Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00642A, Paper

Julian Wailliez, Paul Regazzi, Anniina Salonen, Paul G. Chen, Marc Jaeger, Marc Leonetti, Emmanuelle Rio
We measure the deformation of a drop under an extensional flow. The drop is less deformed than for a pure liquid because of the depletion of surfactants at the tips, which we attribute to the adsorption/desorption dynamics of the surfactants.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01035C, Paper

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James S. Sharp, Nathaniel M. Roberts, Sam Walker
Telephone cord blister formation is studied in PDMS films swollen in four different solvents. Buckling and fracture mechanics theories are developed to interpret blister morphology and growth rates. A simple surface patterning method is introduced.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00969J, Paper

Nabila Ali, Connor J. Demott, Olivia F. Dingus, Melissa A. Grunlan, Alison C. Dunn
Tough hydrogels with a charge-variable third network were assessed for biomimicking lubricity in both water and FBS solution.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01006J, Paper

Nathan Bigan, Mathieu Lizée, Marc Pascual, Antoine Niguès, Lydéric Bocquet, Alessandro Siria
In confinement, liquid flows are governed by a complex interplay of molecular, viscous and elastic forces.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00860J, Paper

Mayssa Medfai, Antonio Stocco, Christophe Blanc, Maurizio Nobili, Martin In
The interface of semidilute Gemini surfactant solutions remains fluid and is less viscous than the bulk. Depletion of the viscosity near the interface plays a key role in microrheology.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00670D, Paper

Piyaporn Srisura, Yuwaporn Pinyakit, Umphan Ngoensawat, Pongsakorn Yuntasiri, Khoiria Nur Atika Putri, Theerapat Chanamuangkon, Waranyoo Phoolcharoen, Varol Intasanta, Voravee P. Hoven
Carboxymethyl cellulose-stabilized calcium phosphate particles well-dispersed in aqueous solution can be integrated into an injectable hydrogel made of methacrylated hyaluronic acid which is a promising material for bone regeneration applications.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01040J, Paper

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Lorenzo Miele, Antonio Abate, Kentaro Taki, Ernesto Di Maio
The inverse pressure quenching treatment is proposed to decouple bubble nucleation from growth, advancing our understanding of the physics governing bubble growth and evolution in polymer foaming.
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Soft Matter, 2024, 20,8353-8362
DOI: 10.1039/D4SM00908H, Paper

Moumita Dasgupta, Sougata Guha, Leon Armbruster, Dibyendu Das, Mithun K. Mitra
The nature of barriers control the first passage times in heterogenous media. For entropic barriers, the first passage times increases monotonically with increasing number of barriers, while for energetic barriers, passage times show a non-monotonic behaviour with increasing barriers.
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Soft Matter, 2024, 20,8363-8372
DOI: 10.1039/D4SM00577E, Paper

Xiangshen Meng, Xiaowei Li, Jian Li, Yueqiang Lin, Xiaodong Liu, Zhenghong He
The dynamic rotational behavior of composite chains under a rotating magnetic field was observed. The birefringence and dichroism variations in FNLCs mainly stem from the magnetic response of the composite chains, indicating local effects.
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Soft Matter, 2024, 20,8373-8384
DOI: 10.1039/D4SM00828F, Paper

Open Access

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Larissa J. Lubitz, Harden Rieger, Gero Leneweit
An optimized PFC/W emulsion contains 1 mM lipid per 1% (v/v) dispersed phase for an emulsifying monolayer; higher ratios result in triple layers. Low viscosity ratios η_D/η_C ≤ 5 and low PFC volume fractions lead to smaller monodisperse droplets.
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Soft Matter, 2024, 20,8337-8352
DOI: 10.1039/D4SM00445K, Paper

Open Access

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Hossein Nemati, J. de Graaf
Extending the cellular Potts model to disordered Voronoi lattices reduces artifacts observed on regular lattices. An order–disorder transition is observed as a function of surface tension on the disordered lattice and the regular lattices.
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Soft Matter, 2024, 20,8407-8419
DOI: 10.1039/D4SM00800F, Paper

Hexiang Wang, Zhimeng Jia, Yuqiang Fang
We establish a multiscale model of a cell to explore the chemomechanical mechanisms of cell polarization initiated by structural polarity. The two-dimensional vertex model is built by coupling the cytoskeletal reorganization and the Cdc42 activation.
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Soft Matter, 2024, 20,8420-8435
DOI: 10.1039/D4SM00919C, Paper

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Friedrich Walzel, Jonathan Dijoux, Leandro Jacomine, Élodie Harle, Pierre Muller, Thierry Charitat, Wiebke Drenckhan
Combining experiments, simulations and theory, we provide a complete shape analysis of two bubbles held by circular frames in the parameter space of different frame radii, distances between frames and contact angle between bubbles (0°, 60° and 90°).
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Soft Matter, 2024, 20,8395-8406
DOI: 10.1039/D4SM00634H, Paper

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Luke Neville, Jens Eggers, Tanniemola B. Liverpool
The interaction between a disk and wall in an active nematic depends on a combination of activity and anchoring, with contractile nematics repelling disks with planar anchoring.
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Soft Matter, 2024, 20,8436-8445
DOI: 10.1039/D4SM01058B, Paper

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Andrei Filippov, Maiia Rudakova, Victor P. Archipov, Faiz Ullah Shah
Diffusivity is controlled by exchange of ions between “narrow” and “large” pores that results in an abnormal temperature variation. Li⁺ ions are solvated inside the porous glasses and their diffusivity remains slower as compared to the organic ions.
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Soft Matter, 2024, 20,8480-8492
DOI: 10.1039/D4SM00875H, Paper

Weikang Xian, Amitesh Maiti, Andrew P. Saab, Ying Li
Polydimethylsiloxane and its copolymer systems have a wide range of application. We systematically develop a coarse-grained MD model for PDMS-co-PDPS system. The model preserves the structural and dynamic properties of the material quantitatively.
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Soft Matter, 2024, 20,8455-8467
DOI: 10.1039/D4SM00867G, Paper

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Jens Weimar, Frank Hirschmann, Martin Oettel
Critical points of an anisotropic, coarse-grained protein model are used to detemine an “effective patchiness” by comparison to the Kern–Frenkel patchy model.
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Soft Matter, 2024, 20,8446-8454
DOI: 10.1039/D4SM00992D, Paper

Troy Singletary, Nima Iranmanesh, Carlos E. Colosqui
This work proposes an analytical model considering the effects of hydrodynamic drag and energy barriers induced by liquid solvation forces to predict the in-plane translational diffusivity of a nanoparticle physically adsorbed on a wetted surface.
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Soft Matter, 2024, 20,8505-8514
DOI: 10.1039/D4SM00994K, Paper

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Conner H. Chee, Rotem Benharush, Lexi R. Knight, Jennifer E. Laaser
Complexes of strong polyelectrolytes prepared well above the binodal are shown to undergo hydrophobicity-driven segregative phase separation.
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Soft Matter, 2024, 20,8385-8394
DOI: 10.1039/D4SM00616J, Paper

D. A. Mitkovskiy, A. A. Lazutin, A. L. Talis, V. V. Vasilevskaya
Amphiphilic macromolecules grafted onto spherical nanoparticles can self-assemble into morphological structures corresponding to the family of complete embedded minimal surfaces. They arise situationally, can coexist and transform into each other.
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Soft Matter, 2024, 20,8515-8523
DOI: 10.1039/D4SM00704B, Paper

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Christine Linne, Eva Heemskerk, Jos W. Zwanikken, Daniela J. Kraft, Liedewij Laan
Our study shows that DNA nanostars with three binding sites (ligands) can (1) bind superselectively to surfaces based on receptor density, and (2) that interactions between ligands affect the optimum number of ligands required for superselectivity.
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Soft Matter, 2024, 20,8493-8504
DOI: 10.1039/D4SM00721B, Paper

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Stephen Kronenberger, Nitant Gupta, Benjamin Gould, Colin Peterson, Arthi Jayaraman
We present a computational method to analyze 2D small-angle scattering data from three-phase soft materials systems with structural anisotropy and output representative real-space structures of the three phases.
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Soft Matter, 2024, 20,8468-8479
DOI: 10.1039/D4SM00625A, Paper

Blake Langeslay, Gabriel Juarez
A model of cell alignment in confined growing bacterial monolayers connecting net monolayer deformation to the behavior of individual cells.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00952E, Paper

Ifunanya Nwogbaga, Brian A. Camley
We study the physical factors that control the accuracy with which elongated cells can sense the direction of an electric field, exploring whether cells are more accurate sensors when oriented parallel to the field or perpendicular to it.
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Soft Matter, 2024, 20,8524-8537
DOI: 10.1039/D4SM00706A, Paper

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Arash Yahyazadeh Shourabi, Roland Kieffer, Djanick de Jong, Daniel Tam, Marie-Eve Aubin-Tam
Lipid membranes formed in a microfluidic device are studied with temperature-controlled optical tweezers, revealing how mechanical properties of ripple phase and gel-fluid phase-separated membranes change when heated above the transition temperature.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01004C, Paper

Keke Yang, Hou Bo, Dewei Ma, Mingwei Peng, Qinglong Liu, Ziwen Heng, Zhongwei Gu, Xuhan Liu, Siyuan Chen
Phenylboronic acid (PBA) is a widely exploited glucose-sensitive element for constructing glucose-responsive hydrogels to enable smart insulin delivery.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00761A, Paper

Setarehalsadat Changizrezaei, Mikko Karttunen, Colin Denniston
A polymer confined in a nanochannel undergoes a crossover to a jammed state when pushed by a large spherical colloid. We examine the system using simulations that incorporate the full hydrodynamic driving and fluctuating forces.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM90171A, Retraction

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Naohiro Kameta, Masumi Asakawa, Mitsutoshi Masuda, Toshimi Shimizu
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM90172J, Retraction

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Naohiro Kameta, Hiroyuki Minamikawa, Mitsutoshi Masuda
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00486H, Paper

Open Access

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Max Huisman, Axel Huerre, Saikat Saha, John C. Crocker, Valeria Garbin
Machine learning predicts possible crack location in experiments of a fracturing colloid monolayer, shown along with the actual crack path.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00999A, Paper

Open Access

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Martin Wittmann, Igor M. Kulić, Antonio Stocco, Juliane Simmchen
We use experiments and theoretical models to investigate the rolling and translational motion of rod-shaped micro particles close to a solid wall in the presence or absence of shear flow.
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00528G, Paper

Nicolas Herard, Raja Annapooranan, Todd Henry, Martin Kroger, Shengqiang Cai, Nicholas Boechler, Yelena Sliozberg
This paper presents a coarse-grained molecular dynamics simulation study of the synthesis, mechanics, and thermal actuation of nematic phase main-chain liquid crystal elastomers (LCEs), a type of soft, temperature-responsive, polymeric...
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01123F, Paper

Open Access

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Daniel Weidig, Joachim Wagner
Self- and collective dynamics in mixtures of highly charged binary colloidal particles is analyzed by Brownian dynamics simulations. For equally charged, but differently sized particles coupling effects in their long-time dynamics are observed.
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00827H, Paper

Nastassia Pricoupenko, Flavia Marsigliesi, Philippe Marcq, Carles Blanch-Mercader, Isabelle A Bonnet
Collective cell migration is key during development, wound healing and metastasis and relies on coordinated cell behaviors at the group level. Src kinase is a key signalling protein for physiological...
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00989D, Paper

Yan Wen, Jiayu Liu, Wei Wang, Pik-Yin Lai, Penger Tong
We report a systematic study of barrier-crossing dynamics of bottom-heavy self-propelled particles (SPPs) over a one-dimensional periodic potential landscape $U_0(x)$, which is fabricated on a microgroove-patterned polydimethylsiloxane (PDMS) substrate. From...
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00886C, Paper

Open Access

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Ji Zhang, Jeremy J. Baumberg, Sohini Kar-Narayan
Trilayer electrochemical actuators comprising an electrolyte layer sandwiched between two electrode layers have been shown to exhibit large deformations at low actuation voltages. Here we report aerosol-jet printing (AJP) of...
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00879K, Paper

Man Xu, Ying Lan, Yuehua Yang, Hongyuan Jiang
We present the dynamics of particles in a device divided into two chambers by V-shaped barriers and connected by a narrow channel. Here three distinct movement modes occur, including stochastic movement, oscillation and unidirectional flows.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01065E, Paper

Karthik R. Peddireddy, Ryan McGorty, Rae M. Robertson-Anderson
We leverage in situ enzymatic topological conversion and OpTiDDM to map the deformation dynamics of DNA blends with over 70 fractions of linear, ring and supercoiled molecules that span the phase space of possible topological compositions.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00988F, Paper

Julie Pinchiaroli, Renita Saldanha, Alison E. Patteson, Rae M. Robertson-Anderson, Bekele J. Gurmessa
The unique mechanical behaviors of actin–vimentin composites in both linear and nonlinear regimes are shaped by the complex interactions among actin entanglements, vimentin crosslinking, and poroelastic properties.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00534A, Paper

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Homa Ghaiedi, Luis Carlos Pinzon Herrera, Saja Alshafeay, Leonard Harris, Jorge Almodovar, Karthik Nayani
Collagen is a key component of the extracellular matrix (ECM) and well-oriented domains of collagen are important for mimicking the local cell environment in vitro. Here, we demonstrate macroscopic alignment on collagen in 2-D substrates and 3-D hydrogels.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00931B, Paper

Muchu Zhou, Reza Foudazi
Foam fractionation offers a promising solution for the separation of surface-active contaminants from water.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM00987H, Paper

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Sunilkumar Khandavalli, Jae Hyung Park, Robin Rice, Diana Y. Zhang, Sarah A. Berlinger, Guido Bender, Deborah J. Myers, Michael Ulsh, Scott A. Mauger
Steady-shear rheology showing evolution of the microstructure of iridium oxide catalyst inks of PEM water electrolyzers with aging time.
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Soft Matter, 2024, Advance Article
DOI: 10.1039/D4SM01076K, Paper

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Yihao Chen, Mina Mandić, Charlotte G. Slaughter, Michio Tanaka, James M. Kikkawa, Peter J. Collings, A. G. Yodh
This work characterizes twist disclinations in nematic liquid crystals, using confocal microscopy to measure their 3D profile and test theoretical predictions, and using magnetic fields to deform the disclinations and measure their line tension.
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Soft Matter, 2024, Accepted Manuscript
DOI: 10.1039/D4SM00651H, Paper

Ignasi Vélez Cerón, Jordi Ignes-Mullol, Francesc Sagues
A photoresponsive variant of the paradigmatic active nematic fluid made of microtubules and powered by kinesin motors is studied in the conventional two-dimensional interfaced form when forced under blue-light illumination....
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Soft Matter, 2024, 20,8561-8569
DOI: 10.1039/D4SM00322E, Paper

Rafał Węgłowski, Anna Spadło, Dorota Węgłowska
In this study, DNA extracted from bananas was functionalized and used as a homeotropic alignment layer for liquid crystals.
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Soft Matter, 2024, 20,8638-8653
DOI: 10.1039/D4SM00350K, Paper

Subhajit Paul, Abhishek Dhar, Debasish Chaudhuri
We explore the dynamics of a tracer in a harmonic chain of active particles, investigating the influence of interactions. Depending upon the time-scales governed by the interaction and the persistence of activity, we explore crossovers between different scaling behaviors of its dynamics.
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Soft Matter, 2024, 20,8663-8674
DOI: 10.1039/D4SM00578C, Paper

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L. V. Tiihonen, M. P. Weir, A. J. Parnell, S. C. Boothroyd, D. W. Johnson, R. M. Dalgliesh, M. Bleuel, C. P. Duif, W. G. Bouwman, R. L. Thompson, K. S. Coleman, N. Clarke, W. A. Hamilton, A. L. Washington, S. R. Parnell
Spin-echo small-angle neutron scattering (SESANS) revealed structure in polymer–carbon nanocomposites over multiple length scales with unprecedented range (10 nm–16 μm). Data from two SESANS instruments and other methods were analysed with SasView.
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Soft Matter, 2024, 20,8581-8588
DOI: 10.1039/D4SM00902A, Paper

Titus Quah, Kevin J. Modica, James B. Rawlings, Sho C. Takatori
Model predictive control is used to guide the spatiotemporal distribution of active Brownian particles by forecasting future states and optimizing control inputs to achieve tasks like dividing a population into two groups.
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Soft Matter, 2024, 20,8570-8580
DOI: 10.1039/D4SM00868E, Paper

Davi Lazzari, Olivier Dauchot, Carolina Brito
Active solids, more specifically elastic lattices embedded with polar active units, exhibit collective actuation when the elasto-active feedback, generically present in such systems, exceeds some critical value.
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Soft Matter, 2024, 20,8621-8637
DOI: 10.1039/D4SM00993B, Paper

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Simona Migliozzi, Yiting He, Maryam Parhizkar, Yang Lan, Panagiota Angeli
Elucidating the impact of microgels attributes on the microstructure, rheology and functionality of Pickering emulsions.
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