CrystEngComm, 2024, Advance Article
DOI: 10.1039/D4CE00221K, Communication

Open Access

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Sumea Klokic, Benedetta Marmiroli, Denys Naumenko, Giovanni Birarda, Simone Dal Zilio, Miriam de J. Velásquez-Hernández, Paolo Falcaro, Lisa Vaccari, Heinz Amenitsch
Controlling the magnitude of structural dynamics in flexible MOF films by an applied stimulus is largely desired for specific applications such as energy storage.
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Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00336E, Paper

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Bintu Kumar, Anindita Bhatta, Prakriti Saraf, Taur Prakash Pandurang, Krishnan Rangan, Madhushree Sarkar, Sivaprasad Mitra, Dalip Kumar
Using readily available BODIPY and iodoarenes various BODIPY(aryl)iodonium salts were prepared and successfully utilized for the direct syntheses of functionalized BODIPYs, bis-BODIPYs and for the selective detection of serum protein.
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Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00112E, Paper

Debojyoti Bag, Sanghapal D. Sawant
Herein, we describe a highly diastereoselective approach for synthesizing polyfunctionalized spiroindolines from indolyl-ynones involving an ipso-iodocyclization/nucleophile addition cascade.
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Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00229F, Paper

Kalleshappa Sheela, Chikkappaiahnayaka Santhosh, Krishna Ravi Singh, Kalleshappa Sharath, Maralinganadoddi P. Sadashiva
Herein, we report an efficient strategy to synthesize functionalized 1,3-thiazoles using alkyl 2-amino-2-thioxoacetates.
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Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00292J, Paper

Jinkai Hu, Chenglei Yang, Xiaotao Qin, Hui Liu, Tongtong Ma, Ao-tong Shi, Qing-Long Lv, Xingman Liu, Jinhui Yang, Dianjun Li
A visible light-enabled photocatalyst-free radical trihalomethylation/cyano (or benzo[d]thiazol-2-yl) 1,4-migration/carbonylation reaction of 2-hydroxy-2-hex-5-enenitrile (or (benzo[d]thiazol-2-yl)-pent-4-enol) with CX₃SO₂Cl (X = F, Cl) is reported.
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Org. Biomol. Chem., 2024, 22,2958-2962
DOI: 10.1039/D4OB00104D, Communication

Ying Sun, Shaomin Fu, Bo Liu
The asymmetric synthesis of the fully functionalized six-membered A-ring of siphonol A is presented.
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Org. Biomol. Chem., 2024, 22,3059-3067
DOI: 10.1039/D3OB02050A, Paper

Marie M. Le Roy, Sandra Claes, Nathalie Saffon-Merceron, Dominique Schols, Thibault Troadec, Raphaël Tripier
A rare example of C,C'-linked bis-cyclam has been synthesized with controlled manner in mild conditions thanks to the “bis-aminal” tool, and its good CXCR4-recognition properties could be demonstated in vitro.
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Org. Biomol. Chem., 2024, 22,3073-3079
DOI: 10.1039/D4OB00133H, Paper

Wei Chen, Lang-Qi Wen, Xiao-Bing Lu, Hui Zhou
We have developed a clean and efficient iron-catalyzed C(sp³)–H functionalization of indolin-2-ones for the chemodivergent synthesis of value-added indole derivatives, including isatins, and symmetrical and non-symmetrical isoindigos.
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Org. Biomol. Chem., 2024, Advance Article
DOI: 10.1039/D4OB00421C, Communication

Srinivasarao Yaragorla, Tabassum Khan, Sayonika Chakroborty
We report here a simple and atom economic cycloisomerization reaction of indole-tethered alkynols for constructing diverse carbazoles via 1,2-alkly migration using Cu(OTf)₂/HFIP as the excellent promoter system.
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Org. Biomol. Chem., 2024, Accepted Manuscript
DOI: 10.1039/D4OB00243A, Paper

György Keglevich, Petra Regina Varga, Emőke Dinnyési, Zsuzsanna Szalai, Szilvia Bősze, Rita Oláhné Szabó, Laszlo Drahos, Konstantin Karaghiosoff
Beta-Aminophosponates obtained by the Michael addition of primary amines to the double bond of diethyl vinylphosphonate proved to be suitable starting materials (amine components) in the Kabachnik–Fields reaction with formaldehyde...
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Mater. Chem. Front., 2024, 8,3653-3663
DOI: 10.1039/D4QM00438H, Research Article

Yu Jiang, Yuqing Li, Qunting Qu, Linze Lv, Jie Shao, Jing Wang, Honghe Zheng
A green, energy-saving and effective method for recycling graphite from spent Li-ion batteries and its reutilization in high-voltage dual-ion batteries are developed.
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Mater. Chem. Front., 2024, 8,3770-3789
DOI: 10.1039/D4QM00562G, Research Article

Yingjie He, Jiahe Guo, Hua Li, Jiaxi Jiang, Jing Chen, Guichun Yang, Xiaofan Yang, Zhenbing Chen, Cuifen Lu
Construction and application of a MoS₂-based injectable self-healing composite hydrogel with antibacterial and antioxidant dual functions for promoting infected diabetic wound healing.
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Mater. Chem. Front., 2024, 8,3790-3798
DOI: 10.1039/D4QM00578C, Research Article

Yasong Cao, Caili Zhang, Zhonghua Zhao, Haowen Huang, Jiatong Xu, Richao Shen, Cheng Zeng, Jiawei Lv, Ziqiang Lei, Hengchang Ma
Reliable, reasonable isomer effect study based on pyridinium-type cationic fluorophores of o-, m-, and p-TPA-Pyr-BP.
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Nanoscale Horiz., 2024, 9,1962-1977
DOI: 10.1039/D3NH00423F, Communication

Durgesh Kumar, Ramu Maddu, Hong Jing Chung, Hasibur Rahaman, Tianli Jin, Sabpreet Bhatti, Sze Ter Lim, Rachid Sbiaa, S. N. Piramanayagam
Neuromorphic computing based on spin–orbit torque driven domain wall (DW) devices is promising for energy-efficient computation. This study demonstrates energy efficient operations of DW neurons and synapses by novel reading and writing strategies.
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Nanoscale Horiz., 2024, 9,1948-1961
DOI: 10.1039/D4NH00282B, Communication

Open Access

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Fikret Taygun Duvan, Marina Cunquero, Eduard Masvidal-Codina, Steven T. Walston, Maria Marsal, Jose Manuel de la Cruz, Damia Viana, Diep Nguyen, Julie Degardin, Xavi Illa, Julie M. Zhang, Maria del Pilar Bernícola, José Gabriel Macias-Montero, Carles Puigdengoles, Gustavo Castro-Olvera, Elena del Corro, Socrates Dokos, Mokhtar Chmeissani, Pablo Loza-Alvarez, Serge Picaud, Jose A. Garrido
This article presents the development and testing of reduced graphene oxide (rGO) microelectrode arrays for interfacing with retinal neurons, showcasing their potential for high-density visual prosthetics.
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Nanoscale Horiz., 2024, Accepted Manuscript
DOI: 10.1039/D4NH00420E, Communication

Jea Min Cho, Seungsoo Kim, Tae Won Park, Dong Hoon Shin, Yeong Rok Kim, Hyungjun Park, Dong Yun Kim, Soo Hyung Lee, Taegyun Park, Cheol Seong Hwang
The importance of hardware security increases significantly to protect the vast amounts of private data stored on edge devices. Physical unclonable functions (PUFs) are gaining prominence as hardware security primitives...
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J. Mater. Chem. A, 2024, 12,30279-30288
DOI: 10.1039/D4TA04014G, Paper

Kotaro Ishihara, Akinobu Nakada, Hajime Suzuki, Osamu Tomita, Shunsuke Nozawa, Akinori Saeki, Ryu Abe
Function-/site-selective hybridisation of two specific Ru(II) complex catalysts on donor–acceptor conjugated polymers enables bifunctional visible-light water oxidation and CO₂ reduction.
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J. Mater. Chem. A, 2024, 12,30798-30809
DOI: 10.1039/D4TA04194A, Paper

Manigandan Ramadoss, Hesheng Yu, Anand Rajkamal, Gun Jin Yun, Ziheng Zhang, Chengtao Yang, Fei Ma, Yu Wu, Chen Daiqian, Yuanfu Chen
Fe-single-atom-coupled Fe₃C multifunctional catalysts on P-, F-, N-doped CNT deliver comparable OER behavior to RuO₂, better ORR performance than Pt/C, and better ZAB performance than Pt/C–RuO₂, due to the nanoarchitecture and abundant active sites.
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J. Mater. Chem. A, 2024, 12,30743-30756
DOI: 10.1039/D4TA05082G, Paper

Niranjanmurthi Lingappan, Sandhiya Lakshmanan, Wonoh Lee
Designing an efficient and durable electrocatalyst is central to hydrogen production technologies such as hydrogen evolution reaction, oxygen evolution reaction, and urea oxidation reaction.
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J. Mater. Chem. A, 2024, 12,30611-30617
DOI: 10.1039/D4TA05429F, Paper

Yuanzhu Jiang, Aodong Zhu, Teng Liao, Wang Zhao, Mengmeng Cheng, Xinxin Zhang, Yi-Bing Cheng, Junyan Xiao
Phosphate, being a single-component multifunctional additive, serves as a viable material for the carbon electrode in perovskite solar cells. This utilization ensures the device's performance and mitigates the risk of potential lead pollution.
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J. Mater. Chem. A, 2024, 12,30508-30521
DOI: 10.1039/D4TA05908E, Paper

Abdul Basit, Yang-Chin Kao, Yasser A. El-Ossaily, Shiao-Wei Kuo, Mohamed Gamal Mohamed
The Py-Th-TzTz CMP was synthesized through a Schiff base reaction and exhibited a decomposition temperature (T_d10) of 352 °C. In a three-electrode system, it demonstrated a specific capacitance of 652 F g⁻¹.
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J. Mater. Chem. A, 2024, 12,30872-30884
DOI: 10.1039/D4TA05266H, Paper

Haijiao Lin, Hui Wang, Yongguang Yang, Yuxuan Zhang, Ling Li, Youwei Zhao, Wenming Zhang
Smart fabrics with liquid metal reinforced PU/CNT/MXene multilayer structures for constructing multifunctional sensors and wearable electronics.
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J. Mater. Chem. A, 2024, Advance Article
DOI: 10.1039/D4TA06712F, Paper

Jiatong Yan, Meimei Chen, Rui Tan, Chuanxi Lin, Shan Jiang, Weijie Wang, Songyue Pan, Hongyan Xiao, Erhui Ren, Ronghui Guo
With the rapid development of 5G intelligent detection technology, electromagnetic shielding/infrared stealth fabrics with Joule/solar heating performance can meet the needs of wearable electronic devices for multi-application scenarios.
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J. Mater. Chem. C, 2024, 12,17362-17376
DOI: 10.1039/D4TC03397C, Communication

Jungwoo Lee, Chaewon Youn, Jungang Heo, Sungjun Kim
We demonstrate online and offline learning as well as associative learning such as in Pavlov's dog experiments using the non-volatile and volatile properties of HfSiO_x-based FTJs.
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J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC04064C, Paper

Manting Wang, Jiaqi Zhang, Yaoyi Guo, Xiaoyong Zhou, Jie-Xin Wang, Yuan Le
A conductive hydrogel with enhanced mechanical properties and excellent multifunctionality is fabricated by facile direct in situ polymerization. This hydrogel can serve as a wearable strain sensor precisely detecting relative resistance changes.
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J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC03728F, Paper

Junhuan Li, Zhen Tian, Li Su, Yilong Yang, Chang Ding, Chen Wang, Ming Sun, Yong Zhao
A novel WSIT based on TIEL and single-electrode TENG is developed with self-powered optical–electrical dual-mode sensing functionality, which may be widely applicable in fields like intelligent robots, augmented reality, and smart homes.
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J. Mater. Chem. C, 2024, Advance Article
DOI: 10.1039/D4TC04169K, Paper

Shuai Liang, Shi-Kun Yan, Yu-Xuan Wen, Yan-Rui Zhao, Jin Zhang, Ji-Xiang Hu
A novel complex combining photo- and amine-induced chromic, switchable photoluminescence, and photomodulated nonlinear optical properties has been prepared using electron-rich sulfate and electron-deficient 2,4,6-tri(4-pyridyl)-1,3,5-triazine.
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J. Mater. Chem. C, 2024, Accepted Manuscript
DOI: 10.1039/D4TC03444A, Paper

Jiaxuan Pan, JZ Lu, Yichen Shang, Ying Li, Bing Yan
Dopamine and arginine are both important substances in the body and are closely related to human health. Timely detection of their concentration abnormalities is of great significance for dsaevention. In...
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Chem. Soc. Rev., 2024, 53,10523-10574
DOI: 10.1039/D4CS00339J, Review Article

Open Access

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Kanji Saito, Masashi Morita, Tomohiko Okada, Rattanawadee (Ploy) Wijitwongwan, Makoto Ogawa
The replacement of the main components with a small amount of heteroelements in a material affects its properties and imparts novel functions, similar to “wasabi” giving the important taste for “sushi”.
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Chem. Soc. Rev., 2024, 53,11045-11099
DOI: 10.1039/D4CS00369A, Review Article

Open Access

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Vasudevan Dhayalan, Vishal S. Dodke, Marappan Pradeep Kumar, Hatice Seher Korkmaz, Anja Hoffmann-Röder, Pitchamuthu Amaladass, Rambabu Dandela, Ragupathy Dhanusuraman, Paul Knochel
This review presents various new strategies for the functionalization of 5 and 6-membered fused heteroaromatics. These synthetic strategies enable rapid access to complex heterocyclic compounds.
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Environ. Sci.: Processes Impacts, 2024, Accepted Manuscript
DOI: 10.1039/D4EM00010B, Paper

Durgalakshmi Rajendran, Mahalakshmi Kamalakkannan, George Priya Doss C, Natarajan Chandrasekaran
Despite a significant amount of research on micronanoplastics (MNPs), there is still a gap in our understanding of their function as transporters of other environmental pollutants (known as the Trojan...
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Mater. Horiz., 2024, 11,1719-1731
DOI: 10.1039/D3MH02115G, Communication

Liang Xie, Wei Zhou, Yuming Huang, Zhibin Qu, Longhao Li, Chaowei Yang, Yani Ding, Junfeng Li, Xiaoxiao Meng, Fei Sun, Jihui Gao, Guangbo Zhao, Yukun Qin
While current experimental and computational studies often concentrate on introducing external structures or idealized MN₄ models, we emphasize the often-overlooked impact of inherent OGs within the carbon structure of MN₄ materials, presenting a new perspective on their catalytic activity origin.
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Mater. Horiz., 2024, 11,1608-1610
DOI: 10.1039/D4MH90010C, Commentary

Xiang-Sen Meng, Li-Bo Mao, Shu-Hong Yu
Yu et al. reflect on their first Materials Horizons paper (Mater. Horiz., 2014, https://doi.org/10.1039/c3mh00040k) published in the inaugural issue of the journal, and discuss how their work may have influenced the research field over the past decade.
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Mater. Horiz., 2024, Advance Article
DOI: 10.1039/D4MH00228H, Communication

Wenping Ma, Yi Zheng, Guangzhen Yang, Hongjian Zhang, Mingxia Lu, Hongshi Ma, Chengtie Wu, Hongxu Lu
An optimized CS/GelMA composite hydrogel is designed for organoid development, which can be used as a substrate for supporting intestinal and liver organoid formation and functionalization.
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Mater. Horiz., 2024, Accepted Manuscript
DOI: 10.1039/D3MH02108D, Communication

Kai Tuo, Jin Li, Yi Li, Chuyao Liang, Cuicui Shao, Weifeng Hou, Zhijian Li, Shouzhi Pu, Chunhui Deng
Efficient uranium extraction from seawater is critical for developing the nuclear industry. Herein, a polydopamine/salicylaldoxime decorated hierarchical zeolite imidazolate framework-8 (H-PDA/SA-ZIF-8) is constructed by using a controlled etching process. Benefiting...
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Mater. Horiz., 2024, 11,1975-1988
DOI: 10.1039/D3MH02074F, Communication

Ao Yin, Ruiguang Chen, Rui Yin, Shiqiang Zhou, Yang Ye, Yuxin Wang, Peike Wang, Xue Qi, Haipeng Liu, Jiang Liu, Suzhu Yu, Jun Wei
Our study shows an ultra-soft conductive material with excellent adhesive ability to solve the mismatch of the interface. With coupled microstructures, our sensor demonstrates a remarkable sensitivity and a fast response time.
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Inorg. Chem. Front., 2024, 11,2128-2135
DOI: 10.1039/D4QI00002A, Research Article

Ernan Pang, Shijia Li, Jie Wu, Qing Chang, Ning Li, Jinlong Yang, Shengliang Hu
Carbon dots create the appropriate oxygen vacancies (OVs) in CeVO₄ for the chemoselective hydrogenation of functionalized nitroarenes under light irradiation.
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Inorg. Chem. Front., 2024, 11,2152-2163
DOI: 10.1039/D3QI02575F, Research Article

Fengjing Lei, Xunwei Ma, Xinyun Shao, Ziyan Fang, Yuqin Wang, Weiju Hao
An iron-regulated three-dimensional nano-conical, economical, and flexible Fe-NiS@HA electrode exhibiting high intrinsic activity is prepared by gentle one-step electroless plating for efficient, durable hydrogen production in alkaline seawater.
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