information Room meant for M&A Trades

A Data Space is a protect, centralized site for posting information and documents with multiple stakeholders related to a small business transaction. These types of transactions can easily involve M&A or be for every other business activity that will need the transfer of very sensitive data to parties beyond the organization. Handling these trades can […]




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Sachin Tendulkar met Dalai Lama, inaugurated Centre of Excellence in HPCA Dharamshala

The Bharat Ratan, Cricketer Sachin Tendulkar today met 82 years old Tibetan spiritual leader the 14th Dalai Lama at his residence in north Indian hill town Dharmashala. After meeting the Dalai Lama Sachin said, “It’s excellent… very good meeting and always wanted to be here and take the blessings. Just wanted to spend some time […]




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United States’ Ambassador to India Kenneth Juster met the Dalai Lama

Visiting the Tibetan headquarters in Exile for the first time, the United States’ Ambassador to India Kenneth Juster today called on the Tibetan leader the Dalai Lama at the latter’s residence in Dharamshala North India on Friday. “I was very inspired by his presence. We had a discussion on a broad range of subjects. It […]




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Sydney’s ‘mystery’ toxic beach balls are cosmetic waste

Around 2,000 of the mystery black balls had washed onto beaches across Sydney since October 15




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Greenhouse gas emissions surge to new record in 2023: World Meteorological Organization report

The globally averaged surface concentration of carbon dioxide reached 420 parts per million (ppm), methane 1934 parts per billion and nitrous oxide 336.9 parts per billion (ppb) in 2023.




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Your hair-stylist, tattoo artist, tailor can help monitor metabolic health, says Dr Sarin

In his book “Own Your Body,” Dr Shiv Sarin advocates for educating these professionals to look for signs like black lines, skin tags, and waist-to-hip ratios, which could indicate underlying health issues




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TASL’s first ‘sub-metre optical’ satellite launched

The SpaceX’s Falcon 9 rocket catapulted the TASL’s satellite from Launch Complex 39A at Kennedy Space Center on April 7, says TASL




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JD Chakravarthy: I knew from day one that we were on to something big with ‘Dayaa’

Actor J D Chakravarthy, revelling in the reception to his Telugu web series ‘Dayaa’, says he and director Pavan Sadineni would have almost not worked with each other




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Director Shiva Nirvana: ‘Kushi’ will discuss something beyond post-marriage romance, which we have not revealed in the trailer

Ahead of the release of Vijay Deverakonda and Samantha Ruth Prabhu’s ‘Kushi’, director Shiva Nirvana opens up on the Mani Ratnam influence and how he was never inclined to direct romances initially




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META Award winner Hunkaro is back in Bengaluru

The idea of the play came about with the disturbing realisation that the lockdown reduced not only the attention span of people but also the capacity and need to listen




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Cabinet approves Phase 3 of Namma Metro

44.65 km of new line will be added to the network by 2028 at a cost of ₹ 15,611 crore




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Attempts to regulate Auroville’s functioning are met with resistance and litigation, says Madras HC

Justice Anita Sumanth refuses to issue a writ of quo warranto against seven individuals representing the Working Committee of the Residents’ Assembly




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The Metropolitan Museum of Art Puts 490,000 High-Res Images Online & Makes Them Free to Use

Update: The Metropolitan Museum of Art has put online 492,000 high-resolution images of artistic works. Even better, the museum has placed the vast majority of these images into the public domain, meaning they can be downloaded directly from the museum’s website for non-commercial use. When you browse the Met collection and find an image that […]




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Download 1,600+ Publications from the Metropolitan Museum of Art: Books, Guides, Magazines & More

Many of us in these past few generations first heard of the Metropolitan Museum of Art while reading E. L. Konigsburg’s novel From the Mixed-Up Files of Mrs. Basil E. Frankweiler. More than a few of us also fantasized about running away to live in that vast cultural institution like the book’s young protagonists Claudia and […]




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Investigation of 3,4-ethylenedioxythiophene and 3,4-dimethoxythiophene as linkage units for multi-dimensional dimeric acceptors

J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC03646H, Paper
Shaohui Yuan, Baofa Lan, Xinyi Ji, Jiaying Wang, Wenkai Zhao, Guankui Long, Xiangjian Wan, Bin Kan, Yongsheng Chen
Despite the versatile processibility of three-dimensional CH8 series acceptors in efficient organic solar cells (OSCs), understanding the relationship between linkage units and performance continues to present significant challenges. To address...
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An advanced self-powered visible-light photodetector based on the asymmetric Au/CsPbBr3/SmB6 junction

J. Mater. Chem. C, 2024, 12,17395-17402
DOI: 10.1039/D4TC03510K, Paper
Zairan Liu, Gang Cao, Zhaozhi Guan, Yan Tian, Jidong Liu, Jun Chen, Shaozhi Deng, Fei Liu
An asymmetric Au/CsPbBr3/SmB6 self-powered photodetector exhibits greatly enhanced visible-light photosensitive performances with the help of an interfacial built-in field.
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Visible light mediated efficient photoswitching of dimethyldihydropyrenes in thin films for all-photonic logic gate applications and dynamic encryption/decryption capabilities

J. Mater. Chem. C, 2024, 12,17511-17518
DOI: 10.1039/D4TC03321C, Paper
Sariful Molla, Subhajit Bandyopadhyay
Dimethyldihydropyrene (DHP) photoswitches exhibit visible light-induced ring-opening photoisomerization, reversed by UV/visible light or heat in thin films.
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Observation and enhancement through alkali metal doping of p-type conductivity in the layered oxyselenides Sr2ZnO2Cu2Se2 and Ba2Zn1−xO2−xCu2Se2

J. Mater. Chem. C, 2024, 12,17574-17586
DOI: 10.1039/D4TC02458C, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Zahida Malik, Sarah Broadley, Sebastian J. C. Herkelrath, Daniel W. Newbrook, Liam Kemp, George Rutt, Zoltán A. Gál, Jack N. Blandy, Joke Hadermann, Daniel W. Davies, Robert D. Smyth, David O. Scanlon, Ruomeng Huang, Simon J. Clarke, Geoffrey Hyett
The optoelectronic properties of two layered copper oxyselenide compounds, with nominal composition Sr2ZnO2Cu2Se2 and Ba2ZnO2Cu2Se2, have been investigated to determine their suitability as p-type conductors.
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Shear-Structured Piezoelectric Accelerometers based on KNN Lead-Free Ceramics for Vibration Monitoring

J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC04292A, Communication
Yi Ding, Yu Wang, Wenbin Liu, Yongqi Pan, Ping Yang, Dechao Meng, Ting Zheng, Jiagang Wu
The process of promoting the transition of piezoelectric devices to lead-free requires consideration from multiple dimensions, including materials, devices and processes. In the key field of vibration monitoring, there has...
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Silver-incorporated NiCo metal–organic frameworks with controlled morphology for enhanced cycling in flexible supercapacitor applications

J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC02970D, Paper
Chu Chu, Wenjing Zhang, Xuehua Yan, Yingnan Yan, Jianmei Pan, Zohreh Shahnavaz, Jamile Mohammadi Moradian
The specific capacitance of NCA15-MOF/NF was 1317 F g−1, which was significantly higher compared to the NCA0-MOF/NF. After 15 000 charge–discharge cycles, the NCA15-MOF/NF retained 89% of its initial specific capacitance.
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Application of metal organic frameworks (MOFs) and their derivatives in the cathode materials of aqueous zinc-ion batteries

J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC03273J, Review Article
Pingchun Guo, Shisong Ouyang, Hedong Jiang, Jiake Li, Hua Zhu, Yanxiang Wang
Metal–organic frameworks (MOFs) are regarded as potential candidate materials for the cathodes of aqueous zinc-ion batteries. This review presents the applications of MOFs and their derivatives in the cathodes of aqueous zinc-ion batteries.
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A metal–organic framework enhanced single network organohydrogel with superior low-temperature adaptability and UV-blocking capability towards human-motion sensing

J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC03148B, Paper
Ying Li, Zhongquan Yu, Jialuo Zhang, Enke Feng, Xiaoqin Li, Linan Cao, Zhiming Yang, Zhiqiang Wu
A UiO-66-NH2 nanoparticle reinforced organohydrogel with anti-freezing and UV-blocking properties was synthesized for sensing complex human movements and transmitting different messages even at subzero temperature.
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Microfluidic synthesis of monodispersed sharp emitting perovskite CsPbBr3 quantum dots via multidimensional parameterization

J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC04104F, Paper
Yunhao Ning, Shuo Guan, Chuantong Cheng, Bao Zhang, Bingyu Qin, Beiju Huang
A microfluidic chip is employed for continuous synthesis of CsPbBr3 perovskite quantum dots, which feature tunable emission across various dimensions and wavelengths, and effects of multidimensional parameters on their properties are investigated.
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Viscoplastic photoalignment modeling of asymmetric surface restructuring in azopolymer films by elliptically polarized light

J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC04226C, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Nina Tverdokhleb, Biagio Audia, Pasquale Pagliusi, Marina Saphiannikova
This study aims to test and validate the modern orientation approach of Saphiannikova & co. within the context of viscoplastic photoalignment (VPA) modeling. We focus on the formation of topographical...
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High-performance solar-blind imaging photodetectors based on micrometer-thick β-Ga2O3 films grown by thermal oxidation of gallium

J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC04116J, Paper
Haitao Zhou, Hongbin Wang, Jiangang Ma, Bingsheng Li, Haiyang Xu, Yichun Liu
A preparation method for micrometer-sized β-Ga2O3 films was developed. The MSM device has a responsivity greater than 1.7 A W−1 and has good solar-blind ultraviolet imaging performance.
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The grapevine, an accurate thermometer of global warming

Grapevines may withstand warmer temperatures of one or two degrees this century, but if the temperature rises four or five degrees, as experts predict, the consequences will be disastrous.



  • Solutions & Co

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Nanomaterial-based regulation of redox metabolism for enhancing cancer therapy

Chem. Soc. Rev., 2024, Advance Article
DOI: 10.1039/D4CS00404C, Review Article
Xiaodan Jia, Yue Wang, Yue Qiao, Xiue Jiang, Jinghong Li
This review provides a comprehensive summary of the dysregulation of redox metabolism in cancer cells and the advantages and the latest advances in nanomaterial-assisted redox metabolic regulation therapy.
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Understanding deNOx mechanisms in transition metal exchanged zeolites

Chem. Soc. Rev., 2024, Advance Article
DOI: 10.1039/D3CS00468F, Review Article
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Jamal Abdul Nasir, Andrew M. Beale, C. Richard A. Catlow
Transition metal-containing zeolites have received considerable attention, owing to their application in the selective catalytic reduction of NOx. To understand their chemistry, both structural and mechanistic aspects at the atomic level are needed.
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Metal–support interactions in metal oxide-supported atomic, cluster, and nanoparticle catalysis

Chem. Soc. Rev., 2024, 53,10450-10490
DOI: 10.1039/D4CS00527A, Review Article
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Denis Leybo, Ubong J. Etim, Matteo Monai, Simon R. Bare, Ziyi Zhong, Charlotte Vogt
Metal–support interactions (MSI) impact catalyst activity, stability, and selectivity. This review critically evaluates recent findings, theoretical advances, and MSI tuning strategies, offering new perspectives for future research in the field.
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From cyclotrons to chromatography and beyond: a guide to the production and purification of theranostic radiometals

Chem. Soc. Rev., 2024, 53,10409-10449
DOI: 10.1039/D4CS00802B, Tutorial Review
Brooke L. McNeil, Caterina F. Ramogida
This tutorial review explores the fundamentals and applications behind the production and purification of radiometals in the burgeoning field of radio-theranostics.
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