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[ASAP] Sesquicarbene Complexes: Bonding at the Interface Between M–C Single Bonds and M-C Double Bonds

By feedproxy.google.com
Published On :: Thu, 07 May 2020 04:00:00 GMT

Organometallics
DOI: 10.1021/acs.organomet.0c00102


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[ASAP] Catalytic Dimerization of Alkynes via C–H Bond Cleavage by a Platinum–Silylene Complex

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Published On :: Fri, 08 May 2020 04:00:00 GMT

Organometallics
DOI: 10.1021/acs.organomet.0c00195


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[ASAP] Synthesis, Structures, and Electronic Properties of O- and S-Heterocyclic Carbene Complexes of Iridium, Copper, Silver, and Gold

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Published On :: Fri, 08 May 2020 04:00:00 GMT

Organometallics
DOI: 10.1021/acs.organomet.0c00066


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The Difficult First Episode

By backtofrontshow.com
Published On :: Sat, 19 Jan 2013 03:00:00 +0000

In our very first episode we discuss the difficulty of writing your own online biography, the pros and cons of co-working, the move towards flat file site generation, the upcoming New Adventures in Web Design conference, the shiny new Rode iXY microphone and end with bespoke fixed gear bikes.


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Celebrities on KickStarter

By backtofrontshow.com
Published On :: Mon, 13 May 2013 09:00:00 +0000

This weeks show is kindly supported by Insites: ConfShop — A unique one day event for web workers focused on openness, sharing and learning taking place in London on Friday July 5th. Tickets are limited to 100 and are available for £125.

In this episode we tell you about our new “studio”, discuss the route to inner nirvana (no really), the “problem” of celebrities on KickStarter and ask whether Ghost is the future of blogging as we know it.

Thanks again to Insites: ConfShop for supporting this weeks episode.


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New Flickr, New Digg!

By backtofrontshow.com
Published On :: Sat, 22 Jun 2013 05:00:00 +0000

We are back behind the Yeti’s to discuss Keir’s trip to Beyond Tellerrand, the new Flickr subscription model, Digg Reader, Prism and our recent Mac email client woes. We round out the show with quite possibly the best use of technology we have come across – intrigued? You should be!


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The Problem of Overfunding on KickStarter

By backtofrontshow.com
Published On :: Thu, 25 Jul 2013 05:00:00 +0000

As the web appears to have gone on holiday we present a mixed bag of goodness on Episode 010. We lament the loss of one of our zero’s, Kieran brings forth the news and the funny and we engage in a almost academic level of discourse on the issues associated with overfunding on crowdfunding platforms. Also included – a bit of Startup talk, a new Mac code editor, the new Royal baby and our first ever competition.

Lunchbox Competition

To enter the Back to Front Show lunchbox giveaway simply tweet the answer to the following question before Friday 2nd August 2013. All correct answers will be entered into the draw. If nobody guesses correctly the closest response will win.

Question: What is the height difference in inches between Kieran and Keir?


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Six Choice Cuts

By backtofrontshow.com
Published On :: Thu, 29 Aug 2013 07:00:00 +0000

Episode #013 is brought to you in association with Squarespace, the all-in-one platform that makes it fast and easy to create your own professional website or online portfolio. For a free trial and 10% off, go to squarespace.com and use offer code Backtofront8.

This week there’s a change to our format as we strive to go weekly. In our new “8bit-minified-compressed” format we discuss six choice cuts found around the web including Google and Uber, Local Tunnel and the trend of coffee cups in web marketing.

Thanks again to Squarespace for supporting the show


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'Pvt hosp staff at par with govt medical staff'

By timesofindia.indiatimes.com
Published On :: Fri, 08 May 2020 19:55:52 IST


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Covid-19 medical staff to get addl compensation

By timesofindia.indiatimes.com
Published On :: Fri, 08 May 2020 17:44:55 IST

The Amdavad Municipal Corporation (AMC) has decided to give additional financial compensation to health and paramedical staff of AMC and private designated Covid-19 hospitals who contact coronavirus infection on duty.


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Gujarat HC restores land to civic body from royals

By timesofindia.indiatimes.com
Published On :: Sat, 09 May 2020 06:42:55 IST

The Gujarat high court rebuked the erstwhile royal family of the princely state of Bhavnagar for its "dishonest intention" to claim a land parcel in an unauthorized manner from the Bhavnagar Municipal Corporation.


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Migrant workers clash with police in Surat

By timesofindia.indiatimes.com
Published On :: Sat, 09 May 2020 12:46:48 IST

Demanding a return passage to their home states, hundreds of agitated migrant workers clashed with the police at Mora village in Gujarat's Surat district on Saturday, an official said.


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Resource Showcase: Daily Mirror Historical Archive

By www.dur.ac.uk
Published On :: Thu, 07 May 2020 09:57:36 +0100

The archive features more than 800,000 pages of brand-new, full text searchable, scans of the complete run of the Mirror from 1903-2000, including the Sunday Mirror. This is one of many e-resources we currently have on trial. You can see the complete list and gain access via our trial e-resources page. Please remember to leave feedback – your opinions help shape our collections. See what other newspapers and news services are available via Durham University Library and Collections


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Synthesis of lignin-functionalized phenolic nanosphere supported Ag nanoparticles with excellent dispersion stability and catalytic performance

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/C9GC04311J, Paper
Shilin Chen, Guanhua Wang, Wenjie Sui, Ashak Mahmud Parvez, Chuanling Si
This work presents a novel and green lignin-based nanocomposite and highlights the synergism of lignin's multiple functions (surfactant, sacrificial template, and reducing agent) in the material preparation process.
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Simplifying levulinic acid conversion towards a sustainable biomass valorisation

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Green Chem., 2020, Advance Article
DOI: 10.1039/C9GC04306C, Paper
Chiara Defilippi, Daily Rodríguez-Padrón, Rafael Luque, Cristina Giordano
In the range of biomass valorisation, hydroconversion of levulinic acid (one of the products of the hydrolysis of lignocellulosic biomass) was tested for the first time using nanosized Ni3N and Ni0 catalysts, with very promising results alongside high stability.
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One-pot hydrodeoxygenation of biomass furan derivatives into decane under mild conditions over Pd/C combined with phosphotungstic acid

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00428F, Paper
Song Li, Long Yan, Qiying Liu, Jianguo Liu, Qiyu Liu, Wei Fan, Xuelai Zhao, Xinghua Zhang, Chenguang Wang, Longlong Ma, Qi Zhang
One-pot hydrodeoxygenation of δ-furfurylidenelevulinic acid over Pd/C combined with phosphotungstic acid through successive hydrogenolysis and HDO of furans and lactones.
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Water Effects in the Heterogeneous Catalytic Valorization of Levulinic Acid into γ-Valerolactone and its Derivatives

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC01082K, Critical Review
Rengui Weng, Zhihao Yu, Jian Xiong, Xuebin Lu
Levulinic acid (LA), which has been hailed as a versatile biomass-derived platform molecular, typically occupy a core position in the cellulosic biorefinery system. The heterogeneous catalytic valorization of LA for...
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Humin based resin for wood modification and property improvement

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Green Chem., 2020, Advance Article
DOI: 10.1039/C9GC03620B, Paper
Open Access
Anna Sangregorio, Anitha Muralidhara, Nathanael Guigo, Lisbeth G. Thygesen, Guy Marlair, Carlo Angelici, Ed de Jong, Nicolas Sbirrazzuoli
Focus on humins, a co-product from sugar conversion, to highlight their capacity to impregnate wood cell walls for making durable wood products.
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Methylation-triggered fractionation of lignocellulosic biomass to afford cellulose-, hemicellulose-, and lignin-based functional polymers via click chemistry

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00451K, Paper
Kentaro Miki, Hiroshi Kamitakahara, Arata Yoshinaga, Yuki Tobimatsu, Toshiyuki Takano
This paper reports a new concept for the biorefinery of lignocellulosic biomass where the derivatisation and fractionation of lignocellulose are accomplished at the same time.
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Sustainable synthesis of cobalt and cobalt oxide nanoparticles and their catalytic and biomedical applications

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00885K, Critical Review
Siavash Iravani, Rajender S. Varma
Recent advances and essential challenges as well as catalytic and biomedical applications of cobalt oxide and cobalt nanoparticles are highlighted.
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Aqueous miscible organic layered double hydroxides as catalyst precursors for biodiesel synthesis

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00571A, Paper
Chunping Chen, Maxwell Greenwood, Jean-Charles Buffet, Dermot O'Hare
Surface area and basicity density dependence of base-catalysed transesterification of sunflower oil by potassium salt prepared AMO-layered double hydroxides.
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Eco-friendly and sustainable synthesis of biocompatible nanomaterials for diagnostic imaging: current challenges and future perspectives

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00734J, Critical Review
Ghazaleh Jamalipour Soufi, Siavash Iravani
Current advancements, important challenges and future perspectives of biocompatible nanomaterials for diagnostic imaging are discussed as well as their greener synthesis.
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New biobased-zwitterionic ionic liquids: efficiency and biocompatibility for the development of sustainable biorefinery processes

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Published On ::

Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC01002B, Paper
Gaël Huet, Monica Araya-Farias, Ranim Alayoubi, Sylvain Laclef, Benjamin Bouvier, Isabelle Gosselin, Christine Cézard, Romain Roulard, Matthieu Courty, Caroline Hadad, Eric Husson, Catherine Sarazin, Albert Nguyen Van Nhien
A combination of experiments and modeling reveals the influence of alkyl chain lengths in biobased ZILs on the biocompatibility towards various microorganisms.
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Synthesis of amorphous Geobacter-manganese oxide biohybrid as efficient water oxidation catalysts

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/C9GC04353E, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Shafeer Kalathil, Krishna Katuri, Pascal Saikaly
The development of low cost and efficient oxygen evolution reaction (OER) catalyst has paramount importance to meet future sustainable energy demand. Nature’s photosynthetic machinery deploy manganese-based complex in photosystem II...
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Thermophilic bio-electro CO2 recycling into organic compounds

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Green Chem., 2020, Advance Article
DOI: 10.1039/D0GC00320D, Paper
Open Access
Laura Rovira-Alsina, Elisabet Perona-Vico, Lluís Bañeras, Jesús Colprim, M. Dolors Balaguer, Sebastià Puig
Many industrial combustion processes produce carbon dioxide (CO2) at high temperature, which may be electrically recycled into valuable chemicals using microorganisms as catalysts.
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Solvent-free hydrogenation of levulinic acid to γ-valerolactone using a Shvo catalyst precursor: optimization, thermodynamic insights, and life cycle assessment

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Published On ::

Green Chem., 2020, 22,2443-2458
DOI: 10.1039/C9GC02088H, Paper
Open Access
  This article is licensed under a Creative Commons Attribution 3.0 Unported Licence.
Christian A. M. R. van Slagmaat, Marie A. F. Delgove, Jules Stouten, Lukas Morick, Yvonne van der Meer, Katrien V. Bernaerts, Stefaan M. A. De Wildeman
We studied the solvent-free hydrogenation of levulinic acid to γ-valerolactone with the Shvo catalyst involving comparative catalysis, DFT, and LCA.
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Ga/ZSM-5 catalyst improves hydrocarbon yields and increases alkene selectivity during catalytic fast pyrolysis of biomass with co-fed hydrogen

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Published On ::

Green Chem., 2020, 22,2403-2418
DOI: 10.1039/C9GC03408K, Paper
Kristiina Iisa, Yeonjoon Kim, Kellene A. Orton, David J. Robichaud, Rui Katahira, Michael J. Watson, Evan C. Wegener, Mark R. Nimlos, Joshua A. Schaidle, Calvin Mukarakate, Seonah Kim
An integrated experimental and computational study to understand the catalytic upgrading of biomass vapors into high yield of alkenes.
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Insights into pressure tunable reaction rates for electrochemical reduction of CO2 in organic electrolytes

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Published On ::

Green Chem., 2020, 22,2434-2442
DOI: 10.1039/D0GC00013B, Paper
Charles I. Shaughnessy, David J. Sconyers, Hyun-Jin Lee, Bala Subramaniam, James D. Blakemore, Kevin C. Leonard
Modeling and simulation reveal the mechanistic basis for the pressure-tunable rates of CO2 reduction at elevated pressures of CO2.
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Dioxomolybdenum complex as an efficient and cheap catalyst for the reductive depolymerization of plastic waste into value-added compounds and fuels

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Published On ::

Green Chem., 2020, 22,2419-2425
DOI: 10.1039/C9GC04206G, Paper
Beatriz F. S. Nunes, M. Conceição Oliveira, Ana C. Fernandes
Several types of PCL, PLA, PDO, PET and PBT plastic waste were efficiently converted into value-added compounds and fuels catalyzed by MoO2Cl2(H2O)2.
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Synthesis of renewable C–C cyclic compounds and high-density biofuels using 5-hydromethylfurfural as a reactant

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Published On ::

Green Chem., 2020, 22,2468-2473
DOI: 10.1039/D0GC00195C, Paper
Taimei Cai, Qiang Deng, Hailong Peng, Jin Zhong, Rui Gao, Jun Wang, Zheling Zeng, Ji-Jun Zou, Shuguang Deng
Renewable C–C six-membered ring compound and high-density biofuel are synthesized using 5-hydromethylfurfural as a reactant.
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Novel insights into biomass delignification with acidic deep eutectic solvents: a mechanistic study of β-O-4 ether bond cleavage and the role of the halide counterion in the catalytic performance

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Published On ::

Green Chem., 2020, 22,2474-2487
DOI: 10.1039/C9GC02569C, Paper
André M. da Costa Lopes, José R. B. Gomes, João A. P. Coutinho, Armando J. D. Silvestre
The potentiality of acidic deep eutectic solvents for β-O-4 ether bond cleavage is herein demonstrated from a mechanistic point of view.
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Efficient base-free oxidation of monosaccharide into sugar acid under mild conditions using hierarchical porous carbon supported gold catalysts

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Published On ::

Green Chem., 2020, 22,2588-2597
DOI: 10.1039/C9GC04333K, Paper
Xintong Meng, Zengyong Li, Di Li, Yiming Huang, Jiaojiao Ma, Chuanfu Liu, Xinwen Peng
The highly selective synthesis of D-xylonic acid and D-gluconic acid from monosaccharide catalyzed by Au/NC-3 under base-free aerobic oxidation conditions.
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Direct C(sp3)–H acyloxylation of indolin-3-ones with carboxylic acids catalysed by KI

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Published On ::

Green Chem., 2020, 22,2354-2358
DOI: 10.1039/C9GC04446A, Communication
Yong-Long Zhao, Yong-Qin Tang, Xing-Hai Fei, Fen-Fen Yang, Zhuo-Xian Cao, Dong-Zhu Duan, Qing-Jie Zhao, Yuan-Yong Yang, Meng Zhou, Bin He
The first KI-catalyzed direct acyloxylation of indolin-3-ones with carboxylic acids has been developed using 30% aq. H2O2 as a green oxidant at room temperature. Moreover, mechanism studies indicated that a radical oxidation process may be involved for this transformation.
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Synthesis of bioderived polycarbonates with adjustable molecular weights catalyzed by phenolic-derived ionic liquids

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Green Chem., 2020, 22,2488-2497
DOI: 10.1039/D0GC00493F, Paper
Wei Qian, Lei Liu, Zengliang Zhang, Qian Su, Weizhen Zhao, Weiguo Cheng, Li Dong, Zifeng Yang, Ruibing Bai, Fei Xu, Yanqiang Zhang, Suojiang Zhang
Phenolic ionic liquid structure can be designed readily to control the molecular weight of isosorbide-derived polycarbonates.
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Fabrication of highly proton-conductive chitosan whole-bio-membrane materials functionalized with adenine and adenosine monophosphate

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Published On ::

Green Chem., 2020, 22,2426-2433
DOI: 10.1039/C9GC04104D, Paper
Guanglei Zhao, Yuanyuan Chen, Xiao-Feng Li, Sihan Zhang, Yuanqiu Situ
A successful strategy to prepare novel proton-conductive chitosan membrane biomaterials functionalized with adenine and adenosine monophosphate via a one-pot grafting procedure.
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A facile solution-phase synthetic approach for constructing phenol-based porous organic cages and covalent organic frameworks

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Green Chem., 2020, 22,2498-2504
DOI: 10.1039/C9GC04033A, Paper
Lei Zhang, Rongran Liang, Cheng Hang, Haiying Wang, Lin Sun, Lei Xu, Dairong Liu, Zhenyi Zhang, Xingmin Zhang, Feifan Chang, Shengyu Zhao, Wei Huang
A general solution-phase synthetic strategy is developed to construct both porous organic cages (POCs) and covalent organic frameworks (COFs) by simply stirring and heating organic solvent/water solutions of aldehydes and amines in the presence of MOH (M = Na, K, and Cs).
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Upgrading 1-butanol to unsaturated, carbonyl and aromatic compounds: a new synthesis approach to produce important organic building blocks

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Green Chem., 2020, 22,2365-2369
DOI: 10.1039/D0GC00254B, Communication
Jorge Mora Vargas, Luiz Henrique Tofaneli Morelato, Julieth Orduna Ortega, Mauricio Boscolo, Gustavo Metzker
Conversion of 1-butanol into added-value organic building blocks was achieved using fixed-bed flow reactor and Cu-based catalyst at 550 and 600 °C with and without methanol as addictive.
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A non-phosgene process for bioderived polycarbonate with high molecular weight and advanced property profile synthesized using amino acid ionic liquids as catalysts

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Green Chem., 2020, 22,2534-2542
DOI: 10.1039/D0GC00265H, Paper
Zhencai Zhang, Fei Xu, Yaqin Zhang, Chenhao Li, Hongyan He, Zifeng Yang, Zengxi Li
Bio-based polycarbonate with high molecular weight and advanced property profile was synthesized using amino acid ionic liquids as catalysts.
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Hierarchically porous covalent organic frameworks assembled in ionic liquids for highly effective catalysis of C–C coupling reactions

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Green Chem., 2020, 22,2605-2612
DOI: 10.1039/D0GC00223B, Paper
Jikuan Qiu, Huiyong Wang, Yuling Zhao, Pengxin Guan, Zhiyong Li, Hucheng Zhang, Hongshuai Gao, Suojiang Zhang, Jianji Wang
A simple and environmentally benign strategy was reported for the synthesis of hierarchically porous COFs in ionic liquids, and the obtained materials show highly effective catalytic performance for C–C bond formation reactions.
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Reusable, homogeneous water soluble photoredox catalyzed oxidative dehydrogenation of N-heterocycles in a biphasic system: application to the synthesis of biologically active natural products

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Published On ::

Green Chem., 2020, 22,2575-2587
DOI: 10.1039/D0GC00569J, Paper
S. Srinath, R. Abinaya, Arun Prasanth, M. Mariappan, R. Sridhar, B. Baskar
Herein, a simple and efficient method for the oxidative dehydrogenation (ODH) of tetrahydro-β-carbolines, indolines and (iso)quinolines is described using a reusable, homogeneous cobalt-phthalocyanine photoredox catalyst in a biphasic medium.
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One-pot synthesis of 1,3-butanediol by 1,4-anhydroerythritol hydrogenolysis over a tungsten-modified platinum on silica catalyst

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Published On ::

Green Chem., 2020, 22,2375-2380
DOI: 10.1039/D0GC00244E, Communication
Lujie Liu, Takehiro Asano, Yoshinao Nakagawa, Masazumi Tamura, Keiichi Tomishige
Chemical production of 1,3-butanediol from biomass-derived compounds was first reported by 1,4-anhydroerythritol hydrogenolysis over a Pt–WOx/SiO2 catalyst.
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Using dialkyl amide via forming hydrophobic deep eutectic solvents to separate citric acid from fermentation broth

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Green Chem., 2020, 22,2526-2533
DOI: 10.1039/C9GC04401A, Paper
Lijuan Liu, Qifeng Wei, Yong Zhou, Xiulian Ren
The separation of citric acids was realized by utilizing hydrophobic deep eutectic solvents (DESs), which were formed by using N,N-dibutylacetamide as a hydrogen acceptor and citric acid as the hydrogen bond.
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Mechanochemical synthesis of mixed metal, mixed linker, glass-forming metal–organic frameworks

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Green Chem., 2020, 22,2505-2512
DOI: 10.1039/D0GC00546K, Paper
Michael F. Thorne, María Laura Ríos Gómez, Alice M. Bumstead, Shichun Li, Thomas D. Bennett
Methods to produce glass forming metal–organic frameworks (MOFs) rely on solvothermal syntheses which have high energy requirements, low yields and large teratogenic solvent usage. We present mechanochemical methods to overcome these issues.
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Evaluating lignin valorization via pyrolysis and vapor-phase hydrodeoxygenation for production of aromatics and alkenes

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Published On ::

Green Chem., 2020, 22,2513-2525
DOI: 10.1039/C9GC04245H, Paper
Open Access
Alireza Saraeian, Alvina Aui, Yu Gao, Mark M. Wright, Marcus Foston, Brent H. Shanks
Lignin valorization to chemicals is an important component of creating economically viable biofuels production from lignocellulosic biomass.
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Improving process efficiency of gold-catalyzed hydration of alkynes: merging catalysis with membrane separation

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Green Chem., 2020, 22,2598-2604
DOI: 10.1039/D0GC00498G, Paper
Tahani A. C. A. Bayrakdar, Fady Nahra, Oihane Zugazua, Lies Eykens, Dominic Ormerod, Steven P. Nolan
In this report, we investigate the integration of a membrane separation protocol in line with the gold-catalyzed hydration of alkynes.
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Introducing deep eutectic solvents as flux boosting and surface cleaning agents for thin film composite polyamide membranes

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Green Chem., 2020, 22,2381-2387
DOI: 10.1039/D0GC00762E, Communication
Nidhi Maalige R., Sweedal A. Dsouza, Matheus M. Pereira, Veerababu Polisetti, Dibyendu Mondal, Sanna Kotrappanavar Nataraj
This study introduced DESs as versatile and multi-tasking agents to modify the surface roughness and wettability of a TFC-PA membrane to boost the permeate flux rate and they also proved to be cleaning agents for organically fouled TFC-PA membranes.
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Scalable synthesis of hydroxymethyl alkylfuranoates as stable 2,5-furandicarboxylic acid precursors

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Green Chem., 2020, 22,2399-2402
DOI: 10.1039/D0GC00770F, Communication
Martin Jæger Pedersen, Arminas Jurys, Christian Marcus Pedersen
Hydroxymethyl furanoic acid and its derivatives have been synthesized in high yields and purity from gluconolactone.
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Visible Light-Induced Aerobic Oxidation of Diarylalkynes to -Diketones Catalyzed by Copper-superoxo at Room Temperature

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Published On ::

Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00975J, Communication
Vaibhav Pramod Charpe, Arunachalam Sagadevan, Kuo Chu Hwang
We have developed the visible light induced simple copper(II) chloride catalyzed the oxidation of diarylacetylenes to -diketones by molecular oxygen at room temperature. The in-situ generated copper(II)-superoxo complex is a...
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Computer-aided Nanotoxicology: Risk Assessment of Metal Oxide Nanoparticles via nano-QSAR

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Green Chem., 2020, Accepted Manuscript
DOI: 10.1039/D0GC00933D, Paper
Jiakai Cao, Yong Pan, Yanting Jiang, Ronghua Qi, Beilei Yuan, Zhenhua Jia, Juncheng Jiang, Qingsheng Wang
Since the applications of nanomaterials have been expanded to serve as a therapeutic methodology, the cytotoxicity accompanying with the nanomaterials drew lots of attention during the therapeutic process. It is...
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