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Portable Photochemical Vapor Generation-Microwave Plasma Optical Emission Spectrometer

J. Anal. At. Spectrom., 2020, Accepted Manuscript
DOI: 10.1039/D0JA00104J, Technical Note
Yujia Deng, Wen Zeng, Xiaoming Jiang, Xiandeng Hou
A low power microwave plasma torch as an excitation source was combined with photochemical vapor generation (PVG) and a miniaturized charge-coupled device to construct a portable optical emission spectrometer. The...
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The matrix effect in TOF-SIMS analysis of two-element inorganic thin films

J. Anal. At. Spectrom., 2020, Advance Article
DOI: 10.1039/C9JA00428A, Paper
Agnieszka Priebe, Tianle Xie, Gerhard Bürki, Laszlo Pethö, Johann Michler
Investigation of the matrix effect in Zr-based two-element alloys under continuous bombardment of a Ga+ primary ion beam in a study of ionization probability towards exploring the potential and limitations of gas-assisted TOF-SIMS.
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Ultra-sensitive determination of antimony valence by solution cathode glow discharge optical emission spectrometry coupled with hydride generation

J. Anal. At. Spectrom., 2020, Advance Article
DOI: 10.1039/D0JA00009D, Paper
Mingyue Zhao, Xiaoxu Peng, Bingcheng Yang, Zheng Wang
An ultra-sensitive solution cathode glow discharge-optical emission spectrometry (SCGD-OES) method coupled with hydride generation (HG) for the determination of antimony valence is described.
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A total consumption (up to 75 μL min−1) infrared-heated sample introduction system for inductively coupled plasma optical emission spectrometry

J. Anal. At. Spectrom., 2020, Advance Article
DOI: 10.1039/D0JA00068J, Paper
Ahmed Al Hejami, Mirah J. Burgener, John Burgener, Diane Beauchemin
A compact infrared-heated sample introduction system provides similar analytical performance with higher robustness and faster washout than commercially available nebulization systems.
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High-resolution atomic structure of rubidium compounds in L X-ray spectral lines: a promising explores for chemical analysis

J. Anal. At. Spectrom., 2020, Accepted Manuscript
DOI: 10.1039/D0JA00063A, Paper
Harpreet Singh Kainth
The outcomes of X-ray fluorescence (XRF) analysis have been made an immense influence on the chemical profiles in various materials used for industrial and medical purposes. In the beginning of...
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Evidence for Photochemical Synthesis of Fluoromethane

J. Anal. At. Spectrom., 2020, Accepted Manuscript
DOI: 10.1039/D0JA00108B, Communication
Ralph E Sturgeon, Enea Pagliano
Photochemical generation of volatile fluoromethane in a dilute acetic acid medium is demonstrated. Radical halogen atom transfer (XAT) from an intermediate Cu-F transition metal fluorocomplex to abundant •CH3 generated by...
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Extractive separation of rare earth elements and their determination by inductively coupled plasma optical emission spectrometry in geological samples

J. Anal. At. Spectrom., 2020, Accepted Manuscript
DOI: 10.1039/D0JA00190B, Paper
Susanta Kumar Pradhan, Balram Ambade
A simple, rapid and effective solvent extraction separation of rare earth elements (REEs) has been developed for their determination in geological samples such as rock, soil and core samples by...
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What kind of balance should we strike between the Easter bunny and the empty grave?




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Social media should be a complement to real life. Not a substitute.

One effective way to correct unhealthy social-media habits is to fast for a few weeks and then come back with strict limits on use — for example, as in the University of Pennsylvania study, a few minutes per day on any individual platform. That puts social media where it rightfully belongs: under each user’s control, and as a complement to real life.

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Stop Doing These 7 Embarrassing Things on Social Media

When you think about embarrassing social media behavior, you probably think about octogenarians who accidentally post their phone numbers in a Facebook status. But embarrassing social media perils are everywhere for users of all ages, particularly for actors. But it is 2019 and social media is as important to your acting brand as your signature monologue or audition song, so we want to help you avoid these digital landmines and lead with your best online foot forward.

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Law Enforcement RSS Feeds from Police One

If you hate missing out on the latest news from PoliceOne, are having a hard time managing the deluge of information you receive from our newsletters, or simply want a more convenient way to manage and control your online news and information, RSS feeds may be the answer.

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The Rise and Demise of RSS

Before the internet was consolidated into centralized information silos, RSS imagined a better way to let users control their online personas.

About a decade ago, the average internet user might well have heard of RSS. Really Simple Syndication, or Rich Site Summary—what the acronym stands for depends on who you ask—is a standard that websites and podcasts can use to offer a feed of content to their users, one easily understood by lots of different computer programs. Today, though RSS continues to power many applications on the web, it has become, for most people, an obscure technology.

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What if Fake News Is Not the Real Problem on Social Media?

With another US Presidential election on the way in 2020, we can expect the debate around fake news to once again ramp up, and become a key focus of discussion as we look at how political influence spreads online.

What if Fake News Is Not the Real Problem on Social Media?




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Emerging Social Media Channels & Trends

Social media trends are like friends; they come and go.

However, the best friends and trends end up sticking around and evolving into permanent parts of our lives with qualities such as integrity, dependability, trust, quality and even ROI.

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Emerging Social Media Channels & Trends

Social media trends are like friends; they come and go.

However, the best friends and trends end up sticking around and evolving into permanent parts of our lives with qualities such as integrity, dependability, trust, quality and even ROI.

The bad friends and trendamies need to get weeded out before too much time, and resources get depleted.

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Mailbrew launches to create auto email newsletters from Reddit, Twitter, YouTube, RSS feeds

A new service called Mailbrew is live that lets you created automated email newsletters. You can set them up from multiple sources including Twitter, Reddit, YouTube, RSS feeds, and more.

Mailbrew aims to save you time by rounding up the news and updates you care about from a variety of sources and popping it in a daily, weekly, or monthly automated email newsletter.

To start, you can create custom brews, choose from pre-made ones, or make use of both. You even get to choose the layout you’d like to use for the newsletters.

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Stop Travel Memories From Appearing in Your Social Media Feeds

Our stress levels are at an all-time high right now, which means our attentiveness to our own self-care should be, too—especially those of us with wanderlust. Traveling from the living room to the kitchen and back is no one’s ideal of a vacation, yet here we are. On top of that, our social media platforms seem determined to remind us of better days: Hey, look where you were a year ago today! blares Facebook, serving up a photo of a gorgeous beach or other getaway spot much more alluring than the permanent butt-groove you have formed in your couch.

For many of us, looking back on our travels past is not doing us much good at the moment. Luckily, there are a few methods to keep them from showing up in your social media feeds.




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Social media use spikes during pandemic

While usage of most mobile apps has remained neutral during the coronavirus pandemic, social media app usage has exploded during the lockdown, according to new data from Nielsen.

Why it matters: Prior to the pandemic, consumers and tech companies were both becoming more aware of the overuse of social media and actively trying to limit it. In a time when people can not connect with friends and family in person, companies have put these efforts on pause.

By the numbers: Prior to the pandemic, social media usage for most of January, February and early March remained relatively flat at around 20% of total mobile app usage, according to Nielsens data.

But beginning in mid-March, when statewide stay-at-home orders went into effect, social media app usage began to increase significantly, and now consumes around 25% of all mobile app usage for U.S. adults.

Other media app usage, like video, lifestyle, and finance apps have mostly remained the same, in part because consumers are now leveraging other devices, like desktops and television screens, for more activities while home.




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Private mobile phones restored in Kashmir; situation remains calm




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'Inhuman' comments about Amit Shah's health 'extremely condemnable': JP Nadda




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Fred Smoot thinks Arizona's Isaiah Simmons reminds him of Sean Taylor

Fred Smoot compared the Cardinals' defender to his former teammate Sean Taylor.




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Patriots sign 4 additional members of draft class

FOXBOROUGH, Mass. (AP) -- The New England Patriots have signed four additional members of their 2020 draft class.




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Thoughts of opening SoFi Stadium minus fans brings an empty feeling

When the Rams debut in SoFi Stadium, will the 70,240-seat stadium be filled with fans, empty or somewhere in between? Ticket holders are anxious to know.




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An analytical method to characterize the crystal structure of layered double hydroxides: synthesis, characterization, and electrochemical studies of zinc-based LDH nanoplates

J. Mater. Chem. A, 2020, 8,8692-8699
DOI: 10.1039/D0TA01774D, Paper
Jiyong Chung, Jaeyoung Lee, Jae Kyeom Kim, Minseong Kim, Kug-Seung Lee, Seung-Joo Kim, Min Hyung Lee, Taekyung Yu
Due to their unique soft and complex structure, it has been difficult to analyze the exact crystal structure of layered double hydroxides (LDHs), which has been a major obstacle to understanding and improving the catalytic properties of LDHs.
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Engineering yolk–shell P-doped NiS2/C spheres via a MOF-template for high-performance sodium-ion batteries

J. Mater. Chem. A, 2020, 8,8612-8619
DOI: 10.1039/D0TA02568B, Paper
Liqin Wang, Zhanli Han, Quanqing Zhao, Xiuyun Yao, Youqi Zhu, Xilan Ma, Shide Wu, Chuanbao Cao
The stable yolk–shell P-doped NiS2/C spheres were successfully fabricated via MOFs template, and first adopted phytic acid as P source. Due to the unique framework and synergistic effect, P-doped NiS2/C sample displayed high sodium storage capacity.
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Enhancing the average thermoelectric figure of merit of elemental Te by suppressing grain boundary scattering

J. Mater. Chem. A, 2020, 8,8455-8461
DOI: 10.1039/D0TA02660C, Paper
Yehao Wu, Feng Liu, Qi Zhang, Tiejun Zhu, Kaiyang Xia, Xinbing Zhao
Suppressed grain boundary scattering contributes to enhanced electrical conductivity and device zT in elemental Te based thermoelectric materials.
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The favourable thermodynamic properties of Fe-doped CaMnO3 for thermochemical heat storage

J. Mater. Chem. A, 2020, 8,8503-8517
DOI: 10.1039/D0TA02031A, Paper
Open Access
Emanuela Mastronardo, Xin Qian, Juan M. Coronado, Sossina M. Haile
The CaFe0.1Mn0.9O3−δ0 oxide can reversibly release oxygen over a relatively wide range of temperatures and oxygen partial pressures and its favourable thermodynamic properties make it a promising candidate for thermochemical heat storage.
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Robust FeOOH/BiVO4/Cu(In, Ga)Se2 tandem structure for solar-powered biocatalytic CO2 reduction

J. Mater. Chem. A, 2020, 8,8496-8502
DOI: 10.1039/D0TA02069A, Paper
Jinhyun Kim, Yang Woo Lee, Eun-Gyu Choi, Passarut Boonmongkolras, Byoung Wook Jeon, Hojin Lee, Seung Tae Kim, Su Keun Kuk, Yong Hwan Kim, Byungha Shin, Chan Beum Park
A robust, scalable FeOOH/BiVO4/Cu(In,Ga)Se2 tandem structure achieves unbiased, long-term photobiocatalytic conversion of CO2 to formate.
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PCE11-based polymer solar cells with high efficiency over 13% achieved by room-temperature processing

J. Mater. Chem. A, 2020, 8,8661-8668
DOI: 10.1039/D0TA02271C, Paper
Jianyun Zhang, Wenrui Liu, Ming Zhang, Shengjie Xu, Feng Liu, Xiaozhang Zhu
Non-fullerene acceptors featuring excellent miscibility with temperature-dependent aggregation polymer PCE11 enable room-temperature processed polymer solar cells with high efficiency over 13%.
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The critical effect of water content in the electrolyte on the reversible electrochemical performance of Zn–VPO4F cells

J. Mater. Chem. A, 2020, 8,8262-8267
DOI: 10.1039/D0TA01622E, Communication
Hooman Yaghoobnejad Asl, Shyam Sharma, Arumugam Manthiram
The critical role of water as a source of H+ working ions and reactive species in the Zn–VPO4F electrochemical system with an ionic liquid electrolyte.
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Understanding the mechanism of byproduct formation with in operando synchrotron techniques and its effects on the electrochemical performance of VO2(B) nanoflakes in aqueous rechargeable zinc batteries

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA00858C, Paper
Qiang Pang, Hainan Zhao, Ruqian Lian, Qiang Fu, Yingjin Wei, Angelina Sarapulova, Junqi Sun, Chunzhong Wang, Gang Chen, Helmut Ehrenberg
The byproduct protects the vanadium-based positive electrode of ARZBs and facilitates Zn2+ insertion into the electrode.
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Decoupled electrolytes towards enhanced energy and high temperature performance of thermally regenerative ammonia batteries

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03236K, Paper
Weiguang Wang, Gequn Shu, Xiuping Zhu, Hua Tian
An electrolyte decoupling strategy is proposed for ammonia batteries to restrain the self-discharge and enhance energy density as well as power generation at high temperatures.
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A highly efficient artificial light-harvesting system with two-step sequential energy transfer based on supramolecular self-assembly

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03169K, Paper
Guangping Sun, Weirui Qian, Jianmin Jiao, Tingting Han, Yukun Shi, Xiao-Yu Hu, Leyong Wang
An efficient artificial light-harvesting system with two-step sequential energy transfer has been successfully constructed based on supramolecular self-assembly.
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Inexpensive thermochemical energy storage utilising additive enhanced limestone

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03080E, Paper
Kasper T. Møller, Ainee Ibrahim, Craig E. Buckley, Mark Paskevicius
A thermochemical energy storage capacity retention of up to 90% over 500 cycles is achieved in cheap and abundant limestone.
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Synchronous surface and bulk composition management for red-shifted light absorption and suppressed interfacial recombination in perovskite solar cells

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02449J, Paper
Jun-Xing Zhong, Jin-Feng Liao, Yong Jiang, Lianzhou Wang, Dai-Bin Kuang, Wu-Qiang Wu
Perovskite solar cells with a reverse vertical gradient distribution of α/δ-FAPbI3 achieved a record efficiency of up to 21.9% owing to synergistic advantages of expanded photon harvesting and robust surface defect passivation.
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The rational and effective design of nonfullerene acceptors guided by a semi-empirical model for an organic solar cell with an efficiency over 15%

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03087B, Paper
Xin Ke, Lingxian Meng, Xiangjian Wan, Mingpeng Li, Yanna Sun, Ziqi Guo, Simin Wu, Hongtao Zhang, Chenxi Li, Yongsheng Chen
Guided by a semi-empirical model, two small-molecule acceptors were rationally designed and an impressive PCE of 15.05% was achieved.
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Semiconducting polymer contributes favorably to the Seebeck coefficient in multi-component, high-performance n-type thermoelectric nanocomposites

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA02388D, Paper
Junhui Tang, Ruisi Chen, Lidong Chen, Guillermo C. Bazan, Ziqi Liang
n-Type Co NWs/N2200 TENCs yield a high S, mainly from the semiconducting polymer, yet σ is limited by poor connectivity between inorganic and organic domains. By adding flexible n-doped SWCNTs to yield more conductive paths, σ and mechanical bendability are greatly enhanced.
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Graphene oxide laminates intercalated with 2D covalent-organic frameworks as a robust nanofiltration membrane

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA01727B, Paper
Xiao Sui, Ziwen Yuan, Chang Liu, Li Wei, Meiying Xu, Fei Liu, Alejandro Montoya, Kunli Goh, Yuan Chen
Porous yet rigid 2D covalent–organic framework nanosheets can not only increase the interlayer spacing between graphene oxide nanosheets and provide direct transfer channels but also enhance the self-supporting capacity of graphene oxide laminates.
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Perovskite-Sensitized β-Ga2O3 Nanorod Arrays for Highly Selective and Sensitive NO2 Detection at High Temperature

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02691C, Paper
Bo Zhang, Hui-Jan Lin, Haiyong Gao, Xingxu Lu, Chang-Yong Nam, Pu-Xian Gao
Amongst various gaseous pollutants, NO2 is one of the major exhausts originating from fossil fuel and gas combustions in vehicle engines and power plants at high temperature. Under such scenario,...
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Smart Porous Wood Supported Flower-like NiS/Ni Conjuction with Vitrimer Co-effect as Multifunctional Material with Reshaping, Shape-memory and Self-healing for High-Performance Supercapacitors, Catalysts and Sensors

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03664A, Paper
Chuanyin Xiong, Bingbing Li, Heguang Liu, Wei Zhao, Chao Duan, Haiwei Wu, Yong Ni
Wood-based materials are attracting more and more attention for applications in energy storage, due to their environment friendly and numerous channels structure. However, the poor conductivity and flexibility of wood...
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A novel integrated Cr(VI) adsorption–photoreduction system using MOF@polymer composite beads

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA01046D, Paper
Bardiya Valizadeh, Tu N. Nguyen, Stavroula Kampouri, Daniel T. Sun, Mounir D. Mensi, Kyriakos Stylianou, Berend Smit, Wendy L. Queen
Herein, a novel integrated adsorption–photoreduction system, which captures highly mobile and toxic hexavalent chromium (Cr(VI)) from real-world water samples and reduces it to less mobile and benign Cr(III) species, was designed.
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Flexible and transparent sensors for ultra-low NO2 detection at room temperature under visible lights

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02934C, Paper
Xiao-Xue Wang, Hua-Yao Li, Xin Guo
Metal oxide based gas sensors should mostly work at high temperatures; the high working temperature possesses safety concerns and high energy consumption, which makes portable and wearable devices almost impossible,...
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Polyimide/ZIF-7 Mixed-Matrix Membranes: Understanding in-situ Confined Formation of ZIF-7 Phases inside Polymer and Their Effects on Gas Separations

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02761H, Paper
Sunghwan Park, Kie Yong Cho, Hae-Kwon Jeong
Polymer-modification-enabled in-situ metal-organic framework formation (PMMOF) is potentially a paradigm-shifting preparation method for polymer/MOF mixed-matrix membranes (MMMs). However, the actual reaction conditions of in-situ formation of MOF in the confined...
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Ferrites: emerging light absorbers for solar water splitting

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA01554G, Review Article
Jeong Hun Kim, Hyo Eun Kim, Jin Hyun Kim, Jae Sung Lee
Ferrites are promising photoelectrode materials for solar water splitting to produce clean and storable hydrogen energy.
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Highly efficient removal of uranium from highly acidic media achieved on a phosphine oxide and amino functionalized superparamagnetic composite polymer adsorbent

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA01633K, Paper
Shiao Zhang, Dingzhong Yuan, Qinghua Zhang, Yun Wang, Yan Liu, Jizhou Zhao, Bibo Chen
It is very necessary to develop the magnetic adsorbents for the efficient extraction of uranium from highly acidic media. In this work, a novel magnetic adsorbent Fe3O4/P (DMAA-DMP) functionalized with...
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In Situ Confinement of Pt within Three-Dimensional MoO2@Porous Carbon for Efficient Hydrogen Evolution

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02507K, Paper
Yimin Jiang, Miao Yang, Meijiao Qu, Yi Wang, Zhouchunyu Yang, Qingliang Feng, Xia Deng, Wei Shen, Ming Li, Rongxing He
Promoting the industrialization and widespread application of Pt-based catalysts is essential to electrochemical water-splitting systems. However, the development of cost-effective Pt-based catalysts still remains a high challenge. Here we report...
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Ultrahigh Photothermal Temperature in Graphene/Conducting Polymer System Enables Contact Thermochemical Reaction

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03347B, Paper
Yuqiao Chai, Hui Ma, Xinlei Ma, Xinyue Zhang, Yonglin He, Yapei Wang, Qianqian Jiang, Xusheng Wang, Junhui Ji, Mianqi Xue
Photothermal conversion in near-infrared (NIR) wavelengths, which converts light energy into heat energy, has caused great concern and been developing rapidly in recent years for its wide applications in health...
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Surface-Functionalized Palladium Catalysts for Electrochemical CO2 Reduction

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA03427D, Paper
Rong Xia, Sheng Zhang, Xinbin Ma, Feng Jiao
Rational design and synthesis of efficient catalysts for electrochemical CO2 reduction is a critical step towards practical CO2 electrolyzer systems. In this work, we report a strategy to tune the...
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Hydrophilic ultrafiltration membranes with surface-bound eosin Y for an integrated synthesis-separation system of aqueous RAFT photopolymerization

J. Mater. Chem. A, 2020, Advance Article
DOI: 10.1039/D0TA03112G, Paper
Yujie Zhao, Senlin Shao, Jiangbin Xia, Ya Huang, Yu Chi Zhang, Xue Li, Tao Cai
The photocatalyst-based ultrafiltration membrane fitted integrated synthesis–separation system holds the promises to bridge the gap between the precision of PET-RAFT polymerization and the efficiency of membrane separation process.
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Catalyst design strategies for stable electrochemical CO2 reduction reaction

J. Mater. Chem. A, 2020, Accepted Manuscript
DOI: 10.1039/D0TA02633F, Review Article
Woong Choi, Da Hye Won, Yun Jeong Hwang
The gradual increase in the atmospheric CO2 concentration due to the combustion of fossil fuels is an urgent issue that poses a threat to human beings. Recently, the electrochemical CO2...
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