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Structural and thermodynamic properties of the Li6PS5Cl solid electrolyte using first-principles calculations

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA05159A, Paper
Tarek Ayadi, Maylise Nastar, Fabien Bruneval
We perform static and dynamic ab initio simulations to investigate the structural and the thermodynamic properties of Li6PS5Cl, a solid electrolyte actively considered for solid-state batteries. Our simulations account for...
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Bifunctional conjugated polymer photocatalysts for visible light water oxidation and CO2 reduction: function- and site-selective hybridisation of Ru(II) complex catalysts

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J. Mater. Chem. A, 2024, 12,30279-30288
DOI: 10.1039/D4TA04014G, Paper
Kotaro Ishihara, Akinobu Nakada, Hajime Suzuki, Osamu Tomita, Shunsuke Nozawa, Akinori Saeki, Ryu Abe
Function-/site-selective hybridisation of two specific Ru(II) complex catalysts on donor–acceptor conjugated polymers enables bifunctional visible-light water oxidation and CO2 reduction.
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Electrode process regulation for high-efficiency zinc metal anodes

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J. Mater. Chem. A, 2024, 12,30169-30189
DOI: 10.1039/D4TA05143B, Review Article
Longkun Wu, Xinyan Zhu, Zhi Peng, Zekun Zhang, Ningning Zhao, Bin Li, Jing Zhu, Lei Dai, Ling Wang, ZhangXing He
Regulation strategies for zinc anode ion deposition.
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Enhanced electrocatalytic overall alkaline water splitting induced by interfacial electron coupling of Mn3O4 nano-cube@CeO2/γ-FeOOH nanosheet hetero-structure

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J. Mater. Chem. A, 2024, 12,30783-30797
DOI: 10.1039/D4TA05336B, Paper
Debasish Ghosh, Dimple K. Bora, Asit Baran Panda
Mn3O4@CeO2/γ-FeOOH hetero-structure showed interfacial electron coupling induced superior bifunctional electrocatalytic activity suitable for AEM electrolyser.
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Tuning the acidity and textural properties of polyethyleneimine-supported adsorbents for enhanced economical CO2 capture

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J. Mater. Chem. A, 2024, 12,30309-30317
DOI: 10.1039/D4TA05215C, Paper
Bitan Ray, Sathyapal R. Churipard, Arjun Cherevotan, Diku Raj Deka, Devender Goud, Harishankar Kopperi, Sebastian C. Peter
The acidity and textural properties of polyethyleneimine-supported adsorbents are tuned to enhance the capture of carbon dioxide in an economical way.
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Modulating the band gap of a pyrazinoquinoxaline-based metal–organic framework through orbital hybridization for enhanced visible light-driven CN bond construction

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J. Mater. Chem. A, 2024, 12,30582-30590
DOI: 10.1039/D4TA06282E, Paper
Zitong Chen, Linghui Cao, Aogang Liu, Pengda Liu, Yuan Chen, Juntao Yan, Bao Li
An indium-based metal–organic framework bearing a pyrazinoquinoxaline derivative is synthesized to facilitate two methods for the construction of CN bonds, and their mechanisms are investigated through detailed theoretical calculations.
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A matter of design and coupling: high indoor charging efficiencies with organic solar modules directly coupled to a sodium ion battery

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J. Mater. Chem. A, 2024, 12,30862-30871
DOI: 10.1039/D4TA04729J, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Li-Chung Kin, Andreas Distler, Oleksandr Astakhov, Bakary Kone, Hans Kungl, André Karl, Tsvetelina Merdzhanova, Rüdiger-A. Eichel, Christoph J. Brabec, Uwe Rau
Generalized framework for the design of indoor power units for autonomous Internet of Things (IOT) devices results in record efficiency combination of organic PV and sodium ion battery.
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Fe-single-atom-coupled Fe3C multifunctional catalysts on P-, F-, N-doped carbon nanotubes for stable Zn–air batteries with ultra-high power densities

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J. Mater. Chem. A, 2024, 12,30798-30809
DOI: 10.1039/D4TA04194A, Paper
Manigandan Ramadoss, Hesheng Yu, Anand Rajkamal, Gun Jin Yun, Ziheng Zhang, Chengtao Yang, Fei Ma, Yu Wu, Chen Daiqian, Yuanfu Chen
Fe-single-atom-coupled Fe3C multifunctional catalysts on P-, F-, N-doped CNT deliver comparable OER behavior to RuO2, better ORR performance than Pt/C, and better ZAB performance than Pt/C–RuO2, due to the nanoarchitecture and abundant active sites.
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Free-standing films of nickel nanowires anchored with Ni3S2 nanosheets for stable Li anodes

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J. Mater. Chem. A, 2024, 12,30534-30547
DOI: 10.1039/D4TA06163B, Paper
Yang Xu, Gang Li, Jiangtao Hai, Hewei Yuan, Haotian Weng, Kun Li, Xiaolu Huang, Yanjie Su, Nantao Hu, Yafei Zhang
A free-standing 3D scaffold of nickel nanowires decorated with lithiophilic Ni3S2 nanosheets was successfully constructed for stable Li anodes.
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Ultrathin two-dimensional membranes by assembling graphene and MXene nanosheets for high-performance precise separation

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J. Mater. Chem. A, 2024, 12,30121-30168
DOI: 10.1039/D4TA05097E, Review Article
Yifan He, Shanshan Guo, Xueji Zhang, Lijun Qu, Tingting Fan, Jinlei Miao
Ultrathin 2D membranes were assembled by graphene and MXene nanosheets for separation to overcome the “trade-off” limitation between permeability and selectivity.
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Unsaturated coordination modulation and enlarged pore size in nanoflower-like metal organic frameworks for enhanced lithium–oxygen battery performance

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J. Mater. Chem. A, 2024, 12,30591-30600
DOI: 10.1039/D4TA06346E, Paper
Lingwen Zhao, Juanjuan Feng, Adeel Abbas, Hao Sun, Chunlei Wang, Hongchao Wang
Unsaturated coordination modulation alters the discharge path and increased pore size accelerates ion exchange and oxygen transport, synergistically improving the electrochemical performance of LOBs.
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An advanced passive radiative cooling emitter with ultrahigh sub-ambient cooling performance

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J. Mater. Chem. A, 2024, 12,30351-30361
DOI: 10.1039/D4TA05869K, Paper
Jiawei Huang, Weifeng Chen, Qiyan Kuang, Ting Xiao, Lihua Jiang, Xinyu Tan, Yizhu Lei
This study develops a state-of-the-art passive radiative cooling emitter with 95.5% reflectance and 97.9% emissivity, achieving an average temperature reduction of 20.1 °C and a cooling power of 121.0 W m−2 under intense sunlight.
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Multifunctional characteristics of a one-dimensional bimetallic oxyhydroxide nanorod-coupled polyaniline interface for accelerated water and urea electrolysis

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J. Mater. Chem. A, 2024, 12,30743-30756
DOI: 10.1039/D4TA05082G, Paper
Niranjanmurthi Lingappan, Sandhiya Lakshmanan, Wonoh Lee
Designing an efficient and durable electrocatalyst is central to hydrogen production technologies such as hydrogen evolution reaction, oxygen evolution reaction, and urea oxidation reaction.
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Recyclable microcellular rubber foams with superior photothermal performance via constructing Fe3+ heterodentate coordination between epoxidized natural rubber and polyaniline

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J. Mater. Chem. A, 2024, 12,30486-30497
DOI: 10.1039/D4TA06543C, Paper
Jingyi Zhu, Yukun Chen, Patrick C. Lee, Shuidong Zhang
Developing recyclable microcellular rubber foams with excellent photothermal conversion ability can reduce resource waste and harvest solar energy to alleviate environmental pollution and the energy crisis simultaneously.
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Optimization of the electron transfer kinetics between a photoanode and biocathode for enhanced carbon-neutral pollutant removal in photocatalytic fuel cells

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J. Mater. Chem. A, 2024, 12,30371-30379
DOI: 10.1039/D4TA05290K, Paper
Xiaofei Gu, Jianyu Han, Zhi Wang, Yixin Hong, Tianyi Huang, Yafeng Wu, Yuanjian Zhang, Songqin Liu
A PFC system with collaborative dynamics between the photoanode and biocathode is constructed for using solar energy to efficiently convert refractory organic pollutants into green fuel and generate electricity.
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Synthesis of a Cu@ZnO1−x/Al2O3 catalyst with high-density ZnO1−x–Cu interfacial sites for enhanced CO2 hydrogenation to methanol

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J. Mater. Chem. A, 2024, 12,30692-30706
DOI: 10.1039/D4TA05801A, Paper
Yunshuo Wu, Haiqiang Wang, Zhongbiao Wu
The development of catalysts with high-density interfacial sites is crucial for enhancing catalytic performance.
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Sulfur-doped g-C3N4/V2C MXene Schottky junctions for superior photocatalytic H2 evolution

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J. Mater. Chem. A, 2024, 12,30429-30441
DOI: 10.1039/D4TA05929H, Paper
Haitao Wang, Jipeng Fan, Jing Zou, Yujie Zheng, Dingsheng Wang, Jizhou Jiang
An advanced sulfur-doped g-C3N4/V2C MXene (SCN/V2C) Schottky junction HER photocatalyst was prepared via vacuum ball milling and subsequent annealing.
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Multifunctional additive enables lead-adsorbing carbon electrodes for perovskite solar cells

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J. Mater. Chem. A, 2024, 12,30611-30617
DOI: 10.1039/D4TA05429F, Paper
Yuanzhu Jiang, Aodong Zhu, Teng Liao, Wang Zhao, Mengmeng Cheng, Xinxin Zhang, Yi-Bing Cheng, Junyan Xiao
Phosphate, being a single-component multifunctional additive, serves as a viable material for the carbon electrode in perovskite solar cells. This utilization ensures the device's performance and mitigates the risk of potential lead pollution.
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Sodium storage performance of a high entropy sulfide anode with reduced volume expansion

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J. Mater. Chem. A, 2024, 12,30629-30641
DOI: 10.1039/D4TA05122J, Paper
Jianping Ma, Jinyi Guo, Weizheng Li, Xiaohan Yang, Chengde Huang
The introduction of a high-entropy structure into multi-metal sulfides has successfully mitigated volume expansion during the cycling process of sodium-ion batteries!
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Rational engineering and synthesis of pyrene and thiazolo[5,4-d]thiazole-functionalized conjugated microporous polymers for efficient supercapacitor energy storage

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J. Mater. Chem. A, 2024, 12,30508-30521
DOI: 10.1039/D4TA05908E, Paper
Abdul Basit, Yang-Chin Kao, Yasser A. El-Ossaily, Shiao-Wei Kuo, Mohamed Gamal Mohamed
The Py-Th-TzTz CMP was synthesized through a Schiff base reaction and exhibited a decomposition temperature (Td10) of 352 °C. In a three-electrode system, it demonstrated a specific capacitance of 652 F g−1.
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Enhancing the surface Lewis basicity of phosphorene-hosted NiO nanosheets for sensitive and selective H2S gas sensing

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J. Mater. Chem. A, 2024, 12,30380-30387
DOI: 10.1039/D4TA05682E, Paper
Yahui Tian, Wenfang Zhai, Jie Su, Yuxin Zhao, Zhengfei Dai, Wei Gan, Hui Li
A black phosphorene-hosted NiO nanosheet heterostructure achieves enhanced surface Lewis basicity, delivering sensitive and selective sensor properties to trace H2S gas.
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Tailoring biobased polythiourethane crosslinking networks with flame-retardancy and remote ultrafast infrared “welding” performance

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J. Mater. Chem. A, 2024, 12,30398-30408
DOI: 10.1039/D4TA05966B, Paper
Ning Ding, Yi Yang, Wei Zhou, Debora Puglia, Pengwu Xu, Deyu Niu, Weijun Yang, Piming Ma
Biobased polythiourethane/MXene nanocomposites with intrinsic flame-retardancy and remote ultrafast infrared “welding” performance.
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Probing the key roles of the back interface in the performance of carbon-based hole-transport-layer free perovskite solar cells

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J. Mater. Chem. A, 2024, 12,30388-30397
DOI: 10.1039/D4TA06143H, Paper
Xinwei Li, Nianqing Fu, Xiaocao Peng, Hehui Lin, Jiaang Cheng, Ziming Chen, Peng Lin, Jun Du
The key roles of perovskite films in the photovoltaic performance of carbon-based PSCs employing various absorbers were comprehensively studied and elucidated.
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One-pot spatial engineering of multi-enzymes in metal–organic frameworks for enhanced cascade activity

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J. Mater. Chem. A, 2024, 12,30318-30328
DOI: 10.1039/D4TA06211F, Paper
Wenqing Fan, Kang Liang, Jieying Liang
A one-pot strategy was developed for the first time to achieve the precise spatial arrangement of multiple enzymes in MOFs, improving multi-enzyme cascade efficiency.
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Achieving dynamic stability of single-crystal low-Co Ni-rich cathode material for high performance lithium batteries

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J. Mater. Chem. A, 2024, 12,30831-30841
DOI: 10.1039/D4TA04698F, Paper
Adil Saleem, Leon L. Shaw, Mehwish Khalid Butt, Javed Rehman, Arshad Hussain, Zawar Hussain, Rashid Iqbal, Muhammad Kashif Majeed
The demand for high-energy-density lithium-ion batteries (LIBs) has driven intensive research into cathode materials that exhibit both superior performance and stability over multiple charge–discharge cycles.
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Advancing energy safety via stepwise nucleophilic substitution on tetrazine

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J. Mater. Chem. A, 2024, 12,30548-30557
DOI: 10.1039/D4TA06039C, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Jatinder Singh, Richard J. Staples, Jean'ne M. Shreeve
This study presents a feasible approach to synthesizing hydrazine/nitroamine and amino/nitroamine substituted tetrazine derivatives.
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A sustainable redox-mediated pathway for improved transition metal organic framework activation and CO2 uptake performance

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J. Mater. Chem. A, 2024, 12,30454-30464
DOI: 10.1039/D4TA02526A, Paper
Taylor Jade Self, Jiabin Niu, Wen Liu, Chaobin He, Mei Chee Tan
Sustainable substitutions in MOF fabrication and processing can confidently be made by employing redox engineering for synergistic valency and defect constitution, based on application, without sacrificing active site functionality.
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Smart fabrics with liquid metal reinforced PU/CNT/MXene multilayer structures for constructing multifunctional sensors and wearable electronics

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J. Mater. Chem. A, 2024, 12,30872-30884
DOI: 10.1039/D4TA05266H, Paper
Haijiao Lin, Hui Wang, Yongguang Yang, Yuxuan Zhang, Ling Li, Youwei Zhao, Wenming Zhang
Smart fabrics with liquid metal reinforced PU/CNT/MXene multilayer structures for constructing multifunctional sensors and wearable electronics.
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Development and application of Few-shot learning methods in materials science under data scarcity

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J. Mater. Chem. A, 2024, 12,30249-30268
DOI: 10.1039/D4TA06452F, Review Article
Yongxing Chen, Peng Long, Bin Liu, Yi Wang, Junlong Wang, Tian Ma, Huilin Wei, Yue Kang, Haining Ji
Machine learning, as a significant branch of artificial intelligence, shortens the cycle of material discovery and synthesis by exploring the characteristics of data.
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Electrode–electrolyte interphases in lithium-based rechargeable batteries with ionic liquid electrolytes: recent advances and future perspectives

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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06184E, Review Article
Taohong He, Yushan Han, Bofang Shi, Jianan Wang, Honghui Yang
The characteristics of interphase formation between ionic liquid-based electrolytes and various electrodes are reviewed to support the development of improved electrolyte designs for lithium-based batteries.
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Dually encapsulated LiMn0.6Fe0.4PO4 architecture with MXenes and amorphous carbon to achieve high-performance and ultra-stable lithium batteries

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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06323F, Paper
Yang Song, Haidong Zhong, Tingting Hu, Qizhi Chen, Lei Shi, Jun Du, Changyuan Tao, Qian Zhang
An LMFP@MXene@C cathode material was fabricated by electrostatic adsorption and in situ graphitization, providing optimized Li+ transmission and a stable structure featuring ultrahigh average capacity and cycle stability.
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Recent Advances on Non-noble Metal Catalysts toward N-ethylcarbazole Hydrogen Storage

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06468B, Review Article
Hansai Wu, junming Zhang, Zicong Wang, Xianglong Kong, Gaofu Li, Ying Zhao, Piaoping Yang, Zhiliang Liu
N-ethylcarbazole (NEC) hydrogen storage has garnered significant attention owing to its large-scale safe storage of hydrogen superiority. However, the sluggish hydrogenation kinetics in NEC are extremely dependent on catalysts with...
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Enhanced oxygen exchange kinetics and long-term stability of Ruddlesden-Popper phase Pr4Ni3O10+δ cathode for solid oxide fuel cells

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA01845A, Paper
Saim Saher, Affaq Qamar, Chou Yong Tan, Singh Ramesh, Walied Alfraidi
This research explores the intricacies of oxygen exchange kinetics in Pr4Ni3O10+δ (PNO), aiming to assess its potential as a viable cathode material for solid oxide fuel cell applications. Utilizing a...
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Recent Advances p-type Polymeric Electrode Materials towards High-Voltage 4.0 V-class Organic Lithium-ion Batteries

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06028H, Review Article
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Febri Baskoro, Santosh U. Sharma, Andre Lammiduk Lubis, Hung-Ju Yen
Lithium-ion batteries stand at the forefront of energy storage technologies, facilitating the transition towards sustainable and electrified systems. To meet the increasing demands for energy density, safety, and longevity, the...
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Regulating oxygen redox reactions in lithium-rich materials via an Al2O3-doped ZnO layer for enhanced stability and performance

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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06843B, Paper
Xinyu Cheng, Yuke Wang, Jia Lu, Wangqi Dai, Huanhao Lei, Jinning Zuo, Hong Li, Zhengwen Fu
An ultrathin Al2O3-doped ZnO (AZO) layer on LRM regulates oxygen redox by suppressing anion migration and inhibiting surface oxygen oxidation, enhancing cycling performance.
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Machine learning aided design of high performance copper-based sulfide photocathodes

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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06128D, Paper
Yuxi Cao, Kaijie Shen, Yuanfei Li, Fumei Lan, Zeyu Guo, Kelu Zhang, Kang Wang, Feng Jiang
With the help of machine learning algorithms, we developed software that can predict the performance of copper-based sulfide photocathodes and this system shows excellent accuracy of up to 96%.
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Retraction: Thermally reduced graphene oxide/polymelamine formaldehyde nanocomposite as a high specific capacitance electrochemical supercapacitor electrode

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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA90211D, Retraction
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Ali A. Ensafi, Hossein A. Alinajafi, B. Rezaei
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Advancing Paper-Based Sensors with MXenes and MOFs: Exploring the Cutting-Edge Innovations

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06561A, Review Article
Sepehr Larijani, Atefeh Zarepour, Arezoo Khosravi, Siavash Iravani, Mahnaz Eskandari, Ali Zarrabi
MXenes and metal-organic frameworks (MOFs) are emerging as promising materials for integration into paper-based sensors (PSs), offering unique properties that can enhance sensor performance in various applications. MXenes, with their...
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Vertical Macroporous Chitosan Aerogel Adsorbents for Simple and Efficient Enhancement of Atmospheric Water Harvesting and Air Dehumidification

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA07005D, Paper
Zhiguang Guo, Changhui Fu, Yuxuan He, Anhui Yu, Guangyi Tian, Danyan Zhan, Huimin Zhang
Adsorption-based atmospheric water harvesting (SAWH) has become one of the effective methods to extract water from the air in arid regions due to its high efficiency and low energy consumption....
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Pre-lithiation carbon anodes mitigating potassium loss toward for high-performance potassium-ion energy storage devices

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06451H, Paper
Danni Du, Qingyuan Liu, Jing Gao, Yuying Qin, Xiaobo Jiang, Yuanchang Shi, Minghao Hua, Xiaohang Lin, Zhiwei Zhang, Chengxiang Wang, Long-Wei Yin, Rutao Wang
Pre-potassiation technologies with the functions of providing additional potassium sources and/or mitigating potassium loss during cycling, make them capable of enhancing the energy density and cycling life of potassium-ion capacitors...
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Radiofrequency-Triggered Surface-Heated Laser-Induced Graphene Membranes for Enhanced Membrane Distillation

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA05611F, Paper
Md Hasib Al Mahbub, Fouzia Hasan Nowrin, Mohammad Saed, Mahdi Malmali
Membrane distillation (MD) has attracted significant research interest for desalinating hypersaline brine. However, the lack of robust hydrophobic membrane and lower energy efficiency requirements restrict its true potential. Designing and...
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Flexible multifunctional MXene@Ag nanowires/cotton fabric inspired by transport of nutrients by roots for electromagnetic shielding, infrared stealth, Joule/solar heating and flame retardancy

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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06712F, Paper
Jiatong Yan, Meimei Chen, Rui Tan, Chuanxi Lin, Shan Jiang, Weijie Wang, Songyue Pan, Hongyan Xiao, Erhui Ren, Ronghui Guo
With the rapid development of 5G intelligent detection technology, electromagnetic shielding/infrared stealth fabrics with Joule/solar heating performance can meet the needs of wearable electronic devices for multi-application scenarios.
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Synergetic Effects from a High-Entropy NASICON-type Cathode for Advanced Sodium-Ion Batteries

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06950A, Paper
Shouyue Wang, Taiding Xu, Huitao Leng, Shengyu Liang, Wei Zhang, Yuheng Jin, Jingxia Qiu, Sheng Li
Na3V2(PO4)3 (NVP) is recognized as one of the most promising NASICON-type cathodes for sodium-ion storage. Enhancing electronic conductivity and further ensuring long-term structural stability when activating the high-voltage V⁴⁺/V⁵⁺ redox...
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High-throughput Screening of Mechanically Interlocked Catenane Metal Complexes for Enhanced Electrocatalytic Activity

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06497F, Paper
Mohsen Tamtaji, William A. Goddard III, Guanhua Chen
Metal complexes have been thoroughly investigated for a wide range of electrochemical reactions. However, mechanically interlocked molecular machines (MIM) have not been investigated for electrochemistry through a systematic high throughput...
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Ternary NiFeCo-Glycerolate Catalysts: Rational Design for Improved Oxygen Evolution Reaction Efficiency

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J. Mater. Chem. A, 2024, Accepted Manuscript
DOI: 10.1039/D4TA06455K, Paper
Irlan Santos Lima, Josué M. Gonçalves, Lúcio Angnes
Catalysts capable of overcoming the bottleneck of water splitting, known as the oxygen evolution reaction (OER), are indispensable to the expansion of renewable energy systems. Thus, we report the synthesis...
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