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Updates from the Veterans History Project (VHP):

By memory.loc.gov
Published On :: Thu, 03 Jan 2019 14:03:36 -0600

Join VHP in our remembrance of World War II veteran Richard Overton, formerly, the oldest World War II veteran in the United States. His decorated career ranged from aftermath of the Attack on Pearl Harbor through intense ground combat on the island of Iwo Jima. Our hearts go out to his family and our utmost thanks go to Corporal Overton for his service to our country.

Through the voluntary efforts of the American Red Cross of Central Texas, we are lucky enough to have an oral history interview from this American hero, and you can watch it at https://go.usa.gov/xEYj5

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

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The Power of a Story: In Memoriam of Medal of Honor Recipient Charles S. Kettles

By memory.loc.gov
Published On :: Thu, 24 Jan 2019 11:37:41 -0600

 

How do you measure the weight of a story? Through deeds, dates, or perhaps, a combination of the two? 

Join VHP in our remembrance of Vietnam veteran Charles Seymour Kettles, who received the Medal of Honor in 2016 - nearly 50 years after his helicopter, bleeding fuel and missing its windscreen, touched down with its last load of rescued GIs.

Hear his story and read about the power of recording a veteran's story in Owen Rogers' blog post. 

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

Visit VHP on Facebook.

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The Veterans History Project Asks ‘Which One Do You Love Most?’

By blogs.loc.gov
Published On :: Thu, 14 Feb 2019 10:30:12 -0600

The Veterans History Project (VHP) is asking all LC staff and the general public to help them select images for their new bookmarks. Go to Folklife Today to view 10 images pulled from the VHP collection. Then tell VHP which one you love most either in the blog’s comments section, by email at vohp@loc.gov or in person in room LJ-G51 from now until March 1. VHP will reveal the chosen images on March 15.


The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.


Visit VHP on Facebook.


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Updates from the Veterans History Project (VHP): Veterans Herstory: Decoding Mom’s WWII Service

By blogs.loc.gov
Published On :: Mon, 11 Mar 2019 11:24:24 -0500

 

In her story (herstory), Jean Ashby placed herself and other Navy WAVES into the historical record. Learn more about Ashby's secret encoding work on the VHP Blog and at the Veterans History Project "Code Girls Reunion" broadcast live at 1200 ET on Friday, March 22, 2019. 

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

Visit VHP on Facebook.

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Updates from the Veterans History Project (VHP): The Ones You Love Most

By blogs.loc.gov
Published On :: Fri, 15 Mar 2019 11:08:40 -0500

Thank you to everyone who answered our call to participate in the Veterans History Project’s bookmark image selection! We are pleased to announce the top five images.

See the results, ranked in order of popularity, on the VHP Blog!

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

Visit VHP on Facebook.

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Updates from the Veterans History Project (VHP): Code Girls Reunite!

By content.govdelivery.com
Published On :: Wed, 03 Apr 2019 15:22:49 -0500

"What did you do in the war, mommy?"

VHP commemorated WAVES' wartime contributions with a "Code Girl’s Reunion." This past weekend, NBCs “Sunday Today with Willie Geist” aired a story about this historic event, and interviewed a few of these living legends. If you missed it, you can watch it, here.

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

Visit VHP on Facebook.

Click here for more information.


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Updates from the Veterans History Project (VHP): Wave-Off! VHP Information Center Closed on April 9, 2019

By www.loc.gov
Published On :: Thu, 04 Apr 2019 09:30:25 -0500

On Tuesday, April 9, the Great Hall, all exhibitions, and the Library Shop in the Thomas Jefferson Building of the Library of Congress will be closed for a special event, including the VHP Information Center.

Researchers with Library-issued credentials may access the Jefferson Building reading rooms, including the American Folklife Center Reading Room, as they will be open normal hours of service with access via the Southeast (2nd Street) entrance from 8:30AM to 5:00PM. All reading rooms and exhibitions in the Madison and Adams buildings will operate under normal hours of service.

The Jefferson building will resume regular hours on Wednesday, April 10, 2019.

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

Visit VHP on Facebook.

Click here for more information.


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Updates from the Veterans History Project (VHP): Remembering Richard Lugar: 1932-2019

By memory.loc.gov
Published On :: Mon, 29 Apr 2019 09:52:41 -0500

The Honorable Richard Lugar passed away last night, leaving behind a legacy of both lawmaking and local history. Through the efforts of his Senate Office, nearly 9,000 Indianan veterans’ voices were recorded and preserved – a capstone achievement accessible through the Library of Congress Veterans History Project (VHP).

Years after leaving office, Lugar returned to the mission of the Veterans History Project, this time, offering his oral history of Cold War naval service. As have many VHP participants, he shared his story with a close friend, the Honorable Joe Donnelly.

The mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of U.S. veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets.

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Updates from the Veterans History Project (VHP): Veteran Art Showcase at the Library of Congress

By www.eventbrite.com
Published On :: Tue, 29 Oct 2019 13:20:44 -0500

From November 5-9th, the Library of Congress Veterans History Project (VHP) will host a Veteran Art Showcase. This series of cultural events highlights art and artists with a focus on the myriad experiences of military veterans. The five-day Showcase begins a yearlong commemoration of VHP’s 20th anniversary, and will be held in the Library of Congress Jefferson Building, located at 10 First Street SE, Washington, DC. The schedule is as follows:

Tues., Nov. 5

Craft in America: Ceramic Demonstration, 9 am- 3:30pm -LJG-51

Ceramic artists Matthew Krousey, Judas Recendez, and Ehren Tool participate in a clay throwing demonstration. While throwing, Tool will engage in conversation on the experience of service and war. He will share his pieces with military connected audience members.

Tues., Nov. 5

Craft in America: Veteran Potters Panel Discussion, 5 pm- Whitall Pavilion

Artists Judas Recendez, Matthew Krousey, and Ehren Tool will discuss their ceramic art and process in relation to their military service.  The panel will be moderated by Carol Sauvion, creator and co-executive producer of the PBS series Craft in America.

Weds., Nov. 6

Occupational Poetry, 1pm- Room LJ-119

Poets Bill Jones, (veteran poet)  Vess Quinlan (cowboy poet), Jerry Brooks (miner poet), and Meezie Hermansen (fisher poet) recite some of their work related to their profession, and participate in a panel discussion. The panel will be moderated by John Fenn, Head of Research and Programs at the American Folklife Center.

Thurs. Nov. 7

Combat Paper, 11 am- Whitall Pavilion

Veterans and civilians discuss the process and experience of paper-making and printmaking as a creative outlet in a panel featuring Tara Tappert, Drew Matott, Ruth Lynne McIntosh, and Patrick Sargent.  The panel will be moderated by Katherine Blood, Curator of Fine Prints at the Prints and Library’s Photographs Division.

The Telling Project, 7pm- Great Hall

An autobiographical performance of “She Went to War,” featuring four female veterans, all of whom experienced significant combat exposure while serving in the military.

Sat. Nov. 9

Operation Song and Jamie Fox Perform Live, 7pm- Coolidge Auditorium

Tennessee-based not-for-profit program “Operation Song” performs a selection of songs written by and about veterans, active duty service members and their loved ones. Jamie Fox, an Air Force veteran and Metis fiddler of the Aaniih and Nakoda tribes performs tunes that were derived from a mixture of Celtic, French, and Native American cultures.

The Veteran Art Showcase is free of charge, and open to the public; however, due to expected demand, tickets are recommended and available on a first –come, first served basis. For more information, visit https://www.eventbrite.com/o/library-of-congress-11132539071 or VHP’s Facebook page at www.facebook.com/vetshistoryproject.

Request ADA accommodations at least five business days in advance by contacting (202) 707-6362 or ada@loc.gov.

Click here for more information.


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Updates from the Veterans History Project (VHP): Call for Applicants: 2020 Bartis Folklife Internships

By www.usajobs.gov
Published On :: Wed, 29 Jan 2020 13:05:18 -0600

The Library of Congress American Folklife Center (AFC) recently announced two paid internship opportunities. For 10 weeks, interns will be immersed in the environment and activities of the American Folklife Center, which pairs robust cultural programming with the world's largest ethnographic archive.

Applications for the Bartis Folklife Internship will be considered until March 28, 2018. This fellowship is named for - and supported by - the generosity of Dr. Peter Bartis, the longest serving AFC employee. From 2001 – 2008, his expertise and unique vision established VHP as one of the largest oral history projects in the world. His collegiality defined the character, spirit, and intersections of AFC and VHP.

The Mission of the Veterans History Project of the Library of Congress American Folklife Center is to collect, preserve and make accessible the personal accounts of American war veterans so that future generations may hear directly from veterans and better understand the realities of war. Learn more at http://www.loc.gov/vets. Share your exciting VHP initiatives, programs, events and news stories with VHP to be considered for a future RSS. Email vohp@loc.gov and place “My VHP RSS Story” in the subject line.

Visit VHP on Facebook.

Click here for more information.


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Transferring Axial Molecular Chirality Through a Sequence of On-Surface Reactions

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01653E, Edge Article
Open Access
Néstor Merino-Díez, Mohammed S. G. Mohammed, Jesus Castro, Luciano Colazzo, Alejandro Berdonces-Layunta, James Lawrence, Jose Ignacio Pascual, Dimas G. de Oteyza, Diego Peña
Fine management of chiral processes on solid surfaces has progressed over the years, yet still faces the need for the controlled and selective production of advanced chiral materials. Here, we...
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Cascade polymerizations: recent developments in the formation of polymer repeat units by cascade reactions

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01475C, Perspective
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Gregory I. Peterson, Tae-Lim Choi
Cascade polymerizations provide new routes to unique polymer structures. In this perspective, we summarize their performance, monomer scope, and mechanisms.
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Copper-catalysed photoinduced decarboxylative alkynylation: a combined experimental and computational study

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC02213F, Edge Article
Open Access
Yu Mao, Wenxuan Zhao, Shuo Lu, Lei Yu, Yi Wang, Yong Liang, Shengyang Ni, Yi Pan
Redox-active esters (RAEs) as alkyl radical precursors have demonstrated great advantages for Cu-catalysed C–C bond formation.
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Spectroscopic investigations under whole-cell conditions provide new insight into the metal hydride chemistry of [FeFe]-hydrogenase

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00512F, Edge Article
Open Access
Lívia S. Mészáros, Pierre Ceccaldi, Marco Lorenzi, Holly J. Redman, Emanuel Pfitzner, Joachim Heberle, Moritz Senger, Sven T. Stripp, Gustav Berggren
The mechanism of hydrogen gas formation by [FeFe] hydrogenase is probed under whole cell conditions, revealing the formation of reactive metal hydride species under physiologically relevant conditions.
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Retrosynthetic strategies and their impact on synthesis of arcutane natural products

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01441A, Minireview
Open Access
Shelby V. McCowen, Nicolle A. Doering, Richmond Sarpong
Decisions, decisions, decisions: the interplay between different retrosynthetic strategies in the synthesis of the highly bridged, polycyclic arcutane natural products.
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Evolutionary chemical space exploration for functional materials: computational organic semiconductor discovery

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00554A, Edge Article
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Chi Y. Cheng, Josh E. Campbell, Graeme M. Day
Evolutionary optimisation and crystal structure prediction are used to explore chemical space for molecular organic semiconductors.
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Structure-mechanics statistical learning unravels the linkage between local rigidity and global flexibility in nucleic acids

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00480D, Edge Article
Open Access
Yi-Tsao Chen, Haw Yang, Jhih-Wei Chu
The mechanical properties of nucleic acids underlie biological processes ranging from genome packaging to gene expression. We devise structural mechanics statistical learning method to reveal their molecular origin in terms of chemical interactions.
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The assemble, grow and lift-off (AGLO) strategy to construct complex gold nanostructures with pre-designed morphologies

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00553C, Edge Article
Open Access
Xin Luo, Christophe Lachance-Brais, Amy Bantle, Hanadi F. Sleiman
The AGLO strategy generates complex gold nanostructures with user-designed morphologies in solution, using only a simple 2D DNA origami sheet as a versatile transient template. The products are robust and stable as standalone gold nanostructures.
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Aerosol-assisted route to low-E transparent conductive gallium-doped zinc oxide coatings from pre-organized and halogen-free precursor

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00502A, Edge Article
Open Access
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Clara Sanchez-Perez, Sebastian C. Dixon, Jawwad A. Darr, Ivan P. Parkin, Claire J. Carmalt
A pre-organised and halogen-free ZnO precursor is used to deposit GZO coatings via aerosol-assisted CVD with properties that exceed industrial standards for low-E coatings and photovoltaics.
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When Hollow Multi-Shelled Structures (HoMSs) Meet Metal-Organic Frameworks (MOFs)

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01284J, Perspective
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Zumin Wang, Nailiang Yang, Dan Wang
Hollow multishelled structures (HoMSs) have distinguished advantages, such as large effective surface area, short mass transport route, and high loading capacity, but the fabrication of HoMS was a big challenge....
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Spontaneous mirror symmetry breaking in benzil-based soft crystalline, cubic liquid crystalline and isotropic liquid phases

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01396J, Edge Article
Open Access
Tino Reppe, Silvio Poppe, Xiaoqian Cai, Yu Cao, Feng Liu, Carsten Tschierske
Benzil (diphenylethane-1,2-dione), which is a long known example for an achiral molecule crystallizing in a chiral space group, can also show mirror symmetry breaking in the fluid state if it...
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Palladium-catalysed 5-endo-trig allylic (hetero)arylation

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01932A, Edge Article
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Bara Singh, Siddheshwar K. Bankar, Ketan Kumar, S. S. V. Ramasastry
A palladium-catalysed intramolecular allylic (hetero)arylation strategy for the synthesis of fused cyclopentenes incorporated with all-carbon quaternary and spiro centres is described.
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Allylic C(sp3)–H alkylation via synergistic organo- and photoredox catalyzed radical addition to imines

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00819B, Edge Article
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Jiaqi Jia, Rajesh Kancherla, Magnus Rueping, Long Huang
A new catalytic method for the direct alkylation of allylic C(sp3)–H bonds from unactivated alkenes via synergistic organo- and photoredox catalysis is described.
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Transformation from helical to layered supramolecular organization of asymmetric perylene diimides via multiple intermolecular hydrogen bonding

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01911A, Edge Article
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Mengmeng Li, Wojciech Zajaczkowski, Gangamallaiah Velpula, Daniel Jänsch, Robert Graf, Tomasz Marszalek, Sapun H. Parekh, Yulian Zagranyarski, Kunal Mali, Manfred Wagner, Steven De Feyter, Chen Li, Klaus Müllen, Wojciech Pisula
The solid-state supramolecular organization of asymmetric perylene diimide is transformed from helical to layered self-assembly after thermal annealing.
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Ultrafast Amidation of Esters using Lithium Amides under Aerobic Ambient Temperature Conditions in Sustainable Solvents

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01349H, Edge Article
Open Access
Michael Fairley, Leonie Bole, Florian Mulks, Laura Main, Alan Kennedy, Charles T. O'Hara, Joaquín García-Álvarez, Eva Hevia
Lithium amides constitute one of the most commonly used class of reagents in synthetic chemisty. However, despite many applications, their use is handicapped by their requirements of low temperatures, in...
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Covalent Organic Frameworks as Microreactors: Confinement-enhanced Electrochemiluminescence

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01817A, Edge Article
Open Access
Wei-Jia Zeng, Kun Wang, Wenbin Liang, Yaqin Chai, Ruo Yuan, Ying Zhuo
Herein, the electrochemiluminescence (ECL) microreactors with enhanced intensity and extreme stability were firstly established by the assembly of tris(2,2’-bipyridyl) ruthenium (II) (Ru(bpy)32+) onto the covalent organic frameworks (COFs) where a...
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Crystallographic facet selective HER catalysis: exemplified in FeP and NiP2 single crystals

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00676A, Edge Article
Open Access
Bryan Owens-Baird, Juliana P. S. Sousa, Yasmine Ziouani, Dmitri Y. Petrovykh, Nikolai A. Zarkevich, Duane D. Johnson, Yury V. Kolen'ko, Kirill Kovnir
The effect of the crystal structure of ordered transition-metal phosphide catalysts on the hydrogen-evolution reaction is investigated using single crystals of iron-phosphide (FeP) and monoclinic nickel-diphosphide (m-NiP2).
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Thermal effects – an alternative mechanism for plasmon-assisted photocatalysis

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/C9SC06480J, Edge Article
Open Access
Yonatan Dubi, Ieng Wai Un, Yonatan Sivan
A simple Arrhenius-based theory of heating, rather than “hot electrons”, can reproduce some high-profile photocatalysis experimental results to remarkable accuracy. Flaws in temperature measurement may have led to wrong conclusions.
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Programmable synthesis of multiply arylated cubanes through C–H metalation and arylation

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01909G, Edge Article
Open Access
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Ryo Okude, Genki Mori, Akiko Yagi, Kenichiro Itami
Cubane has attracted attention due to its unique 3D structure. Herein, we report the programmable synthesis of multiply arylated cubanes. The developed reaction allows the late-stage and regioselective installation of aryl groups.
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Nitric oxide monooxygenation (NOM) reaction of cobalt-nitrosyl {Co(NO)}8 to CoII-nitrito {CoII(NO2−)}: base induced hydrogen gas (H2) evolution

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01572E, Edge Article
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Sandip Das, Kulbir, Somnath Ghosh, Subash Chandra Sahoo, Pankaj Kumar
Base-induced hydrogen (H2) gas evolution in the nitric oxide monoxygenation reaction.
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Introduction of a 7-aza-6-MeO-indoline auxiliary in Lewis-acid/photoredox cooperative catalysis: highly enantioselective aminomethylation of α,β-unsaturated amides

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01890B, Edge Article
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Santosh K. Pagire, Naoya Kumagai, Masakatsu Shibasaki
An efficient cooperative chiral Lewis acid and photoredox catalytic system towards the highly enantioselective radical conjugate addition of α-amino radicals to α,β-unsaturated amides is developed with the implementation of unique auxiliaries.
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Water-induced formation of an alkali-ion dimer in cryptomelane nanorods

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01517B, Edge Article
Open Access
Shaobo Cheng, Vidushi Sharma, Altug S. Poyraz, Lijun Wu, Xing Li, Amy C. Marschilok, Esther S. Takeuchi, Kenneth J. Takeuchi, Marivi Fernández-Serra, Yimei Zhu
Water displaces potassium ions and initiates the formation of a homonuclear dimer ion (K2+) in the tunnels of hollandite.
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A straightforward approach to antibodies recognising cancer specific glycopeptidic neoepitopes

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00317D, Edge Article
Open Access
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Hajime Wakui, Yoshikazu Tanaka, Toyoyuki Ose, Isamu Matsumoto, Koji Kato, Yao Min, Taro Tachibana, Masaharu Sato, Kentaro Naruchi, Fayna Garcia Martin, Hiroshi Hinou, Shin-Ichiro Nishimura
We developed new class of designated antibodies targeting of “dynamic neoepitopes” elaborated by disease-specific O-glycosylation at the immunodominant mucin domains.
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Dynamic reaction-induced phase separation in tunable, adaptive covalent networks

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00605J, Edge Article
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Katie M. Herbert, Patrick T. Getty, Neil D. Dolinski, Jerald E. Hertzog, Derek de Jong, James H. Lettow, Joy Romulus, Jonathan W. Onorato, Elizabeth M. Foster, Stuart J. Rowan
Dynamic covalent networks comprised of tunable thia-Michael bonds result in phase separated networks with tailorable mechanical and adaptive properties.
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Structure of Copper sites in Zeolites Examined by Fourier and Wavelet Transform Analysis of EXAFS

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01472A, Edge Article
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Vitaly L. Sushkevich, Olga V. Safonova, Dennis Palagin, Mark A Newton, Jeroen van Bokhoven
Copper-exchanged zeolites are a class of redox-active materials that find application in the selective catalytic reduction of exhaust gases of diesel vehicles, and, more recently, the selective oxidation of methane...
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Metal-metal cooperative bond activation by heterobimetallic alkyl, aryl, and acetylide PtII/CuI complexes

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC00646G, Edge Article
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Shubham Deolka, Orestes Rivada, Sandra L. Aristizábal, Robert R. Fayzullin, Shrinwantu Pal, Kyoko Nozaki, Eugene Khaskin, Julia R Khusnutdinova
We report selective formation of heterobimetallic PtII/CuI complexes that demonstrate how facile bond activation processes can be achieved by altering reactivity of common organoplatinum compounds through their interaction with another...
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Molecular recognition of pyrazine N,N'-dioxide using aryl extended calix[4]pyrroles

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01496F, Edge Article
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Chenxing Guo, Hu Wang, Vincent M. Lynch, Xiaofan Ji, Zachariah A. Page, Jonathan L. Sessler
The molecular recognition of pyrazine N,N'-dioxide by aryl extended 'two-walled' calix[4]pyrrole-based receptors is seen to stabilise two different binding modes in the solid state.
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Efficient alkene hydrosilation with bis(8-quinolyl)phosphine (NPN) nickel catalysts. The dominant role of silyl-over hydrido-nickel catalytic intermediates

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00997K, Edge Article
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Jian Yang, Verònica Postils, Michael I. Lipschutz, Meg Fasulo, Christophe Raynaud, Eric Clot, Odile Eisenstein, T. Don Tilley
A cationic nickel complex of the bis(8-quinolyl)(3,5-di-tert-butylphenoxy)phosphine (NPN) ligand, [(NPN)NiCl]+, is a precursor to efficient catalysts for the hydrosilation of alkenes with hydrosilanes under mild conditions and low catalyst loadings.
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Expedient synthesis of conjugated triynes via alkyne metathesis

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01124J, Edge Article
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Idriss Curbet, Sophie Colombel-Rouen, Romane Manguin, Anthony Clermont, Alexandre Quelhas, Daniel S. Müller, Thierry Roisnel, Olivier Baslé, Yann Trolez, Marc Mauduit
The first synthesis of symmetrical and dissymmetrical conjugated triynes by self- and cross-metathesis was successfully achieved thanks to the use of hindered diynes.
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Triblock polyester thermoplastic elastomers with semi-aromatic polymer end blocks by ring-opening copolymerization

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC00463D, Edge Article
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Georgina L. Gregory, Gregory S. Sulley, Leticia Peña Carrodeguas, Thomas T. D. Chen, Alba Santmarti, Nicholas J. Terrill, Koon-Yang Lee, Charlotte K. Williams
A new series of block polyester thermoplastic elastomers are prepared by a one-pot procedure; they show properties competitive or better than conventional materials and can be fully degraded after use.
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Stereo-controlled anti-hydromagnesiation of aryl alkynes by magnesium hydrides

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01773F, Edge Article
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Bin Wang, Derek Yiren Ong, Yihang Li, Jia Hao Pang, Kohei Watanabe, Ryo TAKITA, Shunsuke Chiba
A concise protocol for anti-hydromagnesiation of aryl alkynes was established using 1:1 molar combination of sodium hydride (NaH) and magnesium iodide (MgI2) without the aid of any transition metal catalysts....
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Ring-Fused Cyclobutanes via Cycloisomerization of Alkylidenecyclopropane Acylsilanes

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC02224A, Edge Article
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Erick M Carreira, Sarah S Eichenberger, Moritz Hönig, Matthieu JR Richter, Renana Gershoni-Poranne
A novel Lewis acid-catalyzed cycloisomerization of alkylidenecyclopropane acylsilanes is disclosed. The readily available starting materials participate in tandem Prins addition/ring expansion/1,2-silyl shift to grant access to bicyclo[4.2.0]octanes and bicyclo[3.2.0]heptanes, which...
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Protease-Responsive Mass Barcoded Nanotranslaters for Simultaneously Quantifying the Intracellular Activity of Cascaded Caspases in Apoptosis Pathways

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01534B, Edge Article
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Hongmei Xu, Xiaodan Huang, Zhenzhen Zhang, xuemeng zhang, Qianhao Min, Jun-Jie Zhu
Quantitatively delineating the activation network of multiple proteases that participate in cellular processes is highly essential to understanding physiological and pathological states of cells. In this study, protease-responsive mass barcoded...
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Structure and redox tuning of gas adsorption properties in calixarene-supported Fe(II)-based porous cages

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01833C, Edge Article
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Meaghan Deegan, Tonia Ahmed, Glenn Yap, Eric D Bloch
We describe the synthesis of Fe(II)-based octahedral coordination cages supported by calixarene capping ligands. The most porous of these molecular cages has an argon accessible BET surface area of 898...
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Nickel catalysis enables convergent paired electrolysis for direct arylation of benzylic C–H bonds

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01445A, Edge Article
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Lei Zhang, Xile Hu
A direct arylation of benzylic C–H bonds is achieved by integrating Ni-catalyzed benzyl–aryl coupling into convergent paired electrolysis.
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Highly efficient non-doped blue fluorescent OLEDs with low efficiency roll-off based on hybridized local and charge transfer excited state emitters

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01341B, Edge Article
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Xianhao Lv, Mizhen Sun, Lei Xu, Runzhe Wang, Huayi Zhou, Yuyu Pan, Shitong Zhang, Qikun Sun, Shanfeng Xue, Wenjun Yang
A new pure fluorescent blue HLCT-emitter was designed and synthesized. Highly efficient non-doped blue OLEDs with low efficiency roll-off were achieved.
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Pore engineering of ultrathin covalent organic framework membranes for organic solvent nanofiltration and molecular sieving

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC01679A, Edge Article
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Digambar B. Shinde, Li Cao, A. D. Dinga Wonanke, Xiang Li, Sushil Kumar, Xiaowei Liu, Mohamed N. Hedhili, Abdul-Hamid Emwas, Matthew Addicoat, Kuo-Wei Huang, Zhiping Lai
Pore surface engineering of ultrathin COF membranes by introducing different lengths of alkyl chains into the skeleton, which allows us to precisely control the pore size of COF membranes for OSN applications and molecular sieving.
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Asymmetric synthesis of primary amines catalyzed by thermotolerant fungal reductive aminases

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Chem. Sci., 2020, Advance Article
DOI: 10.1039/D0SC02253E, Edge Article
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Juan Mangas-Sanchez, Mahima Sharma, Sebastian C. Cosgrove, Jeremy I. Ramsden, James R. Marshall, Thomas W. Thorpe, Ryan B. Palmer, Gideon Grogan, Nicholas J. Turner
Fungal reductive aminases as effective biocatalysts for the preparation of chiral primary amines.
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Speciation of Be2+ in acidic liquid ammonia and formation of tetra- and octanuclear beryllium amido clusters

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01112F, Edge Article
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Matthias Müller, Antti J Karttunen, Magnus Richard Buchner
The hexa-μ2-amido-tetraammine-tetraberyllium compounds [Be4(NH2)6(NH3)4]X2 (X = Cl, Br, I, CN, SCN, N3) have been prepared from beryllium metal and NH4X or [Be(NH3)4]X2 in liquid ammonia at ambient temperature. The obtained...
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Regioselective B(3,4)–H Arylation of o-Carboranes by Weak Amide Coordination at Room Temperature

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Chem. Sci., 2020, Accepted Manuscript
DOI: 10.1039/D0SC01515F, Edge Article
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Yu-Feng Liang, Long Yang, Becky Bongsuiru Jei, Rositha Kuniyil, Lutz Ackermann
Palladium-catalyzed regioselective di- or mono-arylation of o-carboranes was achieved by weakly coordinating amides at room temperature. Thereby, a series of B(3,4)-diarylated and B(3)-monoarylated o-carboranes anchored with valuable functional groups were...
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