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Visible Light-Induced Aerobic Oxidation of Diarylalkynes to -Diketones Catalyzed by Copper-superoxo at Room Temperature

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00975J, Communication
Vaibhav Pramod Charpe, Arunachalam Sagadevan, Kuo Chu Hwang
We have developed the visible light induced simple copper(II) chloride catalyzed the oxidation of diarylacetylenes to -diketones by molecular oxygen at room temperature. The in-situ generated copper(II)-superoxo complex is a...
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Bio-based benzoxazine surfactant from amino acid

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00218F, Paper
Zheng Wang, Shu Yao, Kun Song, Xinjian Gong, Sujuan Zhang, Sheng Gao, Zaijun Lu
A novel bio-based benzoxazine (Ca-g) surfactant was synthesized via a Mannich reaction using renewable glycine and cardanol as raw materials. The structure of Ca-g was characterized by NMR, FT-IR, and...
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Visible-light-promoted oxidative desulphurisation: a strategy for the preparation of unsymmetrical ureas from isothiocyanates and amines using molecular oxygen

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00070A, Paper
Ziyu Gan, Guoqing Li, Qiuli Yan, Weiseng Deng, Yuan-Ye Jiang, Daoshan Yang
A green and efficient visible-light promoted oxidative desulphurisation protocol has been proposed for the construction of unsymmetrical ureas under mild conditions with broad substrate scope and good functional group tolerance.
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Sustainable remediation with an electroactive biochar system: mechanisms and perspectives

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00717J, Critical Review
Zhonghao Wan, Yuqing Sun, Daniel C. W. Tsang, Deyi Hou, Xinde Cao, Shicheng Zhang, Bin Gao, Yong Sik Ok
Biochar-based carbocatalysis is synergized from electroactive components including reactive-active moieties, metals, defective sites, heteroatoms, and graphitic structure for sustainable remediation.
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Continuous hydroformylation of 1-decene in an aqueous biphasic system enabled by methylated cyclodextrins

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00820F, Paper
Open Access
K. U. Künnemann, L. Schurm, D. Lange, T. Seidensticker, S. Tilloy, E. Monflier, D. Vogt, J. M. Dreimann
Long-term applications of cyclodextrins in the aqueous biphasic hydroformylation of higher olefins with high selectivities and simultaneous catalyst recycling.
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Boron-doped CuO nanobundles for electroreduction of carbon dioxide to ethylene

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00730G, Communication
Qiang Wan, Jianling Zhang, Bingxing Zhang, Dongxing Tan, Lei Yao, Lirong Zheng, Fanyu Zhang, Lifei Liu, Xiuyan Cheng, Buxing Han
Herein, we synthesize B-doped CuO nanobundles for electrocatalytic CO2 reduction. Ethylene is the only multi-carbon product and a maximum ethylene faradaic efficiency (FE) of 58.4% can be achieved at −1.1 V (versus the reversible hydrogen electrode).
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Chemoselective O-formyl and O-acyl protection of alkanolamines, phenoxyethanols and alcohols catalyzed by nickel(II) and copper(II)-catalysts

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00520G, Paper
Rahul B. Sonawane, Swapnali R. Sonawane, Nishant K. Rasal, Sangeeta V. Jagtap
A crucial chemoselective O-formyl and O-acyl protection of alkanolamines, phenoxyethanols, and alcohols in the presence of amines catalyzed by Ni(II) and Cu(II) complexes with 8-hydroxyquinoline in a homogeneous medium is achieved.
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Degradation of poly(ethylene terephthalate) catalyzed by metal-free choline-based ionic liquids

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00327A, Paper
Yachan Liu, Xiaoqian Yao, Haoyu Yao, Qing Zhou, Jiayu Xin, Xingmei Lu, Suojiang Zhang
Glycolysis of PET is a prospective way for degradation of PET to its monomer bis(hydroxyethyl)terephthalate (BHET) which can be polymerized again to form new qualified PET materials, and hence provides possibilities for a permanent loop recycling.
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One-step catalytic amination of naphthalene to naphthylamine with exceptional yield

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00633E, Communication
Fang Hao, Xin Wang, Linfang Huang, Wei Xiong, Pingle Liu, Hean Luo
This is the first time to synthesize naphthylamine from one-step naphthalene amination by vanadium catalysts with high yield under mild condition. It could obtain ∼70% yield of naphthylamine, with major product of valuable 1,5-diaminonaphthalene.
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Highly efficient bioconversion of flavonoid glycosides from citrus-processing wastes in solvent-buffer systems

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00669F, Paper
Yucong Zou, Xuan Xin, Haixia Xu, Hongwei Yuan, Xiaofeng Li, Yigang Yu, Guanglei Zhao
The present study demonstrates that whole-cell catalysis is a good choice to hydrolyze citrus flavonoid glycosides and their derivatives.
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Nickel-catalyzed and Li-mediated regiospecific C–H arylation of benzothiophenes

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00917B, Paper
Yorck Mohr, Gaëlle Hisler, Léonie Grousset, Yoann Roux, Elsje Alessandra Quadrelli, Florian M. Wisser, Jérôme Canivet
A sustainable nickel-catalyzed direct C–H arylation of benzothiophenes, benzofuran and selenophene is reported for the first time.
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Mechanochemical Cleavage of Lignin Models and lignin via Oxidation and Subsequent Base-Catalyzed Strategy

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00372G, Paper
Weike Su, Chen Sun, Lei Zheng, Wenhao Xu, Alexandr V. Dushkin
Mechanochemical cleavage of lignin dimer model compounds to phenolic monomers has been developed via a two-step strategy under milling conditions. In the first step of this process, the secondary benzylic...
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Role of life-cycle externalities in the valuation of protic ionic liquids – a case study in biomass pretreatment solvents

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00058B, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Husain Baaqel, Ismael Díaz, Víctor Tulus, Benoît Chachuat, Gonzalo Guillén-Gosálbez, Jason P. Hallett
The combination of LCA and monetization has revealed that protic ionic liquids can be sustainable alternatives to conventional solvents.
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Achieving visible light-driven hydrogen evolution at positive bias with a hybrid copper–iron oxide|TiO2-cobaloxime photocathode

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00979B, Paper
C. Tapia, E. Bellet-Amalric, D. Aldakov, F. Boudoire, K. Sivula, L. Cagnon, V. Artero
H2 is an environmentally-friendly fuel that would allow for a circular economy but its sustainable production from solar energy and water using stable, efficient and scalable Earth-abundant materials, remains a challenge.
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Ethyl lactate participated three-component dehydrogenative reactions: biomass feedstock in diversity oriented quinoline synthesis

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00738B, Communication
Lu Yang, Jie-Ping Wan
Ethyl lactate participated three-component dehydrogenative reactions: biomass feedstock in diversity oriented quinoline synthesis
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Photocatalytic Hydrogen Atom Transfer: the Philosopher’s Stone for Late-Stage Functionalization?

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC01035A, Tutorial Review
Luca Capaldo, Lorenzo Lafayette Quadri, Davide Ravelli
An overview about the potentialities of photocatalytic Hydrogen Atom Transfer (HAT) for the Late-Stage Functionalization (LSF) of complex molecules is offered. The examined approach allows the smooth homolytic cleavage of...
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Development and validation of an ecofriendly HPLC-DAD method for the determination of oleuropein and its applicability to several matrices: olive oil, olive leaf extracts and nanostructured lipid carriers.

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00965B, Paper
Amaia Huguet-Casquero, Tania Belen Lopez-Mendez, Eusebio Gainza, Jose Luis Pedraz
Oleuropein is a natural ingredient largely used in nutritional supplements. This study reports on the development, validation and application of an HPLC method based on UV-vis detection for determining oleuropein...
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Sulfonic acid modified hollow polymer nanospheres with tunable wall-thickness for improving biodiesel synthesis efficiency

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00905A, Paper
Wenliang Song, Yu Zhang, Anuraj Varyambath, Ji Su Kim, Il Kim
Precisely designing the morphology and size of nanostructures is vital in green chemistry as various advanced applications depend upon the shapes and dimensions of the functionalised materials. Herein, we report...
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MOFs come up to scratch: an environmentally benign route to oxidative [4 + 2] cycloaddition on maleimides solely via MOFs in water

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00619J, Paper
Masoumeh Abbasnia, Mehdi Sheykhan, Mona Bahmani, Parvaneh Taghizadeh
The first Diels–Alder reaction of vinyl arenes with ene systems catalyzed by MOFs is reported.
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Tandem catalytic aromatization of volatile fatty acids

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00964D, Paper
Open Access
Egor V. Fufachev, Bert M. Weckhuysen, Pieter C. A. Bruijnincx
The transition towards a circular economy requires closing the carbon loop, e.g. by the development of new synthesis routes to valuable intermediates and products from organic-rich waste streams.
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Scalable synthesis and polymerisation of a β-angelica lactone derived monomer

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00338G, Paper
Open Access
Andrea Dell'Acqua, Bernhard M. Stadler, Sarah Kirchhecker, Sergey Tin, Johannes G. de Vries
A new bio-based norbornene polymer was prepared starting from β-angelica lactone, prepared in a sustainable and scalable manner from the platform chemical levulinic acid. The new material displays transparency comparable to petrochemical-derived polynorbornene.
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Chemistry of electrochemical oxidative reactions of sulfinate salts

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC01025A, Tutorial Review
Haibo Mei, Romana Pajkert, Li Wang, Ziyi Li, Gerd-Volker Röschenthaler, Jianlin Han
Recent advances in the oxidative reactions of sulfinate salts under electrochemical conditions, and the reaction mechanism are discussed.
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Yb(OTf)3 and Visible Light Relay Catalyzed [3+2] Cycloaddition/[3,3]-Rearrangement/[4+2] Cycloaddition in One Pot to Prepare Oxazonine-Fused Endoperoxides

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00929F, Paper
Xiao-Pan Ma, Cai-Mei Nong, Yu-Feng Liang, Pei-Pei Xu, Xiu-Yun GUO, Cui Liang, Chengxue Pan, Gui-Fa SU, Dong-Liang Mo
We report a relay catalysis for the highly stereoselective synthesis of densely substituted oxazonine-fused endoperoxides in good yields. This domino reaction is based on a Yb(OTf)3 and visible light promoted...
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Microwave-assisted aqueous carbon–carbon cross-coupling reactions of aryl chlorides catalysed by reduced graphene oxide supported palladium nanoparticles

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00833H, Paper
Qingxiao Zhang, Zhan Mao, Kaixuan Wang, Nam Thanh Son Phan, Fang Zhang
Microwave-assisted reduced graphene oxide supported palladium nanoparticles can efficiently promote aqueous Ullmann and Suzuki coupling reactions of aryl chlorides.
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Functionalized magnetic nanosized materials for efficient biodiesel synthesis via acid–base/enzyme catalysis

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00924E, Critical Review
Anping Wang, Putla Sudarsanam, Yufei Xu, Heng Zhang, Hu Li, Song Yang
This critical review introduces the preparation methods, structural and performance control, protection, and functionalization of magnetic nanoparticles as easily recyclable and efficient heterogeneous catalysts for biodiesel synthesis.
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Metal-catalysed selective transfer hydrogenation of α,β-unsaturated carbonyl compounds to allylic alcohols

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00855A, Critical Review
Ronald Alvaro Alvaro Farrar Tobar, Andrea Dell'Acqua, Sergey Tin, Johannes G. de Vries
Allylic alcohols are highly important compounds which are used in a variety of processes. They can be obtained from α,β-unsaturated carbonyl compounds via stoichiometric or catalytic reductions. Catalytic transfer hydrogenation...
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Highly efficient oxidation of alcohols to carboxylic acids using a polyoxometalate-supported chromium(III) catalyst and CO2

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00388C, Paper
Ying Wang, ZhiKang Wu, Han Yu, Sheng Han, Yongge Wei
A green and highly efficient oxidation of alcohols to carboxylic acids using a polyoxometalate-supported chromium(III) catalyst and CO2.
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A safe and compact flow platform for the neutralization of a mustard gas simulant with air and light

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC01142H, Communication
Noémie Emmanuel, Pauline Bianchi, Julien Legros, Jean-Christophe M. Monbaliu
Intensified chemical neutralization of a chemical warfare agent simulant CEES with air and light under continuous flow conditions.
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Cracking of squalene into isoprene as chemical utilization of algae oil

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00268B, Communication
Kazuya Kimura, Kazuma Shiraishi, Takahiro Kondo, Junji Nakamura, Tadahiro Fujitani
Thermal decomposition of squalene proceeds as a chain reaction to produce isoprene (C5H8) and C10 hydrocarbons.
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Incorporation of novel degradable oligoester crosslinkers into waterborne pressure sensitive adhesives: towards removable adhesives

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00463D, Paper
Fabian Wenzel, Amaia Agirre, Miren Aguirre, Jose Ramon Leiza
Novel partially degradable waterborne pressure sensitive adhesives can be easily removed from substrates under mild alkali conditions opening the door for sustainable (less solvent and energy consumption) recycling processes.
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Photochemical strategies for C–N bond formation via metal catalyst-free (hetero) aryl C(sp2)–H functionalization

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC01088J, Tutorial Review
Qing-Qing Kang, Wenfeng Wu, Qiang Li, Wen-Ting Wei
The development of efficient and mild methods to assemble C–N bonds represents an important and appealing goal in modern synthetic chemistry.
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Boosting the efficiency of solution-based CZTSSe solar cells by using supercritical carbon dioxide treatment

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC01355B, Paper
Hai-Qin Xiao, Wen-Hui Zhou, Dongxing Kou, Zheng-Ji Zhou, Yue-Na Meng, Yafang Qi, Shengjie Yuan, Qingwen Tian, Si-Xin Wu
Cu2ZnSn(S,Se)4 (CZTSSe) solar cells are receiving considerable attention in recent years, owing to the low cost and toxicity as well as high abundance of their constituent elements. Solution-based (mainly precursor...
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Electrochemical Oxidative C(sp3)-H Azolation of Lactams Under Mild Conditions

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00687D, Communication
Zhaohua Wan, Dan Wang, Zixuan Yang, Heng Zhang, Shengchun Wang , Aiwen Lei
Lactam-containing structural compounds are ubiquitous in drugs and biomolecules. An electrochemical oxidative direct C(sp3)-H azolation of lactams has been reported under metal catalyst free and external oxidant free conditions. This...
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Photochemical Synthesis of Acetals utilizing Schreiner’s Thiourea as the Catalyst

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC01135E, Paper
Open Access
Nikoleta Spiliopoulou, Nikolaos Nikitas, Christoforos G Kokotos
Acetalization of aldehydes is an area of great importance in Organic Chemistry for both synthetic and biological puproses. Herein, we report a mild, inexpensive and green photochemical protocol, where Schreiner’s...
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Reporting the unreported: the reliability and comparability of the literature on organic solvent nanofiltration

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00775G, Perspective
Hai Anh Le Phuong, Christopher F Blanford, Gyorgy Szekely
Organic solvent nanofiltration (OSN) is an energy-efficient separation technique that has the potential to improve environmental sustainability in many industrial sectors, including food processing, biorefineries, and in the production of...
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Humidity-responsive Molecular Gate-opening mechanism for Gas Separation in Ultraselective Nanocellulose/IL Hybrid Membranes

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00544D, Paper
Saravanan. Janakiram, Luca Ansaloni, Soo Ah Jin, Xinyi Yu, Zhongde Dai, Richard J Spontak, Liyuan Deng
Nanofibrillated cellulose (NFC) represents an important class of bio-based nanomaterials that possess favorable properties including hydrophilicity, 1D structure, biodegradability, and surface tunability. Although widely known for its effective gas-barrier attributes...
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A direct conversion of blast furnace slag to a mesoporous silica–calcium oxide composite and its application in CO2 captures

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00722F, Paper
Yasutaka Kuwahara, Aiko Hanaki, Hiromi Yamashita
A facile and cost-effective approach is presented that converts blast furnace slag into a mesoporous silica-CaO composite possessing high CO2 adsorption performance.
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Catalyst-Free Photodecarbonylation of 2-Amine Benzaldehyde

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC01256D, Communication
Jingwei Zhou, Lamei Li, Songping Wang, Ming Yan, Wentao Wei
It is almost a consensus that decarbonylation of aldehyde group (-CHO) need to not only be mediated by transition metal catalysts, but also react under severe reaction conditions (high temperature...
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Aqueous Phase Fabrication and Conversion of Pb(OH)Br into CH3NH3PbBr3 Perovskite and its Application in Resistive Memory Switching Devices

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00878H, Paper
Sanam Attique, Nasir Ali, Khatoon Rabia, Shahid Ali, Akmal Abbas, Yangchun Yu, Jiahui Hou, Bingqiang Cao, Huizhen Wu, Shikuan Yang
Organo-metal halide perovskites (OMHPs) have demonstrated promising applications in solar cells, light-emitting diodes, and photodetectors. However, besides the toxic lead, the intensive usage of organic solvents during their fabrication could...
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Manufacturing of Pure Cellulose Films by Recycling Ionic Liquids as Plasticizers

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00046A, Paper
Longhui Li, Yun Zhang, Yanling Sun, Shuang Sun, Guancheng Shen, Peng Zhao, Jingqiang Cui, Haiyu Qiao, Yunming Wang, Huamin Zhou
Cellulose limited in insolubility and non-melting properties is hard to be directly applied to the manufacture of pure cellulose films (PCFs). Although existing progress in eco-friendly fabrication methods including chemical...
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Catalytic production of 1, 4-Pentanediol from furfural in a fix-bed system under mild conditions

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00233J, Paper
QiaoYun Liu, Botao Qiao, Fei Liu, Leilei Zhang, Yang Su, Ai-Qin Wang, Tao Zhang
Furfural is one of the most important biomass-derived chemicals. Its large-scale availability calls for the exploration of new transformation routes for further valorization. Here we report on the direct, one-step...
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Solvent-free ageing reactions of rare earth element oxides: From geomimetic synthesis of new metal-organic materials towards a simple, environmentally friendly separation of scandium

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00454E, Paper
Igor Huskic, Mihails Arhangelskis, Tomislav Friščić
The development of cleaner methodologies for the separation and processing of rare earth elements, including scandium and yttrium, is of high importance to materials science and industry. Here, we explore...
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Co-production of flexible polyurethanes and renewable solvent from a microalgae oil waste stream

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00852D, Communication
Thien An Phung Haia, Nitin Neelakantan, Marissa Tessman, Suryendra Sherman, Graham Griffin, Robert S Pomeroy, Stephen Mayfield, Michael Burkart
Renewable polymers have become an important focus in next-generation materials, and algae biomass offers an environmentally low-impact feedstock that can serve multiple uses. This study aims to develop a scalable...
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Died: Darrin Patrick, Who Used His Fall and Restoration to Help Struggling Pastors

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Published On :: Fri, 08 May 2020 12:52:00 PDT

(UPDATED) The St. Louis pastor spoke up about the difficulties faced by leaders and critiqued “celebrity culture” in ministry.

Darrin Patrick, a megachurch pastor, author, and speaker, has died.

Patrick was a teaching pastor at Seacoast Church, a multi-site megachurch based in Mount Pleasant, South Carolina, and the founding pastor of the Journey Church in St. Louis, where he lived.

In a Friday evening update, Seacoast Church stated: “Darrin was target shooting with a friend at the time of his death. An official cause of death has not been released but it appears to be a self-inflicted gunshot wound. No foul play is suspected.”

Patrick’s unexpected death came as a shock to friends and colleagues. Robby Gallaty, pastor of Long Hollow Baptist, in Hendersonville, Tennessee, said that Patrick was scheduled to speak at his church next weekend.

“I just talked to him Tuesday and Wednesday,” said Gallaty. “This is the second close friend I have lost in a year.”

Gallaty first met Patrick in 2015 and had invited him to speak the following year at a men’s ministry event at Long Hollow. Just before the event, he said, Patrick called and said he was leaving the ministry.

At the time, Patrick had been a rising star among Reformed evangelical circles and was serving as vice-president of the Acts 29 church planting network. He was fired from Journey for what church elders called misconduct including “inappropriate meetings, conversations, and phone calls with two women” and an abuse of power.

Despite Patrick’s fall from ministry, the two stayed friends. Patrick admitted his faults and got counseling. He went through a restoration process that lasted 26 months, according to a 2019 blog interview posted at Christianity Today. He returned to the ministry as a preacher but not as a senior pastor of a church. ...

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Superstitions

By digital.lib.usf.edu
Published On :: Wed, 05 Feb 2014 09:50:24 -0400


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Voodoism or superstition

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Published On :: Wed, 05 Feb 2014 09:50:26 -0400


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Personal observations of emigration of workers

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Published On :: Wed, 05 Feb 2014 09:50:32 -0400


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Autobiography of a person who insisted on writing one

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Published On :: Wed, 05 Feb 2014 09:50:33 -0400


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Ybor City conversation

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Published On :: Wed, 05 Feb 2014 09:50:34 -0400


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Manual of instructions for teachers of the Florida W.P.A. Music Project

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Published On :: Thu, 20 Feb 2014 17:29:26 -0400


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